Chapter Semiconductor Optical Amplifier (SOA)–Based Amplification of Intensity-Modulated Optical Pulses — Deterministic Timing Jitter and Pulse Peak Power Equalization Analysis
This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute...
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Alexoudi, T. [verfasserIn] |
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Englisch |
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Erscheinungsort nicht ermittelbar: InTechOpen ; 2015 |
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Open Access Creative Commons ; https://creativecommons.org/licenses/by/3.0 |
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| 520 | |a This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination | ||
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(DE-627)1836473427 (DE-599)KEP077601637 (OCoLC)1286373015 (OAPEN)49135 (EBP)077601637 DE-627 eng DE-627 rda eng THX bicssc Alexoudi, T. verfasserin aut Chapter Semiconductor Optical Amplifier (SOA)–Based Amplification of Intensity-Modulated Optical Pulses — Deterministic Timing Jitter and Pulse Peak Power Equalization Analysis [Erscheinungsort nicht ermittelbar] InTechOpen 2015 1 Online-Ressource Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Open Access Unrestricted online access star This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination Creative Commons https://creativecommons.org/licenses/by/3.0 cc English Alternative & renewable energy sources & technology Kanellos, G.T oth Dris, S. oth Kalavrouziotis, D. oth Bakopoulos, P. oth Miliou, A. oth Pleros, N. oth https://library.oapen.org/bitstream/id/04269b12-8bf2-4ad4-a0b7-05bedbeaf94d/49482.pdf X:OAPEN Verlag kostenfrei https://library.oapen.org/handle/20.500.12657/49135 X:OAPEN Verlag kostenfrei ZDB-94-OAL GBV_ILN_22 ISIL_DE-18 SYSFLAG_1 GBV_KXP GBV_ILN_23 ISIL_DE-830 GBV_ILN_30 ISIL_DE-104 GBV_ILN_31 ISIL_DE-27 GBV_ILN_34 ISIL_DE-18-302 GBV_ILN_39 ISIL_DE-547 GBV_ILN_40 ISIL_DE-7 GBV_ILN_63 ISIL_DE-Wim2 GBV_ILN_65 ISIL_DE-3 GBV_ILN_70 ISIL_DE-89 GBV_ILN_72 ISIL_DE-35 GBV_ILN_95 ISIL_DE-542 GBV_ILN_110 ISIL_DE-Luen4 GBV_ILN_136 ISIL_DE-Wis1 GBV_ILN_147 ISIL_DE-Fl3 GBV_ILN_161 ISIL_DE-960 GBV_ILN_187 ISIL_DE-Ki95 GBV_ILN_213 ISIL_DE-551 GBV_ILN_230 ISIL_DE-552 GBV_ILN_283 ISIL_DE-Ha163 GBV_ILN_293 ISIL_DE-960-3 GBV_ILN_370 ISIL_DE-1373 GBV_ILN_603 ISIL_DE-B1556 GBV_ILN_808 GBV_ILN_2403 ISIL_DE-LFER BO 22 01 0018 4280129770 OLR-ZDB-94-OAL OAPEN Library zu 01-03-23 23 01 0830 4280681856 OLR-OAPEN f z 01-03-23 30 01 0104 4281042539 GBV-OAPEN z 01-03-23 31 01 0027 4280324530 z 01-03-23 34 01 3551 4278880057 OLR-OAPEN zi002 01-03-23 39 01 0547 4281233776 GBV-OAPEN ke 01-03-23 40 01 0007 4279948542 OLR-OAPEN xsn 01-03-23 63 01 3401 4281615709 E-Books LF GBV-OAPEN z 01-03-23 65 01 0003 428186556X OLR-OAPEN z 01-03-23 70 01 0089 4280502870 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 72 01 0035 4278702663 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 95 01 3095 4343230430 OLR-OAL Vervielfältigungen (z.B. 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(DE-627)1836473427 (DE-599)KEP077601637 (OCoLC)1286373015 (OAPEN)49135 (EBP)077601637 DE-627 eng DE-627 rda eng THX bicssc Alexoudi, T. verfasserin aut Chapter Semiconductor Optical Amplifier (SOA)–Based Amplification of Intensity-Modulated Optical Pulses — Deterministic Timing Jitter and Pulse Peak Power Equalization Analysis [Erscheinungsort nicht ermittelbar] InTechOpen 2015 1 Online-Ressource Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Open Access Unrestricted online access star This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination Creative Commons https://creativecommons.org/licenses/by/3.0 cc English Alternative & renewable energy sources & technology Kanellos, G.T oth Dris, S. oth Kalavrouziotis, D. oth Bakopoulos, P. oth Miliou, A. oth Pleros, N. oth https://library.oapen.org/bitstream/id/04269b12-8bf2-4ad4-a0b7-05bedbeaf94d/49482.pdf X:OAPEN Verlag kostenfrei https://library.oapen.org/handle/20.500.12657/49135 X:OAPEN Verlag kostenfrei ZDB-94-OAL GBV_ILN_22 ISIL_DE-18 SYSFLAG_1 GBV_KXP GBV_ILN_23 ISIL_DE-830 GBV_ILN_30 ISIL_DE-104 GBV_ILN_31 ISIL_DE-27 GBV_ILN_34 ISIL_DE-18-302 GBV_ILN_39 ISIL_DE-547 GBV_ILN_40 ISIL_DE-7 GBV_ILN_63 ISIL_DE-Wim2 GBV_ILN_65 ISIL_DE-3 GBV_ILN_70 ISIL_DE-89 GBV_ILN_72 ISIL_DE-35 GBV_ILN_95 ISIL_DE-542 GBV_ILN_110 ISIL_DE-Luen4 GBV_ILN_136 ISIL_DE-Wis1 GBV_ILN_147 ISIL_DE-Fl3 GBV_ILN_161 ISIL_DE-960 GBV_ILN_187 ISIL_DE-Ki95 GBV_ILN_213 ISIL_DE-551 GBV_ILN_230 ISIL_DE-552 GBV_ILN_283 ISIL_DE-Ha163 GBV_ILN_293 ISIL_DE-960-3 GBV_ILN_370 ISIL_DE-1373 GBV_ILN_603 ISIL_DE-B1556 GBV_ILN_808 GBV_ILN_2403 ISIL_DE-LFER BO 22 01 0018 4280129770 OLR-ZDB-94-OAL OAPEN Library zu 01-03-23 23 01 0830 4280681856 OLR-OAPEN f z 01-03-23 30 01 0104 4281042539 GBV-OAPEN z 01-03-23 31 01 0027 4280324530 z 01-03-23 34 01 3551 4278880057 OLR-OAPEN zi002 01-03-23 39 01 0547 4281233776 GBV-OAPEN ke 01-03-23 40 01 0007 4279948542 OLR-OAPEN xsn 01-03-23 63 01 3401 4281615709 E-Books LF GBV-OAPEN z 01-03-23 65 01 0003 428186556X OLR-OAPEN z 01-03-23 70 01 0089 4280502870 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 72 01 0035 4278702663 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 95 01 3095 4343230430 OLR-OAL Vervielfältigungen (z.B. Kopien, Downloads) sind nur von einzelnen Kapiteln oder Seiten und nur zum eigenen wissenschaftlichen Gebrauch erlaubt. Die Weitergabe an Dritte sowie systematisches Downloaden sind untersagt. z 24-06-23 110 01 3110 4281418776 OLR-GBV-OAPEN Open Access z 01-03-23 136 01 3526 4279589615 OLR-OAPEN z 01-03-23 147 01 3528 428206417X OLR-OAPEN frei verfügbar für Europa-Universität Flensburg, Hochschule Flensburg und Zentrale Hochschulbibliothek Vervielfältigungen (z.B. Kopien, Downloads) sind nur von einzelnen Kapiteln oder Seiten und nur zum eigenen wissenschaftlichen Gebrauch erlaubt. Die Weitergabe an Dritte sowie systematisches Downloaden sind untersagt. z 01-03-23 161 01 0960 4278136471 OLR-OAPEN OAPEN Online Library Open Access eBook z 28-02-23 187 01 3520 4278521219 JSTOR Open Access eBook z 28-02-23 213 01 0551 4279235228 OLR-OAPEN OAPEN Online Library Open Access eBook z 01-03-23 230 01 0552 4279412405 OLR-OAPEN OAPEN Online Library Open Access eBook z 01-03-23 283 01 3283 4279771316 OLR-OAL z 01-03-23 293 01 3293 4278315430 OLR-OAPEN OAPEN Online Library Open Access eBook z 28-02-23 370 01 4370 4279057796 OLR-FREE Kostenloser Zugriff z 01-03-23 603 01 4603 427795846X OLR-OAPEN Bitte beachten Sie die Nutzungsbedingungen und Copyright-Bestimmungen des Verlages/Herausgebers. z 28-02-23 808 01 4808 428086084X OLR-OAPEN OAPEN Library zg 01-03-23 2403 01 DE-LFER 4307811763 00 --%%-- --%%-- n --%%-- l01 12-04-23 22 01 0018 Volltextzugang https://library.oapen.org/handle/20.500.12657/49135 23 01 0830 https://library.oapen.org/handle/20.500.12657/49135 30 01 0104 Open Access https://library.oapen.org/handle/20.500.12657/49135 31 01 0027 eBook GBV-OAPEN https://library.oapen.org/handle/20.500.12657/49135 34 01 3551 OpenAccess https://library.oapen.org/handle/20.500.12657/49135 40 01 0007 Volltext, Open Access https://library.oapen.org/handle/20.500.12657/49135 63 01 3401 E-Book https://library.oapen.org/handle/20.500.12657/49135 65 01 0003 Open Access https://library.oapen.org/handle/20.500.12657/49135 65 01 0003 Dieser Titel ist Teil einer Datenbank http://www.bibliothek.uni-regensburg.de/dbinfo/detail.php?titel_id=10728&bib_id=ulb_hal 70 01 0089 https://library.oapen.org/handle/20.500.12657/49135 LF 72 01 0035 https://library.oapen.org/handle/20.500.12657/49135 95 01 3095 https://library.oapen.org/handle/20.500.12657/49135 110 01 3110 Open Access https://library.oapen.org/handle/20.500.12657/49135 136 01 3526 Open Access https://library.oapen.org/handle/20.500.12657/49135 147 01 3528 https://library.oapen.org/handle/20.500.12657/49135 161 01 0960 https://library.oapen.org/handle/20.500.12657/49135 LF 187 01 3520 https://library.oapen.org/handle/20.500.12657/49135 213 01 0551 https://library.oapen.org/handle/20.500.12657/49135 230 01 0552 https://library.oapen.org/handle/20.500.12657/49135 283 01 3283 https://library.oapen.org/handle/20.500.12657/49135 293 01 3293 https://library.oapen.org/handle/20.500.12657/49135 LF 370 01 4370 https://library.oapen.org/handle/20.500.12657/49135 603 01 4603 https://library.oapen.org/handle/20.500.12657/49135 808 01 4808 Volltextzugang https://library.oapen.org/handle/20.500.12657/49135 2403 01 DE-LFER https://library.oapen.org/bitstream/id/04269b12-8bf2-4ad4-a0b7-05bedbeaf94d/49482.pdf 31 01 0027 00 eBook GBV-OAPEN 22 01 0018 OLR-ZDB-94-OAL 23 01 0830 OLR-OAPEN 30 01 0104 GBV-OAPEN 34 01 3551 OLR-OAPEN 39 01 0547 GBV-OAPEN 39 01 0547 LF 40 01 0007 OLR-OAPEN 63 01 3401 E-Books LF GBV-OAPEN 65 01 0003 OLR-OAPEN 70 01 0089 OLR-OAPEN-OA 72 01 0035 OLR-OAPEN-OA 95 01 3095 OLR-OAL 110 01 3110 OLR-GBV-OAPEN 136 01 3526 OLR-OAPEN 147 01 3528 OLR-OAPEN 161 01 0960 OLR-OAPEN 213 01 0551 OLR-OAPEN 230 01 0552 OLR-OAPEN 283 01 3283 OLR-OAL 293 01 3293 OLR-OAPEN 370 01 4370 OLR-FREE 370 01 4370 olr-ebook GBV-OAPEN 603 01 4603 OLR-OAPEN 808 01 4808 OLR-OAPEN |
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(DE-627)1836473427 (DE-599)KEP077601637 (OCoLC)1286373015 (OAPEN)49135 (EBP)077601637 DE-627 eng DE-627 rda eng THX bicssc Alexoudi, T. verfasserin aut Chapter Semiconductor Optical Amplifier (SOA)–Based Amplification of Intensity-Modulated Optical Pulses — Deterministic Timing Jitter and Pulse Peak Power Equalization Analysis [Erscheinungsort nicht ermittelbar] InTechOpen 2015 1 Online-Ressource Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Open Access Unrestricted online access star This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination Creative Commons https://creativecommons.org/licenses/by/3.0 cc English Alternative & renewable energy sources & technology Kanellos, G.T oth Dris, S. oth Kalavrouziotis, D. oth Bakopoulos, P. oth Miliou, A. oth Pleros, N. oth https://library.oapen.org/bitstream/id/04269b12-8bf2-4ad4-a0b7-05bedbeaf94d/49482.pdf X:OAPEN Verlag kostenfrei https://library.oapen.org/handle/20.500.12657/49135 X:OAPEN Verlag kostenfrei ZDB-94-OAL GBV_ILN_22 ISIL_DE-18 SYSFLAG_1 GBV_KXP GBV_ILN_23 ISIL_DE-830 GBV_ILN_30 ISIL_DE-104 GBV_ILN_31 ISIL_DE-27 GBV_ILN_34 ISIL_DE-18-302 GBV_ILN_39 ISIL_DE-547 GBV_ILN_40 ISIL_DE-7 GBV_ILN_63 ISIL_DE-Wim2 GBV_ILN_65 ISIL_DE-3 GBV_ILN_70 ISIL_DE-89 GBV_ILN_72 ISIL_DE-35 GBV_ILN_95 ISIL_DE-542 GBV_ILN_110 ISIL_DE-Luen4 GBV_ILN_136 ISIL_DE-Wis1 GBV_ILN_147 ISIL_DE-Fl3 GBV_ILN_161 ISIL_DE-960 GBV_ILN_187 ISIL_DE-Ki95 GBV_ILN_213 ISIL_DE-551 GBV_ILN_230 ISIL_DE-552 GBV_ILN_283 ISIL_DE-Ha163 GBV_ILN_293 ISIL_DE-960-3 GBV_ILN_370 ISIL_DE-1373 GBV_ILN_603 ISIL_DE-B1556 GBV_ILN_808 GBV_ILN_2403 ISIL_DE-LFER BO 22 01 0018 4280129770 OLR-ZDB-94-OAL OAPEN Library zu 01-03-23 23 01 0830 4280681856 OLR-OAPEN f z 01-03-23 30 01 0104 4281042539 GBV-OAPEN z 01-03-23 31 01 0027 4280324530 z 01-03-23 34 01 3551 4278880057 OLR-OAPEN zi002 01-03-23 39 01 0547 4281233776 GBV-OAPEN ke 01-03-23 40 01 0007 4279948542 OLR-OAPEN xsn 01-03-23 63 01 3401 4281615709 E-Books LF GBV-OAPEN z 01-03-23 65 01 0003 428186556X OLR-OAPEN z 01-03-23 70 01 0089 4280502870 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 72 01 0035 4278702663 OLR-OAPEN-OA OAPEN Online Library Open Access eBook z 01-03-23 95 01 3095 4343230430 OLR-OAL Vervielfältigungen (z.B. Kopien, Downloads) sind nur von einzelnen Kapiteln oder Seiten und nur zum eigenen wissenschaftlichen Gebrauch erlaubt. Die Weitergabe an Dritte sowie systematisches Downloaden sind untersagt. z 24-06-23 110 01 3110 4281418776 OLR-GBV-OAPEN Open Access z 01-03-23 136 01 3526 4279589615 OLR-OAPEN z 01-03-23 147 01 3528 428206417X OLR-OAPEN frei verfügbar für Europa-Universität Flensburg, Hochschule Flensburg und Zentrale Hochschulbibliothek Vervielfältigungen (z.B. Kopien, Downloads) sind nur von einzelnen Kapiteln oder Seiten und nur zum eigenen wissenschaftlichen Gebrauch erlaubt. 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Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. 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This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination |
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This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination |
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This chapter presents the fate of the charge carriers from the moment of its photogeneration in the perovskite to injection and transport into electrodes. Time-resolved electrical measurement techniques, terahertz (THz) spectroscopy and microwave (MW) conductivity, are primarily used to deconvolute ultrafast processes and to directly access behavior of charged species from the ps to µs timescales. Transient absorption and photoluminescence spectroscopy were also utilized to gain insight on carrier population dynamics and radiatively recombining charges. Photogenerated charged species were converted into highly mobile charges (µe = 12.5 cm2V-1s-1 and µh = 7.5 cm2V-1s-1) almost instantaneously (< 0.2 ps), while the remaining loosely bounded excitons dissociate into mobile charges after 2-3 ps. This high mobility is maintained for at least 1 ns as obtained by THz spectroscopy, while its lifetime is at least few tens of µs as measured by the MW conductivity technique. Lowering the temperature increases carrier mobilities with T-1.6.Dependence and a 75 meV barrier energy is required for temperature-activated recombination. Finally, injection of hole from MAPbI3 to Spiro-OMeTAD was found to be ultrafast and the state and population of dark holes dictate its recombination |
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| score |
7.1641693 |