10 years long-term assessment on characterizing spatiotemporal trend and source apportionment of metal(loid)s in terrestrial soils along the west coast of South Korea

Long-term trends in the spatial distributions and sources of metal(loid)s in soils adjacent to the west coastal areas of South Korea have been systematically investigated for 10 years (2010–2019). Monitoring in 17 sites clearly showed site- and region-specific distributions, being associated with la...
Ausführliche Beschreibung

Long-term trends in the spatial distributions and sources of metal(loid)s in soils adjacent to the west coastal areas of South Korea have been systematically investigated for 10 years (2010–2019). Monitoring in 17 sites clearly showed site- and region-specific distributions, being associated with land use type (significant differences, as road > agriculture > wild) (P 0.05). The degree of metal(loid)s contamination compared to the background levels was identified in the order of Pb > Zn > Cr > Cu > As>Cd > Ni > Hg, with the contaminated hotspots mostly in LS or GG. The potential ecological risk was evidenced for Cd and Hg, but such a trend was temporally irregular over the years, indicating site-specificity. The sources of metal(loid)s were carefully determined as natural (20%), fuel combustion & agricultural pollution (43%), and vehicular emissions (37%) using the Positive Matrix Factorization model. The relative contribution of each source to contamination over the last decade was found to be similar, supporting that site-dependent lesser variation in metal(loid)s contamination in the coastal areas of South Korea. Overall, the distribution of metal(loid)s in the soil near the west coastal areas over the last decade largely depended on land use activities, and contamination degree was associated with non-point sources, such as transportation and fuel combustion. Ausführliche Beschreibung