Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells
Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesi...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wang, Changlei [verfasserIn] Xiao, Chuanxiao [verfasserIn] Constantinou, Iordania [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
September 6, 2017 |
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| Schlagwörter: |
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| Anmerkung: |
Gesehen am 20.11.2018 |
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| Umfang: |
9 |
| Übergeordnetes Werk: |
Enthalten in: Advanced energy materials - Weinheim : Wiley-VCH, 2011, 7(2017), 17, Artikel-ID 1700414 |
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| Übergeordnetes Werk: |
volume:7 ; year:2017 ; number:17 ; elocationid:1700414 ; extent:9 |
| Links: |
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| DOI / URN: |
10.1002/aenm.201700414 |
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| Katalog-ID: |
1583875700 |
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| 245 | 1 | 0 | |a Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells |c Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan |
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| 520 | |a Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. | ||
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10.1002/aenm.201700414 doi (DE-627)1583875700 (DE-576)513875700 (DE-599)BSZ513875700 (OCoLC)1341023918 DE-627 ger DE-627 rda eng Wang, Changlei verfasserin (DE-588)1171844344 (DE-627)1040728081 (DE-576)513873236 aut Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan September 6, 2017 9 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Gesehen am 20.11.2018 Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. hysteresis Kelvin probe force microscopy perovskite solar cells post annealing Xiao, Chuanxiao verfasserin (DE-588)1171844425 (DE-627)1040728154 (DE-576)513873198 aut Constantinou, Iordania verfasserin (DE-588)1171843984 (DE-627)1040727735 (DE-576)513872663 aut Enthalten in Advanced energy materials Weinheim : Wiley-VCH, 2011 7(2017), 17, Artikel-ID 1700414 Online-Ressource (DE-627)647301024 (DE-600)2594556-7 (DE-576)338208070 1614-6840 nnns volume:7 year:2017 number:17 elocationid:1700414 extent:9 http://dx.doi.org/10.1002/aenm.201700414 Verlag Resolving-System Volltext https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201700414 Verlag Volltext GBV_USEFLAG_U GBV_ILN_2013 ISIL_DE-16-250 SYSFLAG_1 GBV_KXP GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_266 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 7 2017 17 1700414 9 2013 01 DE-16-250 3032779456 00 --%%-- --%%-- --%%-- --%%-- l01 20-11-18 2013 01 DE-16-250 00 s hd2017 2013 01 DE-16-250 01 s (DE-627)1410508463 wissenschaftlicher Artikel (Zeitschrift) 2013 01 DE-16-250 02 s per_17 2013 01 DE-16-250 03 s s_9 2013 01 DE-16-250 04 p (DE-627)1583875670 Constantinou, Iordania 2013 01 DE-16-250 04 k (DE-627)1416733221 Zentrum für Molekulare Biologie (ZMBH) 2013 01 DE-16-250 04 s (DE-627)1410501914 Verfasser 2013 01 DE-16-250 04 s pos_8 |
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10.1002/aenm.201700414 doi (DE-627)1583875700 (DE-576)513875700 (DE-599)BSZ513875700 (OCoLC)1341023918 DE-627 ger DE-627 rda eng Wang, Changlei verfasserin (DE-588)1171844344 (DE-627)1040728081 (DE-576)513873236 aut Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan September 6, 2017 9 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Gesehen am 20.11.2018 Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. hysteresis Kelvin probe force microscopy perovskite solar cells post annealing Xiao, Chuanxiao verfasserin (DE-588)1171844425 (DE-627)1040728154 (DE-576)513873198 aut Constantinou, Iordania verfasserin (DE-588)1171843984 (DE-627)1040727735 (DE-576)513872663 aut Enthalten in Advanced energy materials Weinheim : Wiley-VCH, 2011 7(2017), 17, Artikel-ID 1700414 Online-Ressource (DE-627)647301024 (DE-600)2594556-7 (DE-576)338208070 1614-6840 nnns volume:7 year:2017 number:17 elocationid:1700414 extent:9 http://dx.doi.org/10.1002/aenm.201700414 Verlag Resolving-System Volltext https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201700414 Verlag Volltext GBV_USEFLAG_U GBV_ILN_2013 ISIL_DE-16-250 SYSFLAG_1 GBV_KXP GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_266 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 7 2017 17 1700414 9 2013 01 DE-16-250 3032779456 00 --%%-- --%%-- --%%-- --%%-- l01 20-11-18 2013 01 DE-16-250 00 s hd2017 2013 01 DE-16-250 01 s (DE-627)1410508463 wissenschaftlicher Artikel (Zeitschrift) 2013 01 DE-16-250 02 s per_17 2013 01 DE-16-250 03 s s_9 2013 01 DE-16-250 04 p (DE-627)1583875670 Constantinou, Iordania 2013 01 DE-16-250 04 k (DE-627)1416733221 Zentrum für Molekulare Biologie (ZMBH) 2013 01 DE-16-250 04 s (DE-627)1410501914 Verfasser 2013 01 DE-16-250 04 s pos_8 |
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10.1002/aenm.201700414 doi (DE-627)1583875700 (DE-576)513875700 (DE-599)BSZ513875700 (OCoLC)1341023918 DE-627 ger DE-627 rda eng Wang, Changlei verfasserin (DE-588)1171844344 (DE-627)1040728081 (DE-576)513873236 aut Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan September 6, 2017 9 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Gesehen am 20.11.2018 Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. hysteresis Kelvin probe force microscopy perovskite solar cells post annealing Xiao, Chuanxiao verfasserin (DE-588)1171844425 (DE-627)1040728154 (DE-576)513873198 aut Constantinou, Iordania verfasserin (DE-588)1171843984 (DE-627)1040727735 (DE-576)513872663 aut Enthalten in Advanced energy materials Weinheim : Wiley-VCH, 2011 7(2017), 17, Artikel-ID 1700414 Online-Ressource (DE-627)647301024 (DE-600)2594556-7 (DE-576)338208070 1614-6840 nnns volume:7 year:2017 number:17 elocationid:1700414 extent:9 http://dx.doi.org/10.1002/aenm.201700414 Verlag Resolving-System Volltext https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201700414 Verlag Volltext GBV_USEFLAG_U GBV_ILN_2013 ISIL_DE-16-250 SYSFLAG_1 GBV_KXP GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_266 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 7 2017 17 1700414 9 2013 01 DE-16-250 3032779456 00 --%%-- --%%-- --%%-- --%%-- l01 20-11-18 2013 01 DE-16-250 00 s hd2017 2013 01 DE-16-250 01 s (DE-627)1410508463 wissenschaftlicher Artikel (Zeitschrift) 2013 01 DE-16-250 02 s per_17 2013 01 DE-16-250 03 s s_9 2013 01 DE-16-250 04 p (DE-627)1583875670 Constantinou, Iordania 2013 01 DE-16-250 04 k (DE-627)1416733221 Zentrum für Molekulare Biologie (ZMBH) 2013 01 DE-16-250 04 s (DE-627)1410501914 Verfasser 2013 01 DE-16-250 04 s pos_8 |
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10.1002/aenm.201700414 doi (DE-627)1583875700 (DE-576)513875700 (DE-599)BSZ513875700 (OCoLC)1341023918 DE-627 ger DE-627 rda eng Wang, Changlei verfasserin (DE-588)1171844344 (DE-627)1040728081 (DE-576)513873236 aut Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan September 6, 2017 9 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Gesehen am 20.11.2018 Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. hysteresis Kelvin probe force microscopy perovskite solar cells post annealing Xiao, Chuanxiao verfasserin (DE-588)1171844425 (DE-627)1040728154 (DE-576)513873198 aut Constantinou, Iordania verfasserin (DE-588)1171843984 (DE-627)1040727735 (DE-576)513872663 aut Enthalten in Advanced energy materials Weinheim : Wiley-VCH, 2011 7(2017), 17, Artikel-ID 1700414 Online-Ressource (DE-627)647301024 (DE-600)2594556-7 (DE-576)338208070 1614-6840 nnns volume:7 year:2017 number:17 elocationid:1700414 extent:9 http://dx.doi.org/10.1002/aenm.201700414 Verlag Resolving-System Volltext https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201700414 Verlag Volltext GBV_USEFLAG_U GBV_ILN_2013 ISIL_DE-16-250 SYSFLAG_1 GBV_KXP GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_266 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 7 2017 17 1700414 9 2013 01 DE-16-250 3032779456 00 --%%-- --%%-- --%%-- --%%-- l01 20-11-18 2013 01 DE-16-250 00 s hd2017 2013 01 DE-16-250 01 s (DE-627)1410508463 wissenschaftlicher Artikel (Zeitschrift) 2013 01 DE-16-250 02 s per_17 2013 01 DE-16-250 03 s s_9 2013 01 DE-16-250 04 p (DE-627)1583875670 Constantinou, Iordania 2013 01 DE-16-250 04 k (DE-627)1416733221 Zentrum für Molekulare Biologie (ZMBH) 2013 01 DE-16-250 04 s (DE-627)1410501914 Verfasser 2013 01 DE-16-250 04 s pos_8 |
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10.1002/aenm.201700414 doi (DE-627)1583875700 (DE-576)513875700 (DE-599)BSZ513875700 (OCoLC)1341023918 DE-627 ger DE-627 rda eng Wang, Changlei verfasserin (DE-588)1171844344 (DE-627)1040728081 (DE-576)513873236 aut Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan September 6, 2017 9 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Gesehen am 20.11.2018 Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. hysteresis Kelvin probe force microscopy perovskite solar cells post annealing Xiao, Chuanxiao verfasserin (DE-588)1171844425 (DE-627)1040728154 (DE-576)513873198 aut Constantinou, Iordania verfasserin (DE-588)1171843984 (DE-627)1040727735 (DE-576)513872663 aut Enthalten in Advanced energy materials Weinheim : Wiley-VCH, 2011 7(2017), 17, Artikel-ID 1700414 Online-Ressource (DE-627)647301024 (DE-600)2594556-7 (DE-576)338208070 1614-6840 nnns volume:7 year:2017 number:17 elocationid:1700414 extent:9 http://dx.doi.org/10.1002/aenm.201700414 Verlag Resolving-System Volltext https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201700414 Verlag Volltext GBV_USEFLAG_U GBV_ILN_2013 ISIL_DE-16-250 SYSFLAG_1 GBV_KXP GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_266 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 7 2017 17 1700414 9 2013 01 DE-16-250 3032779456 00 --%%-- --%%-- --%%-- --%%-- l01 20-11-18 2013 01 DE-16-250 00 s hd2017 2013 01 DE-16-250 01 s (DE-627)1410508463 wissenschaftlicher Artikel (Zeitschrift) 2013 01 DE-16-250 02 s per_17 2013 01 DE-16-250 03 s s_9 2013 01 DE-16-250 04 p (DE-627)1583875670 Constantinou, Iordania 2013 01 DE-16-250 04 k (DE-627)1416733221 Zentrum für Molekulare Biologie (ZMBH) 2013 01 DE-16-250 04 s (DE-627)1410501914 Verfasser 2013 01 DE-16-250 04 s pos_8 |
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Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells Changlei Wang, Chuanxiao Xiao, Yue Yu, Dewei Zhao, Rasha A. Awni, Corey R. Grice, Kiran Ghimire, Iordania Constantinou, Weiqiang Liao, Alexander J. Cimaroli, Pei Liu, Jing Chen, Nikolas J. Podraza, Chun-Sheng Jiang, Mowafak M. Al‐Jassim, Xingzhong Zhao and Yanfa Yan |
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understanding and eliminating hysteresis for highly efficient planar perovskite solar cells |
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Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells |
| abstract |
Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. Gesehen am 20.11.2018 |
| abstractGer |
Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. Gesehen am 20.11.2018 |
| abstract_unstemmed |
Through detailed device characterization using cross-sectional Kelvin probe force microscopy (KPFM) and trap density of states measurements, we identify that the J-V hysteresis seen in planar organic-inorganic hybrid perovskite solar cells (PVSCs) using SnO2 electron selective layers (ESLs) synthesized by low-temperature plasma-enhanced atomic-layer deposition (PEALD) method is mainly caused by the imbalanced charge transportation between the ESL/perovskite and the hole selective layer/perovskite interfaces. We find that this charge transportation imbalance is originated from the poor electrical conductivity of the low-temperature PEALD SnO2 ESL. We further discover that a facile low-temperature thermal annealing of SnO2 ESLs can effectively improve the electrical mobility of low-temperature PEALD SnO2 ESLs and consequently significantly reduce or even eliminate the J-V hysteresis. With the reduction of J-V hysteresis and optimization of deposition process, planar PVSCs with stabilized output powers up to 20.3% are achieved. The results of this study provide insights for further enhancing the efficiency of planar PVSCs. Gesehen am 20.11.2018 |
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Understanding and eliminating hysteresis for highly efficient planar perovskite solar cells |
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7.3984947 |