CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation

Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on se...
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Autor*in:	Andrea Jouve [verfasserIn] Stefano Cattaneo [verfasserIn] Sofia Capelli [verfasserIn] Marta Stucchi [verfasserIn] Claudio Evangelisti [verfasserIn] Alberto Villa [verfasserIn] Laura Prati [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	ruthenium carbon nanofiber functionalization HMF LA hydrogenation

Übergeordnetes Werk:	In: Molecules - MDPI AG, 2003, 24(2019), 2, p 316
Übergeordnetes Werk:	volume:24 ; year:2019 ; number:2, p 316

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/molecules24020316

Katalog-ID:	DOAJ001398148

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520			\|a Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on selectivity was observed (all the catalysts produced selectively gamma-valerolactone (GVL)), the functionalization strongly affected the activity of the reaction. O-containing and N-containing supports presented a higher activity compared to the bare support. On the contrary, in HMF hydrogenation, functionalization of the support did not have a beneficial effect on the activity of a Ru-catalysed reaction with respect to bare support and only CNFs-O behaved similarly to bare CNFs. In fact, when CNFs-N or CNFs-P were used as the supports, a lower activity was observed, as well as a change in selectivity in which the production of ethers (from the reaction with the solvent) greatly increased.
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allfieldsSound	10.3390/molecules24020316 doi (DE-627)DOAJ001398148 (DE-599)DOAJdf19f9b6b41041f48dc756ef584443ec DE-627 ger DE-627 rakwb eng QD241-441 Andrea Jouve verfasserin aut CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on selectivity was observed (all the catalysts produced selectively gamma-valerolactone (GVL)), the functionalization strongly affected the activity of the reaction. O-containing and N-containing supports presented a higher activity compared to the bare support. On the contrary, in HMF hydrogenation, functionalization of the support did not have a beneficial effect on the activity of a Ru-catalysed reaction with respect to bare support and only CNFs-O behaved similarly to bare CNFs. In fact, when CNFs-N or CNFs-P were used as the supports, a lower activity was observed, as well as a change in selectivity in which the production of ethers (from the reaction with the solvent) greatly increased. ruthenium carbon nanofiber functionalization HMF LA hydrogenation Organic chemistry Stefano Cattaneo verfasserin aut Sofia Capelli verfasserin aut Marta Stucchi verfasserin aut Claudio Evangelisti verfasserin aut Alberto Villa verfasserin aut Laura Prati verfasserin aut In Molecules MDPI AG, 2003 24(2019), 2, p 316 (DE-627)311313132 (DE-600)2008644-1 14203049 nnns volume:24 year:2019 number:2, p 316 https://doi.org/10.3390/molecules24020316 kostenfrei https://doaj.org/article/df19f9b6b41041f48dc756ef584443ec kostenfrei http://www.mdpi.com/1420-3049/24/2/316 kostenfrei https://doaj.org/toc/1420-3049 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 24 2019 2, p 316
language	English
source	In Molecules 24(2019), 2, p 316 volume:24 year:2019 number:2, p 316
sourceStr	In Molecules 24(2019), 2, p 316 volume:24 year:2019 number:2, p 316
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	ruthenium carbon nanofiber functionalization HMF LA hydrogenation Organic chemistry
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container_title	Molecules
authorswithroles_txt_mv	Andrea Jouve @@aut@@ Stefano Cattaneo @@aut@@ Sofia Capelli @@aut@@ Marta Stucchi @@aut@@ Claudio Evangelisti @@aut@@ Alberto Villa @@aut@@ Laura Prati @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
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callnumber-first	Q - Science
author	Andrea Jouve
spellingShingle	Andrea Jouve misc QD241-441 misc ruthenium misc carbon misc nanofiber misc functionalization misc HMF misc LA misc hydrogenation misc Organic chemistry CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation
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topic_title	QD241-441 CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation ruthenium carbon nanofiber functionalization HMF LA hydrogenation
topic	misc QD241-441 misc ruthenium misc carbon misc nanofiber misc functionalization misc HMF misc LA misc hydrogenation misc Organic chemistry
topic_unstemmed	misc QD241-441 misc ruthenium misc carbon misc nanofiber misc functionalization misc HMF misc LA misc hydrogenation misc Organic chemistry
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title	CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation
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title_full	CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation
author_sort	Andrea Jouve
journal	Molecules
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author_browse	Andrea Jouve Stefano Cattaneo Sofia Capelli Marta Stucchi Claudio Evangelisti Alberto Villa Laura Prati
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title_sort	cnf-functionalization as versatile tool for tuning activity in cellulose-derived product hydrogenation
callnumber	QD241-441
title_auth	CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation
abstract	Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on selectivity was observed (all the catalysts produced selectively gamma-valerolactone (GVL)), the functionalization strongly affected the activity of the reaction. O-containing and N-containing supports presented a higher activity compared to the bare support. On the contrary, in HMF hydrogenation, functionalization of the support did not have a beneficial effect on the activity of a Ru-catalysed reaction with respect to bare support and only CNFs-O behaved similarly to bare CNFs. In fact, when CNFs-N or CNFs-P were used as the supports, a lower activity was observed, as well as a change in selectivity in which the production of ethers (from the reaction with the solvent) greatly increased.
abstractGer	Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on selectivity was observed (all the catalysts produced selectively gamma-valerolactone (GVL)), the functionalization strongly affected the activity of the reaction. O-containing and N-containing supports presented a higher activity compared to the bare support. On the contrary, in HMF hydrogenation, functionalization of the support did not have a beneficial effect on the activity of a Ru-catalysed reaction with respect to bare support and only CNFs-O behaved similarly to bare CNFs. In fact, when CNFs-N or CNFs-P were used as the supports, a lower activity was observed, as well as a change in selectivity in which the production of ethers (from the reaction with the solvent) greatly increased.
abstract_unstemmed	Carbon nanofibers (CNFs) have been functionalized by introducing O, N, and P containing groups in order to investigate the effect of support functionalization in Ru catalysed hydroxymethyl furfural (HMF) and levulinic acid (LA) hydrogenation. In the case of HMF, despite the fact that no effect on selectivity was observed (all the catalysts produced selectively gamma-valerolactone (GVL)), the functionalization strongly affected the activity of the reaction. O-containing and N-containing supports presented a higher activity compared to the bare support. On the contrary, in HMF hydrogenation, functionalization of the support did not have a beneficial effect on the activity of a Ru-catalysed reaction with respect to bare support and only CNFs-O behaved similarly to bare CNFs. In fact, when CNFs-N or CNFs-P were used as the supports, a lower activity was observed, as well as a change in selectivity in which the production of ethers (from the reaction with the solvent) greatly increased.
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title_short	CNF-Functionalization as Versatile Tool for Tuning Activity in Cellulose-Derived Product Hydrogenation
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author2	Stefano Cattaneo Sofia Capelli Marta Stucchi Claudio Evangelisti Alberto Villa Laura Prati
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