Gold–Ceria SBA-15-Supported Catalyst for CO Preferential Oxidation: Surface and Reactivity Studies

In this article, the preparation and application of gold and cerium catalysts supported on zirconium-doped mesoporous silica SBA-15 was studied. These materials have been prepared by two different methods and characterized to investigate their textural properties, dispersion of the active phases and...
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Autor*in:	Álvaro Reyes-Carmona [verfasserIn] Aldo Talon [verfasserIn] Elisa Moretti [verfasserIn] Maurizio Lenarda [verfasserIn] Antonio Jiménez-López [verfasserIn] Enrique Rodríguez-Castellón [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2012

Übergeordnetes Werk:	In: Adsorption Science & Technology - SAGE Publications, 2018, 30(2012)
Übergeordnetes Werk:	volume:30 ; year:2012

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc Journal toc

DOI / URN:	10.1260/0263-6174.30.8-9.751

Katalog-ID:	DOAJ00458662X

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callnumber-first	Q - Science
author	Álvaro Reyes-Carmona
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topic_title	QD450-801 Gold–Ceria SBA-15-Supported Catalyst for CO Preferential Oxidation: Surface and Reactivity Studies
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title	Gold–Ceria SBA-15-Supported Catalyst for CO Preferential Oxidation: Surface and Reactivity Studies
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title_sort	gold–ceria sba-15-supported catalyst for co preferential oxidation: surface and reactivity studies
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title_auth	Gold–Ceria SBA-15-Supported Catalyst for CO Preferential Oxidation: Surface and Reactivity Studies
abstract	In this article, the preparation and application of gold and cerium catalysts supported on zirconium-doped mesoporous silica SBA-15 was studied. These materials have been prepared by two different methods and characterized to investigate their textural properties, dispersion of the active phases and oxidation states. Both materials exhibit a marked catalytic activity. The size of the gold nanoparticles is directly related to the CO conversion rate and to the selectivity towards CO 2 exhibiting a strong temperature dependence. An X-ray photoelectron spectroscopic study of the composition and chemical state of the nanoparticles indicates the presence of Au in a metallic state. Transmission electron microscopic micrographs indicate that the best catalyst shows a higher dispersion of Au in spite of its lower gold surface content.
abstractGer	In this article, the preparation and application of gold and cerium catalysts supported on zirconium-doped mesoporous silica SBA-15 was studied. These materials have been prepared by two different methods and characterized to investigate their textural properties, dispersion of the active phases and oxidation states. Both materials exhibit a marked catalytic activity. The size of the gold nanoparticles is directly related to the CO conversion rate and to the selectivity towards CO 2 exhibiting a strong temperature dependence. An X-ray photoelectron spectroscopic study of the composition and chemical state of the nanoparticles indicates the presence of Au in a metallic state. Transmission electron microscopic micrographs indicate that the best catalyst shows a higher dispersion of Au in spite of its lower gold surface content.
abstract_unstemmed	In this article, the preparation and application of gold and cerium catalysts supported on zirconium-doped mesoporous silica SBA-15 was studied. These materials have been prepared by two different methods and characterized to investigate their textural properties, dispersion of the active phases and oxidation states. Both materials exhibit a marked catalytic activity. The size of the gold nanoparticles is directly related to the CO conversion rate and to the selectivity towards CO 2 exhibiting a strong temperature dependence. An X-ray photoelectron spectroscopic study of the composition and chemical state of the nanoparticles indicates the presence of Au in a metallic state. Transmission electron microscopic micrographs indicate that the best catalyst shows a higher dispersion of Au in spite of its lower gold surface content.
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title_short	Gold–Ceria SBA-15-Supported Catalyst for CO Preferential Oxidation: Surface and Reactivity Studies
url	https://doi.org/10.1260/0263-6174.30.8-9.751 https://doaj.org/article/03bc6e905e2a4cb9a5f5838a19c69e00 https://doaj.org/toc/0263-6174 https://doaj.org/toc/2048-4038
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up_date	2024-07-04T00:19:23.180Z
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