Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance

Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchi...
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Autor*in:	Qin Pan [verfasserIn] Aoshuang Li [verfasserIn] Yuanlu Zhang [verfasserIn] Yaping Yang [verfasserIn] Chuanwei Cheng [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	arrays composites hierarchical structure photoanodes photoelectrochemical water spitting

Übergeordnetes Werk:	In: Advanced Science - Wiley, 2015, 7(2020), 3, Seite n/a-n/a
Übergeordnetes Werk:	volume:7 ; year:2020 ; number:3 ; pages:n/a-n/a

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1002/advs.201902235

Katalog-ID:	DOAJ005501806

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520			\|a Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance.
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publishDate	2020
allfields	10.1002/advs.201902235 doi (DE-627)DOAJ005501806 (DE-599)DOAJ57a5fcc6e8c54baf84f40a0708ae7db4 DE-627 ger DE-627 rakwb eng Qin Pan verfasserin aut Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance. arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q Aoshuang Li verfasserin aut Yuanlu Zhang verfasserin aut Yaping Yang verfasserin aut Chuanwei Cheng verfasserin aut In Advanced Science Wiley, 2015 7(2020), 3, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:7 year:2020 number:3 pages:n/a-n/a https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 kostenfrei https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2020 3 n/a-n/a
spelling	10.1002/advs.201902235 doi (DE-627)DOAJ005501806 (DE-599)DOAJ57a5fcc6e8c54baf84f40a0708ae7db4 DE-627 ger DE-627 rakwb eng Qin Pan verfasserin aut Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance. arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q Aoshuang Li verfasserin aut Yuanlu Zhang verfasserin aut Yaping Yang verfasserin aut Chuanwei Cheng verfasserin aut In Advanced Science Wiley, 2015 7(2020), 3, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:7 year:2020 number:3 pages:n/a-n/a https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 kostenfrei https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2020 3 n/a-n/a
allfields_unstemmed	10.1002/advs.201902235 doi (DE-627)DOAJ005501806 (DE-599)DOAJ57a5fcc6e8c54baf84f40a0708ae7db4 DE-627 ger DE-627 rakwb eng Qin Pan verfasserin aut Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance. arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q Aoshuang Li verfasserin aut Yuanlu Zhang verfasserin aut Yaping Yang verfasserin aut Chuanwei Cheng verfasserin aut In Advanced Science Wiley, 2015 7(2020), 3, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:7 year:2020 number:3 pages:n/a-n/a https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 kostenfrei https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2020 3 n/a-n/a
allfieldsGer	10.1002/advs.201902235 doi (DE-627)DOAJ005501806 (DE-599)DOAJ57a5fcc6e8c54baf84f40a0708ae7db4 DE-627 ger DE-627 rakwb eng Qin Pan verfasserin aut Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance. arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q Aoshuang Li verfasserin aut Yuanlu Zhang verfasserin aut Yaping Yang verfasserin aut Chuanwei Cheng verfasserin aut In Advanced Science Wiley, 2015 7(2020), 3, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:7 year:2020 number:3 pages:n/a-n/a https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 kostenfrei https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2020 3 n/a-n/a
allfieldsSound	10.1002/advs.201902235 doi (DE-627)DOAJ005501806 (DE-599)DOAJ57a5fcc6e8c54baf84f40a0708ae7db4 DE-627 ger DE-627 rakwb eng Qin Pan verfasserin aut Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance. arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q Aoshuang Li verfasserin aut Yuanlu Zhang verfasserin aut Yaping Yang verfasserin aut Chuanwei Cheng verfasserin aut In Advanced Science Wiley, 2015 7(2020), 3, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:7 year:2020 number:3 pages:n/a-n/a https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 kostenfrei https://doi.org/10.1002/advs.201902235 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2020 3 n/a-n/a
language	English
source	In Advanced Science 7(2020), 3, Seite n/a-n/a volume:7 year:2020 number:3 pages:n/a-n/a
sourceStr	In Advanced Science 7(2020), 3, Seite n/a-n/a volume:7 year:2020 number:3 pages:n/a-n/a
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	arrays composites hierarchical structure photoanodes photoelectrochemical water spitting Science Q
isfreeaccess_bool	true
container_title	Advanced Science
authorswithroles_txt_mv	Qin Pan @@aut@@ Aoshuang Li @@aut@@ Yuanlu Zhang @@aut@@ Yaping Yang @@aut@@ Chuanwei Cheng @@aut@@
publishDateDaySort_date	2020-01-01T00:00:00Z
hierarchy_top_id	817357777
id	DOAJ005501806
language_de	englisch
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author	Qin Pan
spellingShingle	Qin Pan misc arrays misc composites misc hierarchical structure misc photoanodes misc photoelectrochemical water spitting misc Science misc Q Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance
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topic_title	Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance arrays composites hierarchical structure photoanodes photoelectrochemical water spitting
topic	misc arrays misc composites misc hierarchical structure misc photoanodes misc photoelectrochemical water spitting misc Science misc Q
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title	Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance
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title_full	Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance
author_sort	Qin Pan
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author_browse	Qin Pan Aoshuang Li Yuanlu Zhang Yaping Yang Chuanwei Cheng
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title_sort	rational design of 3d hierarchical ternary sno2/tio2/bivo4 arrays photoanode toward efficient photoelectrochemical performance
title_auth	Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance
abstract	Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance.
abstractGer	Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance.
abstract_unstemmed	Abstract BiVO4 as a promising semiconductor absorber is widely investigated as photoanode in photoelectrochemical water splitting. Herein, the rational design of 3D hierarchical ternary SnO2/TiO2/BiVO4 arrays is reported as photoanode for photoelectrochemical application, in which the SnO2 hierarchically hollow microspheres core/nanosheets shell arrays act as conductive skeletons, while the sandwiched TiO2 and surface BiVO4 are working as hole blocking layer and light absorber, respectively. Arising to the hierarchically ordered structure and synergistic effect between each component in the composite, the ternary SnO2/TiO2/BiVO4 photoanode enables high light harvesting efficiency as well as enhanced charge transport and separation efficiency, yielding a maximum photocurrent density of ≈5.03 mA cm−2 for sulfite oxidation and ≈3.1 mA cm−2 for water oxidation, respectively, measured at 1.23 V versus reversible hydrogen electrode under simulated air mass (AM) 1.5 solar light illumination. The results reveal that electrode design and interface engineering play important roles on the overall PEC performance.
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title_short	Rational Design of 3D Hierarchical Ternary SnO2/TiO2/BiVO4 Arrays Photoanode toward Efficient Photoelectrochemical Performance
url	https://doi.org/10.1002/advs.201902235 https://doaj.org/article/57a5fcc6e8c54baf84f40a0708ae7db4 https://doaj.org/toc/2198-3844
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