Near-ground ozone source attributions and outflow in central eastern China during MTX2006

A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Ausführliche Beschreibung

Gespeichert in:

Autor*in:	J. Li [verfasserIn] Z. Wang [verfasserIn] H. Akimoto [verfasserIn] K. Yamaji [verfasserIn] M. Takigawa [verfasserIn] P. Pochanart [verfasserIn] Y. Liu [verfasserIn] H. Tanimoto [verfasserIn] Y. Kanaya [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2008

Übergeordnetes Werk:	In: Atmospheric Chemistry and Physics - Copernicus Publications, 2003, 8(2008), 24, Seite 7335-7351
Übergeordnetes Werk:	volume:8 ; year:2008 ; number:24 ; pages:7335-7351

Links:	Link aufrufen Link aufrufen Journal toc Journal toc

Katalog-ID:	DOAJ009023720

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700	0		\|a Y. Liu \|e verfasserin \|4 aut
700	0		\|a H. Tanimoto \|e verfasserin \|4 aut
700	0		\|a Y. Kanaya \|e verfasserin \|4 aut
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allfields	(DE-627)DOAJ009023720 (DE-599)DOAJ9f79f1add3fa45cb8cfa395b39bbd2e3 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 J. Li verfasserin aut Near-ground ozone source attributions and outflow in central eastern China during MTX2006 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Physics Chemistry Z. Wang verfasserin aut H. Akimoto verfasserin aut K. Yamaji verfasserin aut M. Takigawa verfasserin aut P. Pochanart verfasserin aut Y. Liu verfasserin aut H. Tanimoto verfasserin aut Y. Kanaya verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 24, Seite 7335-7351 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:24 pages:7335-7351 https://doaj.org/article/9f79f1add3fa45cb8cfa395b39bbd2e3 kostenfrei http://www.atmos-chem-phys.net/8/7335/2008/acp-8-7335-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 24 7335-7351
spelling	(DE-627)DOAJ009023720 (DE-599)DOAJ9f79f1add3fa45cb8cfa395b39bbd2e3 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 J. Li verfasserin aut Near-ground ozone source attributions and outflow in central eastern China during MTX2006 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Physics Chemistry Z. Wang verfasserin aut H. Akimoto verfasserin aut K. Yamaji verfasserin aut M. Takigawa verfasserin aut P. Pochanart verfasserin aut Y. Liu verfasserin aut H. Tanimoto verfasserin aut Y. Kanaya verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 24, Seite 7335-7351 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:24 pages:7335-7351 https://doaj.org/article/9f79f1add3fa45cb8cfa395b39bbd2e3 kostenfrei http://www.atmos-chem-phys.net/8/7335/2008/acp-8-7335-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 24 7335-7351
allfields_unstemmed	(DE-627)DOAJ009023720 (DE-599)DOAJ9f79f1add3fa45cb8cfa395b39bbd2e3 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 J. Li verfasserin aut Near-ground ozone source attributions and outflow in central eastern China during MTX2006 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Physics Chemistry Z. Wang verfasserin aut H. Akimoto verfasserin aut K. Yamaji verfasserin aut M. Takigawa verfasserin aut P. Pochanart verfasserin aut Y. Liu verfasserin aut H. Tanimoto verfasserin aut Y. Kanaya verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 24, Seite 7335-7351 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:24 pages:7335-7351 https://doaj.org/article/9f79f1add3fa45cb8cfa395b39bbd2e3 kostenfrei http://www.atmos-chem-phys.net/8/7335/2008/acp-8-7335-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 24 7335-7351
allfieldsGer	(DE-627)DOAJ009023720 (DE-599)DOAJ9f79f1add3fa45cb8cfa395b39bbd2e3 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 J. Li verfasserin aut Near-ground ozone source attributions and outflow in central eastern China during MTX2006 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Physics Chemistry Z. Wang verfasserin aut H. Akimoto verfasserin aut K. Yamaji verfasserin aut M. Takigawa verfasserin aut P. Pochanart verfasserin aut Y. Liu verfasserin aut H. Tanimoto verfasserin aut Y. Kanaya verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 24, Seite 7335-7351 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:24 pages:7335-7351 https://doaj.org/article/9f79f1add3fa45cb8cfa395b39bbd2e3 kostenfrei http://www.atmos-chem-phys.net/8/7335/2008/acp-8-7335-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 24 7335-7351
allfieldsSound	(DE-627)DOAJ009023720 (DE-599)DOAJ9f79f1add3fa45cb8cfa395b39bbd2e3 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 J. Li verfasserin aut Near-ground ozone source attributions and outflow in central eastern China during MTX2006 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC. Physics Chemistry Z. Wang verfasserin aut H. Akimoto verfasserin aut K. Yamaji verfasserin aut M. Takigawa verfasserin aut P. Pochanart verfasserin aut Y. Liu verfasserin aut H. Tanimoto verfasserin aut Y. Kanaya verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 24, Seite 7335-7351 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:24 pages:7335-7351 https://doaj.org/article/9f79f1add3fa45cb8cfa395b39bbd2e3 kostenfrei http://www.atmos-chem-phys.net/8/7335/2008/acp-8-7335-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 24 7335-7351
language	English
source	In Atmospheric Chemistry and Physics 8(2008), 24, Seite 7335-7351 volume:8 year:2008 number:24 pages:7335-7351
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authorswithroles_txt_mv	J. Li @@aut@@ Z. Wang @@aut@@ H. Akimoto @@aut@@ K. Yamaji @@aut@@ M. Takigawa @@aut@@ P. Pochanart @@aut@@ Y. Liu @@aut@@ H. Tanimoto @@aut@@ Y. Kanaya @@aut@@
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Li</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Near-ground ozone source attributions and outflow in central eastern China during MTX2006</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2008</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (&lt;1.5 km above ground level) ozone at Mt. Tai (36.25&deg; N, 117.10&deg; E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. 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callnumber-first	Q - Science
author	J. Li
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topic_title	QC1-999 QD1-999 Near-ground ozone source attributions and outflow in central eastern China during MTX2006
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title	Near-ground ozone source attributions and outflow in central eastern China during MTX2006
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title_full	Near-ground ozone source attributions and outflow in central eastern China during MTX2006
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title_sort	near-ground ozone source attributions and outflow in central eastern china during mtx2006
callnumber	QC1-999
title_auth	Near-ground ozone source attributions and outflow in central eastern China during MTX2006
abstract	A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC.
abstractGer	A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC.
abstract_unstemmed	A 3-D regional chemical transport model, the Nested Air Quality Prediction Model System (NAQPMS), with an on-line tracer tagging module was used to study the source of the near-ground (<1.5 km above ground level) ozone at Mt. Tai (36.25° N, 117.10° E, 1534 m a.s.l.) in Central Eastern China (CEC) during the Mount Tai eXperiment 2006 (MTX2006). The model reproduced the temporal and spatial variations of near-ground ozone and other pollutants, and it captured highly polluted and clean cases well. The simulated near-ground ozone level over CEC was 60–85 ppbv (parts per billion by volume), which was higher than values in Japan and over the North Pacific (20–50 ppbv). The simulated tagged tracer data indicated that the regional-scale transport of chemically produced ozone over other areas in CEC contributed to the greatest fraction (49%) of the near-ground mean ozone at Mt. Tai in June; in situ photochemistry contributed only 12%. Due to high anthropogenic and biomass burning emissions that occurred in the southern part of the CEC, the contribution to ground ozone levels from this area played the most important role (32.4 ppbv, 37.9% of total ozone) in the monthly mean ozone concentration at Mt. Tai; values reached 59 ppbv (62%) on 6–7 June 2006. The monthly mean horizontal distribution of chemically produced ozone from various ozone production regions indicated that photochemical reactions controlled the spatial distribution of O<sub>3</sub> over CEC. The regional-scale transport of pollutants also played an important role in the spatial and temporal distribution of ozone over CEC. Chemically produced ozone from the southern part of the study region can be transported northeastwardly to the northern rim of CEC; the mean contribution was 5–10 ppbv, and it reached 25 ppbv during high ozone events. Studies of the outflow of CEC ozone and its precursors, as well as their influences and contributions to the ozone level over adjacent regions/countries, revealed that the contribution of CEC ozone to mean ozone mixing ratios over the Korean Peninsula and Japan was 5–15 ppbv, of which about half was due to the direct transport of ozone from CEC and half was produced locally by ozone precursors transported from CEC.
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title_short	Near-ground ozone source attributions and outflow in central eastern China during MTX2006
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