A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)

Using the structural and electronic tunability of molecules to control magnetism is a central challenge of inorganic chemistry. Herein, a ten-member family of the high-ordering temperature (<i<T</i<<sub<c</sub<) molecule-based magnetic coordination networks of the form V[<...
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Autor*in:	David S. Tatum [verfasserIn] Joseph M. Zadrozny [verfasserIn] Gordon T. Yee [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	molecule-based ferrimagnetism

Übergeordnetes Werk:	In: Magnetochemistry - MDPI AG, 2017, 5(2019), 3, p 44
Übergeordnetes Werk:	volume:5 ; year:2019 ; number:3, p 44

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/magnetochemistry5030044

Katalog-ID:	DOAJ012578436

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callnumber-first	Q - Science
author	David S. Tatum
spellingShingle	David S. Tatum misc QD1-999 misc molecule-based ferrimagnetism misc Chemistry A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)
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topic_title	QD1-999 A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene) molecule-based ferrimagnetism
topic	misc QD1-999 misc molecule-based ferrimagnetism misc Chemistry
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title	A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)
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title_full	A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)
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author_browse	David S. Tatum Joseph M. Zadrozny Gordon T. Yee
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title_sort	new family of high <i<t<sub<c</sub<</i< molecule-based magnetic networks: v[<i<x</i<-cl<sub<n</sub<ptce]<sub<2</sub<·ych<sub<2</sub<cl<sub<2</sub< (ptce = phenyltricyanoethylene)
callnumber	QD1-999
title_auth	A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)
abstract	Using the structural and electronic tunability of molecules to control magnetism is a central challenge of inorganic chemistry. Herein, a ten-member family of the high-ordering temperature (<i<T</i<<sub<c</sub<) molecule-based magnetic coordination networks of the form V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·<i<y</i<CH<sub<2</sub<Cl<sub<2</sub< (PTCE = phenyltricyanoethylene, <i<y</i< < 0.5) were synthesized and characterized, where <i<x</i< is (are) the position(s) and n is the number of chlorine substitutions on the phenyl ring. These chlorophenyltricyanoethelenes are tunable analogs of the more commonly investigated tetracyanoethylene (TCNE). Varying the number and position of chlorine substitution around the phenyl ring engendered a family of network solids with significantly different magnetic ordering temperatures ranging from 146 to 285 K. The <i<T<sub<c</sub<</i<s of these ferrimagnets were rationalized with the aid of cyclic voltammetry and Density Functional Theory (DFT) calculations.
abstractGer	Using the structural and electronic tunability of molecules to control magnetism is a central challenge of inorganic chemistry. Herein, a ten-member family of the high-ordering temperature (<i<T</i<<sub<c</sub<) molecule-based magnetic coordination networks of the form V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·<i<y</i<CH<sub<2</sub<Cl<sub<2</sub< (PTCE = phenyltricyanoethylene, <i<y</i< < 0.5) were synthesized and characterized, where <i<x</i< is (are) the position(s) and n is the number of chlorine substitutions on the phenyl ring. These chlorophenyltricyanoethelenes are tunable analogs of the more commonly investigated tetracyanoethylene (TCNE). Varying the number and position of chlorine substitution around the phenyl ring engendered a family of network solids with significantly different magnetic ordering temperatures ranging from 146 to 285 K. The <i<T<sub<c</sub<</i<s of these ferrimagnets were rationalized with the aid of cyclic voltammetry and Density Functional Theory (DFT) calculations.
abstract_unstemmed	Using the structural and electronic tunability of molecules to control magnetism is a central challenge of inorganic chemistry. Herein, a ten-member family of the high-ordering temperature (<i<T</i<<sub<c</sub<) molecule-based magnetic coordination networks of the form V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·<i<y</i<CH<sub<2</sub<Cl<sub<2</sub< (PTCE = phenyltricyanoethylene, <i<y</i< < 0.5) were synthesized and characterized, where <i<x</i< is (are) the position(s) and n is the number of chlorine substitutions on the phenyl ring. These chlorophenyltricyanoethelenes are tunable analogs of the more commonly investigated tetracyanoethylene (TCNE). Varying the number and position of chlorine substitution around the phenyl ring engendered a family of network solids with significantly different magnetic ordering temperatures ranging from 146 to 285 K. The <i<T<sub<c</sub<</i<s of these ferrimagnets were rationalized with the aid of cyclic voltammetry and Density Functional Theory (DFT) calculations.
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title_short	A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)
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A New Family of High <i<T<sub<c</sub<</i< Molecule-Based Magnetic Networks: V[<i<x</i<-Cl<sub<n</sub<PTCE]<sub<2</sub<·yCH<sub<2</sub<Cl<sub<2</sub< (PTCE = Phenyltricyanoethylene)

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