Biofuel from hydrocracking of Cerbera manghas oil over Ni-Zn/HZSM-5 catalyst
The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of cat...
Ausführliche Beschreibung
Autor*in: |
Lenny Marlinda [verfasserIn] Danawati Hari Prajitno [verfasserIn] Achmad Roesyadi [verfasserIn] Ignatius Gunardi [verfasserIn] Yustia Wulandari Mirzayanti [verfasserIn] Muhammad Al Muttaqii [verfasserIn] Agus Budianto [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2022 |
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Übergeordnetes Werk: |
In: Eclética Química - Universidade Estadual Paulista, 2019, 47(2022), 1, Seite 17-39 |
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Übergeordnetes Werk: |
volume:47 ; year:2022 ; number:1 ; pages:17-39 |
Links: |
Link aufrufen |
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DOI / URN: |
10.26850/1678-4618eqj.v47.1.2022.p17-39 |
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Katalog-ID: |
DOAJ014115824 |
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10.26850/1678-4618eqj.v47.1.2022.p17-39 doi (DE-627)DOAJ014115824 (DE-599)DOAJ20870885266140d3aaa0d105b7d90432 DE-627 ger DE-627 rakwb eng QD1-999 Lenny Marlinda verfasserin aut Biofuel from hydrocracking of Cerbera manghas oil over Ni-Zn/HZSM-5 catalyst 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. Chemistry Danawati Hari Prajitno verfasserin aut Achmad Roesyadi verfasserin aut Ignatius Gunardi verfasserin aut Yustia Wulandari Mirzayanti verfasserin aut Muhammad Al Muttaqii verfasserin aut Agus Budianto verfasserin aut In Eclética Química Universidade Estadual Paulista, 2019 47(2022), 1, Seite 17-39 (DE-627)331729164 (DE-600)2053132-1 16784618 nnns volume:47 year:2022 number:1 pages:17-39 https://doi.org/10.26850/1678-4618eqj.v47.1.2022.p17-39 kostenfrei https://doaj.org/article/20870885266140d3aaa0d105b7d90432 kostenfrei http://revista.iq.unesp.br/ojs/index.php/ecletica/article/view/1197 kostenfrei https://doaj.org/toc/0100-4670 Journal toc kostenfrei https://doaj.org/toc/1678-4618 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 47 2022 1 17-39 |
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10.26850/1678-4618eqj.v47.1.2022.p17-39 doi (DE-627)DOAJ014115824 (DE-599)DOAJ20870885266140d3aaa0d105b7d90432 DE-627 ger DE-627 rakwb eng QD1-999 Lenny Marlinda verfasserin aut Biofuel from hydrocracking of Cerbera manghas oil over Ni-Zn/HZSM-5 catalyst 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. Chemistry Danawati Hari Prajitno verfasserin aut Achmad Roesyadi verfasserin aut Ignatius Gunardi verfasserin aut Yustia Wulandari Mirzayanti verfasserin aut Muhammad Al Muttaqii verfasserin aut Agus Budianto verfasserin aut In Eclética Química Universidade Estadual Paulista, 2019 47(2022), 1, Seite 17-39 (DE-627)331729164 (DE-600)2053132-1 16784618 nnns volume:47 year:2022 number:1 pages:17-39 https://doi.org/10.26850/1678-4618eqj.v47.1.2022.p17-39 kostenfrei https://doaj.org/article/20870885266140d3aaa0d105b7d90432 kostenfrei http://revista.iq.unesp.br/ojs/index.php/ecletica/article/view/1197 kostenfrei https://doaj.org/toc/0100-4670 Journal toc kostenfrei https://doaj.org/toc/1678-4618 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 47 2022 1 17-39 |
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10.26850/1678-4618eqj.v47.1.2022.p17-39 doi (DE-627)DOAJ014115824 (DE-599)DOAJ20870885266140d3aaa0d105b7d90432 DE-627 ger DE-627 rakwb eng QD1-999 Lenny Marlinda verfasserin aut Biofuel from hydrocracking of Cerbera manghas oil over Ni-Zn/HZSM-5 catalyst 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. Chemistry Danawati Hari Prajitno verfasserin aut Achmad Roesyadi verfasserin aut Ignatius Gunardi verfasserin aut Yustia Wulandari Mirzayanti verfasserin aut Muhammad Al Muttaqii verfasserin aut Agus Budianto verfasserin aut In Eclética Química Universidade Estadual Paulista, 2019 47(2022), 1, Seite 17-39 (DE-627)331729164 (DE-600)2053132-1 16784618 nnns volume:47 year:2022 number:1 pages:17-39 https://doi.org/10.26850/1678-4618eqj.v47.1.2022.p17-39 kostenfrei https://doaj.org/article/20870885266140d3aaa0d105b7d90432 kostenfrei http://revista.iq.unesp.br/ojs/index.php/ecletica/article/view/1197 kostenfrei https://doaj.org/toc/0100-4670 Journal toc kostenfrei https://doaj.org/toc/1678-4618 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 47 2022 1 17-39 |
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10.26850/1678-4618eqj.v47.1.2022.p17-39 doi (DE-627)DOAJ014115824 (DE-599)DOAJ20870885266140d3aaa0d105b7d90432 DE-627 ger DE-627 rakwb eng QD1-999 Lenny Marlinda verfasserin aut Biofuel from hydrocracking of Cerbera manghas oil over Ni-Zn/HZSM-5 catalyst 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. Chemistry Danawati Hari Prajitno verfasserin aut Achmad Roesyadi verfasserin aut Ignatius Gunardi verfasserin aut Yustia Wulandari Mirzayanti verfasserin aut Muhammad Al Muttaqii verfasserin aut Agus Budianto verfasserin aut In Eclética Química Universidade Estadual Paulista, 2019 47(2022), 1, Seite 17-39 (DE-627)331729164 (DE-600)2053132-1 16784618 nnns volume:47 year:2022 number:1 pages:17-39 https://doi.org/10.26850/1678-4618eqj.v47.1.2022.p17-39 kostenfrei https://doaj.org/article/20870885266140d3aaa0d105b7d90432 kostenfrei http://revista.iq.unesp.br/ojs/index.php/ecletica/article/view/1197 kostenfrei https://doaj.org/toc/0100-4670 Journal toc kostenfrei https://doaj.org/toc/1678-4618 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 47 2022 1 17-39 |
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The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. |
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The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. |
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The effects of reaction temperature on the hydrocarbon composition of biofuel produced in hydrocracking of Cerbera manghas oil with Ni-Zn/HZSM-5 catalyst were investigated. The incipient wetness impregnation method was applied to prepare the Ni-Zn/HZSM-5 catalysts. Furthermore, the properties of catalysts were measured by X-ray diffraction, atomic absorption spectrometry, and nitrogen physisorption. Hydrocracking process was carried out in Parr USA pressure batch reactor at pressure of 20 ± 5 bar after flowing H2 for 1 h. The reaction with a catalyst/oil ratio of 1 g/150 mL proceeded at various temperatures of 350, 375 and 400 °C for 2 h. Gas chromatography-mass spectrometry was used to analyze biofuel. The most abundant hydrocarbon compounds in biofuel were identified as pentadecane and heptadecane (a major diesel fuel compound) with a different amount at different reaction temperatures. It can be said that the hydrodecarboxylation/decarbonylation routes were the predominant reaction pathways and oxygen removal occurred during hydrocracking. The Cerbera manghas oil can be recommended as a promising biofeed to produce the gasoil as an alternative transportation fuel. |
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