Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots
In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We...
Ausführliche Beschreibung
Autor*in: |
Kai Song [verfasserIn] Jianwei Lin [verfasserIn] Yafeng Zhuang [verfasserIn] Zhizhong Han [verfasserIn] Jinghua Chen [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2021 |
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Übergeordnetes Werk: |
In: Micromachines - MDPI AG, 2010, 12(2021), 12, p 1523 |
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Übergeordnetes Werk: |
volume:12 ; year:2021 ; number:12, p 1523 |
Links: |
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DOI / URN: |
10.3390/mi12121523 |
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Katalog-ID: |
DOAJ014156946 |
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10.3390/mi12121523 doi (DE-627)DOAJ014156946 (DE-599)DOAJ428a556db1594ffb9d8d93df5d4785e2 DE-627 ger DE-627 rakwb eng TJ1-1570 Kai Song verfasserin aut Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor Mechanical engineering and machinery Jianwei Lin verfasserin aut Yafeng Zhuang verfasserin aut Zhizhong Han verfasserin aut Jinghua Chen verfasserin aut In Micromachines MDPI AG, 2010 12(2021), 12, p 1523 (DE-627)665016069 (DE-600)2620864-7 2072666X nnns volume:12 year:2021 number:12, p 1523 https://doi.org/10.3390/mi12121523 kostenfrei https://doaj.org/article/428a556db1594ffb9d8d93df5d4785e2 kostenfrei https://www.mdpi.com/2072-666X/12/12/1523 kostenfrei https://doaj.org/toc/2072-666X Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2021 12, p 1523 |
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10.3390/mi12121523 doi (DE-627)DOAJ014156946 (DE-599)DOAJ428a556db1594ffb9d8d93df5d4785e2 DE-627 ger DE-627 rakwb eng TJ1-1570 Kai Song verfasserin aut Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor Mechanical engineering and machinery Jianwei Lin verfasserin aut Yafeng Zhuang verfasserin aut Zhizhong Han verfasserin aut Jinghua Chen verfasserin aut In Micromachines MDPI AG, 2010 12(2021), 12, p 1523 (DE-627)665016069 (DE-600)2620864-7 2072666X nnns volume:12 year:2021 number:12, p 1523 https://doi.org/10.3390/mi12121523 kostenfrei https://doaj.org/article/428a556db1594ffb9d8d93df5d4785e2 kostenfrei https://www.mdpi.com/2072-666X/12/12/1523 kostenfrei https://doaj.org/toc/2072-666X Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2021 12, p 1523 |
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10.3390/mi12121523 doi (DE-627)DOAJ014156946 (DE-599)DOAJ428a556db1594ffb9d8d93df5d4785e2 DE-627 ger DE-627 rakwb eng TJ1-1570 Kai Song verfasserin aut Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor Mechanical engineering and machinery Jianwei Lin verfasserin aut Yafeng Zhuang verfasserin aut Zhizhong Han verfasserin aut Jinghua Chen verfasserin aut In Micromachines MDPI AG, 2010 12(2021), 12, p 1523 (DE-627)665016069 (DE-600)2620864-7 2072666X nnns volume:12 year:2021 number:12, p 1523 https://doi.org/10.3390/mi12121523 kostenfrei https://doaj.org/article/428a556db1594ffb9d8d93df5d4785e2 kostenfrei https://www.mdpi.com/2072-666X/12/12/1523 kostenfrei https://doaj.org/toc/2072-666X Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2021 12, p 1523 |
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10.3390/mi12121523 doi (DE-627)DOAJ014156946 (DE-599)DOAJ428a556db1594ffb9d8d93df5d4785e2 DE-627 ger DE-627 rakwb eng TJ1-1570 Kai Song verfasserin aut Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor Mechanical engineering and machinery Jianwei Lin verfasserin aut Yafeng Zhuang verfasserin aut Zhizhong Han verfasserin aut Jinghua Chen verfasserin aut In Micromachines MDPI AG, 2010 12(2021), 12, p 1523 (DE-627)665016069 (DE-600)2620864-7 2072666X nnns volume:12 year:2021 number:12, p 1523 https://doi.org/10.3390/mi12121523 kostenfrei https://doaj.org/article/428a556db1594ffb9d8d93df5d4785e2 kostenfrei https://www.mdpi.com/2072-666X/12/12/1523 kostenfrei https://doaj.org/toc/2072-666X Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2021 12, p 1523 |
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10.3390/mi12121523 doi (DE-627)DOAJ014156946 (DE-599)DOAJ428a556db1594ffb9d8d93df5d4785e2 DE-627 ger DE-627 rakwb eng TJ1-1570 Kai Song verfasserin aut Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor Mechanical engineering and machinery Jianwei Lin verfasserin aut Yafeng Zhuang verfasserin aut Zhizhong Han verfasserin aut Jinghua Chen verfasserin aut In Micromachines MDPI AG, 2010 12(2021), 12, p 1523 (DE-627)665016069 (DE-600)2620864-7 2072666X nnns volume:12 year:2021 number:12, p 1523 https://doi.org/10.3390/mi12121523 kostenfrei https://doaj.org/article/428a556db1594ffb9d8d93df5d4785e2 kostenfrei https://www.mdpi.com/2072-666X/12/12/1523 kostenfrei https://doaj.org/toc/2072-666X Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2021 12, p 1523 |
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TJ1-1570 Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots titanium dioxide carbon dots black phosphorus quantum dots photoelectrochemical biosensor |
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Construction of Photoelectrochemical DNA Biosensors Based on TiO<sub<2</sub<Carbon Dots@Black Phosphorous Quantum Dots |
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In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. |
abstractGer |
In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. |
abstract_unstemmed |
In this work, carbon dots (CDs) and black phosphorus quantum dots (BPQDs) were used to decorate titanium dioxide to enhance the photoelectrochemical (PEC) properties of the nanocomposites (TiO<sub<2</sub<CDs@BPQDs), and the modified nanocomposites were used to sensitively detect DNA. We used the hydrothermal method and citric acid as a raw material to prepare CDs with good dispersion and strong fluorescence properties. BPQDs with a uniform particle size were prepared from black phosphorus crystals. The nanocomposites were characterized by fluorescence spectroscopy, UV-Vis absorption spectroscopy, Fourier transform infrared spectroscopy (FTIR) and transmission electron microscopy (TEM). The preparation method of the working electrode was explored, the detection conditions were optimized, and the sensitive detection of target DNA was achieved. The results demonstrate that CDs and BPQDs with good optical properties were successfully prepared, and they were successfully combined with TiO<sub<2</sub< to improve the PEC performance of TiO<sub<2</sub<@CDs@BPQDs. The TiO<sub<2</sub<-based PEC DNA detection method was constructed with a detection limit of 8.39 nM. The constructed detection method has many advantages, including good sensitivity, a wide detection range, and good specificity. This work provides a promising PEC strategy for the detection of other biomolecules. |
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