Development of the Chalmers Grouped Actinide Extraction Process

Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(...
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Autor*in:	Halleröd Jenny [verfasserIn] Ekberg Christian [verfasserIn] Löfström-Engdahl Elin [verfasserIn] Aneheim Emma [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2015

Schlagwörter:	btbp-ligands dehba ganex organic diluents tbp solvent extraction

Übergeordnetes Werk:	In: Nukleonika - Sciendo, 2015, 60(2015), 4, Seite 829-835
Übergeordnetes Werk:	volume:60 ; year:2015 ; number:4 ; pages:829-835

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1515/nuka-2015-0115

Katalog-ID:	DOAJ018487815

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520			\|a Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low.
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spelling	10.1515/nuka-2015-0115 doi (DE-627)DOAJ018487815 (DE-599)DOAJ45f08c4107d84c678bda3b9f66f3aa3f DE-627 ger DE-627 rakwb eng Halleröd Jenny verfasserin aut Development of the Chalmers Grouped Actinide Extraction Process 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low. btbp-ligands dehba ganex organic diluents tbp solvent extraction Science Q Ekberg Christian verfasserin aut Löfström-Engdahl Elin verfasserin aut Aneheim Emma verfasserin aut In Nukleonika Sciendo, 2015 60(2015), 4, Seite 829-835 (DE-627)518634310 (DE-600)2253628-0 15085791 nnns volume:60 year:2015 number:4 pages:829-835 https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/article/45f08c4107d84c678bda3b9f66f3aa3f kostenfrei https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/toc/0029-5922 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 60 2015 4 829-835
allfields_unstemmed	10.1515/nuka-2015-0115 doi (DE-627)DOAJ018487815 (DE-599)DOAJ45f08c4107d84c678bda3b9f66f3aa3f DE-627 ger DE-627 rakwb eng Halleröd Jenny verfasserin aut Development of the Chalmers Grouped Actinide Extraction Process 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low. btbp-ligands dehba ganex organic diluents tbp solvent extraction Science Q Ekberg Christian verfasserin aut Löfström-Engdahl Elin verfasserin aut Aneheim Emma verfasserin aut In Nukleonika Sciendo, 2015 60(2015), 4, Seite 829-835 (DE-627)518634310 (DE-600)2253628-0 15085791 nnns volume:60 year:2015 number:4 pages:829-835 https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/article/45f08c4107d84c678bda3b9f66f3aa3f kostenfrei https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/toc/0029-5922 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 60 2015 4 829-835
allfieldsGer	10.1515/nuka-2015-0115 doi (DE-627)DOAJ018487815 (DE-599)DOAJ45f08c4107d84c678bda3b9f66f3aa3f DE-627 ger DE-627 rakwb eng Halleröd Jenny verfasserin aut Development of the Chalmers Grouped Actinide Extraction Process 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low. btbp-ligands dehba ganex organic diluents tbp solvent extraction Science Q Ekberg Christian verfasserin aut Löfström-Engdahl Elin verfasserin aut Aneheim Emma verfasserin aut In Nukleonika Sciendo, 2015 60(2015), 4, Seite 829-835 (DE-627)518634310 (DE-600)2253628-0 15085791 nnns volume:60 year:2015 number:4 pages:829-835 https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/article/45f08c4107d84c678bda3b9f66f3aa3f kostenfrei https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/toc/0029-5922 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 60 2015 4 829-835
allfieldsSound	10.1515/nuka-2015-0115 doi (DE-627)DOAJ018487815 (DE-599)DOAJ45f08c4107d84c678bda3b9f66f3aa3f DE-627 ger DE-627 rakwb eng Halleröd Jenny verfasserin aut Development of the Chalmers Grouped Actinide Extraction Process 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low. btbp-ligands dehba ganex organic diluents tbp solvent extraction Science Q Ekberg Christian verfasserin aut Löfström-Engdahl Elin verfasserin aut Aneheim Emma verfasserin aut In Nukleonika Sciendo, 2015 60(2015), 4, Seite 829-835 (DE-627)518634310 (DE-600)2253628-0 15085791 nnns volume:60 year:2015 number:4 pages:829-835 https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/article/45f08c4107d84c678bda3b9f66f3aa3f kostenfrei https://doi.org/10.1515/nuka-2015-0115 kostenfrei https://doaj.org/toc/0029-5922 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 60 2015 4 829-835
language	English
source	In Nukleonika 60(2015), 4, Seite 829-835 volume:60 year:2015 number:4 pages:829-835
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topic_facet	btbp-ligands dehba ganex organic diluents tbp solvent extraction Science Q
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authorswithroles_txt_mv	Halleröd Jenny @@aut@@ Ekberg Christian @@aut@@ Löfström-Engdahl Elin @@aut@@ Aneheim Emma @@aut@@
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author	Halleröd Jenny
spellingShingle	Halleröd Jenny misc btbp-ligands misc dehba misc ganex misc organic diluents misc tbp misc solvent extraction misc Science misc Q Development of the Chalmers Grouped Actinide Extraction Process
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topic_title	Development of the Chalmers Grouped Actinide Extraction Process btbp-ligands dehba ganex organic diluents tbp solvent extraction
topic	misc btbp-ligands misc dehba misc ganex misc organic diluents misc tbp misc solvent extraction misc Science misc Q
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title	Development of the Chalmers Grouped Actinide Extraction Process
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title_full	Development of the Chalmers Grouped Actinide Extraction Process
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title_sort	development of the chalmers grouped actinide extraction process
title_auth	Development of the Chalmers Grouped Actinide Extraction Process
abstract	Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low.
abstractGer	Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low.
abstract_unstemmed	Several solvents for Grouped ActiNide EXtraction (GANEX) processes have been investigated at Chalmers University of Technology in recent years. Four different GANEX solvents; cyclo-GANEX (CyMe4- -BTBP, 30 vol.% tri-butyl phosphate (TBP) and cyclohexanone), DEHBA-GANEX (CyMe4-BTBP, 20 vol.% N,N-di-2(ethylhexyl) butyramide (DEHBA) and cyclohexanone), hexanol-GANEX (CyMe4-BTBP, 30 vol.% TBP and hexanol) and FS-13-GANEX (CyMe4-BTBP, 30 vol.% TBP and phenyl trifluoromethyl sulfone (FS-13)) have been studied and the results are discussed and compared in this work. The cyclohexanone based solvents show fast and high extraction of the actinides but a somewhat poor diluent stability in contact with the acidic aqueous phase. FS-13-GANEX display high separation factors between the actinides and lanthanides and a good radiolytic and hydrolytic stability. However, the distribution ratios of the actinides are lower, compared to the cyclohexanone based solvents. The hexanol-GANEX is a cheap solvent system using a rather stable diluent but the actinide extraction is, however, comparatively low.
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title_short	Development of the Chalmers Grouped Actinide Extraction Process
url	https://doi.org/10.1515/nuka-2015-0115 https://doaj.org/article/45f08c4107d84c678bda3b9f66f3aa3f https://doaj.org/toc/0029-5922
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Development of the Chalmers Grouped Actinide Extraction Process

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