An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells

Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here...
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Autor*in:	Pengjie Hang [verfasserIn] Jiangsheng Xie [verfasserIn] Ge Li [verfasserIn] Ying Wang [verfasserIn] Desheng Fang [verfasserIn] Yuxin Yao [verfasserIn] Danyan Xie [verfasserIn] Can Cui [verfasserIn] Keyou Yan [verfasserIn] Jianbin Xu [verfasserIn] Deren Yang [verfasserIn] Xuegong Yu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	In: iScience - Elsevier, 2019, 21(2019), Seite 217-227
Übergeordnetes Werk:	volume:21 ; year:2019 ; pages:217-227

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.isci.2019.10.021

Katalog-ID:	DOAJ022807772

Internformat


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520			\|a Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials
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publishDate	2019
allfields	10.1016/j.isci.2019.10.021 doi (DE-627)DOAJ022807772 (DE-599)DOAJ31fe56aa02564be2b0749bfc6fbd7463 DE-627 ger DE-627 rakwb eng Pengjie Hang verfasserin aut An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials Science Q Jiangsheng Xie verfasserin aut Ge Li verfasserin aut Ying Wang verfasserin aut Desheng Fang verfasserin aut Yuxin Yao verfasserin aut Danyan Xie verfasserin aut Can Cui verfasserin aut Keyou Yan verfasserin aut Jianbin Xu verfasserin aut Deren Yang verfasserin aut Xuegong Yu verfasserin aut In iScience Elsevier, 2019 21(2019), Seite 217-227 (DE-627)1019532106 25890042 nnns volume:21 year:2019 pages:217-227 https://doi.org/10.1016/j.isci.2019.10.021 kostenfrei https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219304006 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 21 2019 217-227
spelling	10.1016/j.isci.2019.10.021 doi (DE-627)DOAJ022807772 (DE-599)DOAJ31fe56aa02564be2b0749bfc6fbd7463 DE-627 ger DE-627 rakwb eng Pengjie Hang verfasserin aut An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials Science Q Jiangsheng Xie verfasserin aut Ge Li verfasserin aut Ying Wang verfasserin aut Desheng Fang verfasserin aut Yuxin Yao verfasserin aut Danyan Xie verfasserin aut Can Cui verfasserin aut Keyou Yan verfasserin aut Jianbin Xu verfasserin aut Deren Yang verfasserin aut Xuegong Yu verfasserin aut In iScience Elsevier, 2019 21(2019), Seite 217-227 (DE-627)1019532106 25890042 nnns volume:21 year:2019 pages:217-227 https://doi.org/10.1016/j.isci.2019.10.021 kostenfrei https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219304006 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 21 2019 217-227
allfields_unstemmed	10.1016/j.isci.2019.10.021 doi (DE-627)DOAJ022807772 (DE-599)DOAJ31fe56aa02564be2b0749bfc6fbd7463 DE-627 ger DE-627 rakwb eng Pengjie Hang verfasserin aut An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials Science Q Jiangsheng Xie verfasserin aut Ge Li verfasserin aut Ying Wang verfasserin aut Desheng Fang verfasserin aut Yuxin Yao verfasserin aut Danyan Xie verfasserin aut Can Cui verfasserin aut Keyou Yan verfasserin aut Jianbin Xu verfasserin aut Deren Yang verfasserin aut Xuegong Yu verfasserin aut In iScience Elsevier, 2019 21(2019), Seite 217-227 (DE-627)1019532106 25890042 nnns volume:21 year:2019 pages:217-227 https://doi.org/10.1016/j.isci.2019.10.021 kostenfrei https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219304006 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 21 2019 217-227
allfieldsGer	10.1016/j.isci.2019.10.021 doi (DE-627)DOAJ022807772 (DE-599)DOAJ31fe56aa02564be2b0749bfc6fbd7463 DE-627 ger DE-627 rakwb eng Pengjie Hang verfasserin aut An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials Science Q Jiangsheng Xie verfasserin aut Ge Li verfasserin aut Ying Wang verfasserin aut Desheng Fang verfasserin aut Yuxin Yao verfasserin aut Danyan Xie verfasserin aut Can Cui verfasserin aut Keyou Yan verfasserin aut Jianbin Xu verfasserin aut Deren Yang verfasserin aut Xuegong Yu verfasserin aut In iScience Elsevier, 2019 21(2019), Seite 217-227 (DE-627)1019532106 25890042 nnns volume:21 year:2019 pages:217-227 https://doi.org/10.1016/j.isci.2019.10.021 kostenfrei https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219304006 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 21 2019 217-227
allfieldsSound	10.1016/j.isci.2019.10.021 doi (DE-627)DOAJ022807772 (DE-599)DOAJ31fe56aa02564be2b0749bfc6fbd7463 DE-627 ger DE-627 rakwb eng Pengjie Hang verfasserin aut An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials Science Q Jiangsheng Xie verfasserin aut Ge Li verfasserin aut Ying Wang verfasserin aut Desheng Fang verfasserin aut Yuxin Yao verfasserin aut Danyan Xie verfasserin aut Can Cui verfasserin aut Keyou Yan verfasserin aut Jianbin Xu verfasserin aut Deren Yang verfasserin aut Xuegong Yu verfasserin aut In iScience Elsevier, 2019 21(2019), Seite 217-227 (DE-627)1019532106 25890042 nnns volume:21 year:2019 pages:217-227 https://doi.org/10.1016/j.isci.2019.10.021 kostenfrei https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219304006 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 21 2019 217-227
language	English
source	In iScience 21(2019), Seite 217-227 volume:21 year:2019 pages:217-227
sourceStr	In iScience 21(2019), Seite 217-227 volume:21 year:2019 pages:217-227
format_phy_str_mv	Article
institution	findex.gbv.de
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container_title	iScience
authorswithroles_txt_mv	Pengjie Hang @@aut@@ Jiangsheng Xie @@aut@@ Ge Li @@aut@@ Ying Wang @@aut@@ Desheng Fang @@aut@@ Yuxin Yao @@aut@@ Danyan Xie @@aut@@ Can Cui @@aut@@ Keyou Yan @@aut@@ Jianbin Xu @@aut@@ Deren Yang @@aut@@ Xuegong Yu @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	1019532106
id	DOAJ022807772
language_de	englisch
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author	Pengjie Hang
spellingShingle	Pengjie Hang misc Science misc Q An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
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topic_title	An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
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title	An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
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title_full	An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
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author_browse	Pengjie Hang Jiangsheng Xie Ge Li Ying Wang Desheng Fang Yuxin Yao Danyan Xie Can Cui Keyou Yan Jianbin Xu Deren Yang Xuegong Yu
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author-letter	Pengjie Hang
doi_str_mv	10.1016/j.isci.2019.10.021
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title_sort	interlayer with strong pb-cl bond delivers ultraviolet-filter-free, efficient, and photostable perovskite solar cells
title_auth	An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
abstract	Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials
abstractGer	Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials
abstract_unstemmed	Summary: The inorganic metal oxides (IMOs), including titanium dioxide (TiO2) and tin dioxide (SnO2), inevitably induce decomposition of perovskite under UV illumination owing to their photocatalytic activity, and the use of a UV filter will add extra cost and reduce the effective power output. Here, we first reveal that the weak Pb-I bond in I-based perovskite is prone to breakage under UV photocatalysis, leading to serious degradation of the SnO2/perovskite interface. We introduced a chlorine-rich mixed-halide perovskite interlayer (ClMPI), which possesses an excellent tolerance to photocatalysis owing to the strong Pb-Cl bond, between the SnO2 and I-based perovskite. The ClMPI-based device achieves an enhanced efficiency of up to 21.01% (certified 20.17%). Most importantly, the resultant devices can maintain <94% of their initial performance after 180 h under outdoor solar irradiation, <80% after 500 h under UV irradiation, and 500 h under continuous full spectrum illumination at their maximum power points. : Catalysis; Energy Storage; Energy Materials Subject Areas: Catalysis, Energy Storage, Energy Materials
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title_short	An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells
url	https://doi.org/10.1016/j.isci.2019.10.021 https://doaj.org/article/31fe56aa02564be2b0749bfc6fbd7463 http://www.sciencedirect.com/science/article/pii/S2589004219304006 https://doaj.org/toc/2589-0042
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up_date	2024-07-03T14:08:03.471Z
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An Interlayer with Strong Pb-Cl Bond Delivers Ultraviolet-Filter-Free, Efficient, and Photostable Perovskite Solar Cells

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