A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand

In order to synthesize new coordination polymers with original architectures and interesting magnetic properties, we used the nitranilate ligand (C6O4(NO2)22− = C6N2O82−), derived from the dianionic ligand dhbq2− (2,5-dihydroxy-1,4-benzoquinone = H2C6O42−). The use of this bis-bidentate bridging lig...
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Autor*in:	Samia Benmansour [verfasserIn] Carlos J. Gómez-García [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2016

Schlagwörter:	anilato ligands heterometallic coordination polymers magnetic properties, high spin Fe(III) complex

Übergeordnetes Werk:	In: Polymers - MDPI AG, 2011, 8(2016), 3, p 89
Übergeordnetes Werk:	volume:8 ; year:2016 ; number:3, p 89

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/polym8030089

Katalog-ID:	DOAJ023181311

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callnumber-first	Q - Science
author	Samia Benmansour
spellingShingle	Samia Benmansour misc QD241-441 misc anilato ligands misc heterometallic misc coordination polymers misc magnetic properties, high spin Fe(III) complex misc Organic chemistry A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand
authorStr	Samia Benmansour
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topic_title	QD241-441 A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand anilato ligands heterometallic coordination polymers magnetic properties, high spin Fe(III) complex
topic	misc QD241-441 misc anilato ligands misc heterometallic misc coordination polymers misc magnetic properties, high spin Fe(III) complex misc Organic chemistry
topic_unstemmed	misc QD241-441 misc anilato ligands misc heterometallic misc coordination polymers misc magnetic properties, high spin Fe(III) complex misc Organic chemistry
topic_browse	misc QD241-441 misc anilato ligands misc heterometallic misc coordination polymers misc magnetic properties, high spin Fe(III) complex misc Organic chemistry
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title	A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand
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title_full	A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand
author_sort	Samia Benmansour
journal	Polymers
journalStr	Polymers
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author_browse	Samia Benmansour Carlos J. Gómez-García
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doi_str_mv	10.3390/polym8030089
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title_sort	heterobimetallic anionic 3,6-connected 2d coordination polymer based on nitranilate as ligand
callnumber	QD241-441
title_auth	A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand
abstract	In order to synthesize new coordination polymers with original architectures and interesting magnetic properties, we used the nitranilate ligand (C6O4(NO2)22− = C6N2O82−), derived from the dianionic ligand dhbq2− (2,5-dihydroxy-1,4-benzoquinone = H2C6O42−). The use of this bis-bidentate bridging ligand led to [(DAMS)2{FeNa(C6N2O8)3}·CH3CN]n (1) (DAMS+ = C16H17N2+ = 4-[4-(dimethylamino)-α-styryl]-1-methylpyridinium), a 2D heterometallic coordination polymer presenting an unprecedented structure for any anilato-based compound. This structural type is a 3,6-connected 2D coordination polymer derived from the well-known honeycomb hexagonal structure, where Fe(III) ions alternate with Na+ dimers (as Na2O12 units) in the vertices of the hexagons and with an additional [Fe(C6N2O8)3]3− anion located in the center of the hexagons connecting the three Na+ dimers. The magnetic properties of compound 1 show the presence of paramagnetic isolated high spin Fe(III) complexes with a zero field splitting, \|D\| = 8.5 cm−1.
abstractGer	In order to synthesize new coordination polymers with original architectures and interesting magnetic properties, we used the nitranilate ligand (C6O4(NO2)22− = C6N2O82−), derived from the dianionic ligand dhbq2− (2,5-dihydroxy-1,4-benzoquinone = H2C6O42−). The use of this bis-bidentate bridging ligand led to [(DAMS)2{FeNa(C6N2O8)3}·CH3CN]n (1) (DAMS+ = C16H17N2+ = 4-[4-(dimethylamino)-α-styryl]-1-methylpyridinium), a 2D heterometallic coordination polymer presenting an unprecedented structure for any anilato-based compound. This structural type is a 3,6-connected 2D coordination polymer derived from the well-known honeycomb hexagonal structure, where Fe(III) ions alternate with Na+ dimers (as Na2O12 units) in the vertices of the hexagons and with an additional [Fe(C6N2O8)3]3− anion located in the center of the hexagons connecting the three Na+ dimers. The magnetic properties of compound 1 show the presence of paramagnetic isolated high spin Fe(III) complexes with a zero field splitting, \|D\| = 8.5 cm−1.
abstract_unstemmed	In order to synthesize new coordination polymers with original architectures and interesting magnetic properties, we used the nitranilate ligand (C6O4(NO2)22− = C6N2O82−), derived from the dianionic ligand dhbq2− (2,5-dihydroxy-1,4-benzoquinone = H2C6O42−). The use of this bis-bidentate bridging ligand led to [(DAMS)2{FeNa(C6N2O8)3}·CH3CN]n (1) (DAMS+ = C16H17N2+ = 4-[4-(dimethylamino)-α-styryl]-1-methylpyridinium), a 2D heterometallic coordination polymer presenting an unprecedented structure for any anilato-based compound. This structural type is a 3,6-connected 2D coordination polymer derived from the well-known honeycomb hexagonal structure, where Fe(III) ions alternate with Na+ dimers (as Na2O12 units) in the vertices of the hexagons and with an additional [Fe(C6N2O8)3]3− anion located in the center of the hexagons connecting the three Na+ dimers. The magnetic properties of compound 1 show the presence of paramagnetic isolated high spin Fe(III) complexes with a zero field splitting, \|D\| = 8.5 cm−1.
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container_issue	3, p 89
title_short	A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand
url	https://doi.org/10.3390/polym8030089 https://doaj.org/article/c827b270c289445eb39c34b809e9bcfd http://www.mdpi.com/2073-4360/8/3/89 https://doaj.org/toc/2073-4360
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up_date	2024-07-03T16:11:57.378Z
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A Heterobimetallic Anionic 3,6-Connected 2D Coordination Polymer Based on Nitranilate as Ligand

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