Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production

The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a t...
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Autor*in:	Hao Tian [verfasserIn] Chunlei Pei [verfasserIn] Sai Chen [verfasserIn] Yang Wu [verfasserIn] Zhijian Zhao [verfasserIn] Jinlong Gong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution

Übergeordnetes Werk:	In: Engineering - Elsevier, 2016, 12(2022), Seite 62-69
Übergeordnetes Werk:	volume:12 ; year:2022 ; pages:62-69

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.eng.2020.08.029

Katalog-ID:	DOAJ024993840

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520			\|a The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process.
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700	0		\|a Jinlong Gong \|e verfasserin \|4 aut
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allfields	10.1016/j.eng.2020.08.029 doi (DE-627)DOAJ024993840 (DE-599)DOAJ1c6f9c1b1d1f40f19a2f177f5b7ec249 DE-627 ger DE-627 rakwb eng TA1-2040 Hao Tian verfasserin aut Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process. Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General) Chunlei Pei verfasserin aut Sai Chen verfasserin aut Yang Wu verfasserin aut Zhijian Zhao verfasserin aut Jinlong Gong verfasserin aut In Engineering Elsevier, 2016 12(2022), Seite 62-69 (DE-627)88146578X (DE-600)2886869-9 20960026 nnns volume:12 year:2022 pages:62-69 https://doi.org/10.1016/j.eng.2020.08.029 kostenfrei https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 kostenfrei http://www.sciencedirect.com/science/article/pii/S2095809922000777 kostenfrei https://doaj.org/toc/2095-8099 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 12 2022 62-69
spelling	10.1016/j.eng.2020.08.029 doi (DE-627)DOAJ024993840 (DE-599)DOAJ1c6f9c1b1d1f40f19a2f177f5b7ec249 DE-627 ger DE-627 rakwb eng TA1-2040 Hao Tian verfasserin aut Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process. Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General) Chunlei Pei verfasserin aut Sai Chen verfasserin aut Yang Wu verfasserin aut Zhijian Zhao verfasserin aut Jinlong Gong verfasserin aut In Engineering Elsevier, 2016 12(2022), Seite 62-69 (DE-627)88146578X (DE-600)2886869-9 20960026 nnns volume:12 year:2022 pages:62-69 https://doi.org/10.1016/j.eng.2020.08.029 kostenfrei https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 kostenfrei http://www.sciencedirect.com/science/article/pii/S2095809922000777 kostenfrei https://doaj.org/toc/2095-8099 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 12 2022 62-69
allfields_unstemmed	10.1016/j.eng.2020.08.029 doi (DE-627)DOAJ024993840 (DE-599)DOAJ1c6f9c1b1d1f40f19a2f177f5b7ec249 DE-627 ger DE-627 rakwb eng TA1-2040 Hao Tian verfasserin aut Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process. Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General) Chunlei Pei verfasserin aut Sai Chen verfasserin aut Yang Wu verfasserin aut Zhijian Zhao verfasserin aut Jinlong Gong verfasserin aut In Engineering Elsevier, 2016 12(2022), Seite 62-69 (DE-627)88146578X (DE-600)2886869-9 20960026 nnns volume:12 year:2022 pages:62-69 https://doi.org/10.1016/j.eng.2020.08.029 kostenfrei https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 kostenfrei http://www.sciencedirect.com/science/article/pii/S2095809922000777 kostenfrei https://doaj.org/toc/2095-8099 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 12 2022 62-69
allfieldsGer	10.1016/j.eng.2020.08.029 doi (DE-627)DOAJ024993840 (DE-599)DOAJ1c6f9c1b1d1f40f19a2f177f5b7ec249 DE-627 ger DE-627 rakwb eng TA1-2040 Hao Tian verfasserin aut Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process. Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General) Chunlei Pei verfasserin aut Sai Chen verfasserin aut Yang Wu verfasserin aut Zhijian Zhao verfasserin aut Jinlong Gong verfasserin aut In Engineering Elsevier, 2016 12(2022), Seite 62-69 (DE-627)88146578X (DE-600)2886869-9 20960026 nnns volume:12 year:2022 pages:62-69 https://doi.org/10.1016/j.eng.2020.08.029 kostenfrei https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 kostenfrei http://www.sciencedirect.com/science/article/pii/S2095809922000777 kostenfrei https://doaj.org/toc/2095-8099 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 12 2022 62-69
allfieldsSound	10.1016/j.eng.2020.08.029 doi (DE-627)DOAJ024993840 (DE-599)DOAJ1c6f9c1b1d1f40f19a2f177f5b7ec249 DE-627 ger DE-627 rakwb eng TA1-2040 Hao Tian verfasserin aut Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process. Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General) Chunlei Pei verfasserin aut Sai Chen verfasserin aut Yang Wu verfasserin aut Zhijian Zhao verfasserin aut Jinlong Gong verfasserin aut In Engineering Elsevier, 2016 12(2022), Seite 62-69 (DE-627)88146578X (DE-600)2886869-9 20960026 nnns volume:12 year:2022 pages:62-69 https://doi.org/10.1016/j.eng.2020.08.029 kostenfrei https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 kostenfrei http://www.sciencedirect.com/science/article/pii/S2095809922000777 kostenfrei https://doaj.org/toc/2095-8099 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 12 2022 62-69
language	English
source	In Engineering 12(2022), Seite 62-69 volume:12 year:2022 pages:62-69
sourceStr	In Engineering 12(2022), Seite 62-69 volume:12 year:2022 pages:62-69
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution Engineering (General). Civil engineering (General)
isfreeaccess_bool	true
container_title	Engineering
authorswithroles_txt_mv	Hao Tian @@aut@@ Chunlei Pei @@aut@@ Sai Chen @@aut@@ Yang Wu @@aut@@ Zhijian Zhao @@aut@@ Jinlong Gong @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	88146578X
id	DOAJ024993840
language_de	englisch
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callnumber-first	T - Technology
author	Hao Tian
spellingShingle	Hao Tian misc TA1-2040 misc Chemical looping misc Ethanol steam reforming misc Nickel misc Hydrogen production misc Solid solution misc Engineering (General). Civil engineering (General) Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production
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topic_title	TA1-2040 Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production Chemical looping Ethanol steam reforming Nickel Hydrogen production Solid solution
topic	misc TA1-2040 misc Chemical looping misc Ethanol steam reforming misc Nickel misc Hydrogen production misc Solid solution misc Engineering (General). Civil engineering (General)
topic_unstemmed	misc TA1-2040 misc Chemical looping misc Ethanol steam reforming misc Nickel misc Hydrogen production misc Solid solution misc Engineering (General). Civil engineering (General)
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title	Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production
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title_full	Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production
author_sort	Hao Tian
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title_sort	regulation of oxygen activity by lattice confinement over nixmg1−xo catalysts for renewable hydrogen production
callnumber	TA1-2040
title_auth	Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production
abstract	The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process.
abstractGer	The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process.
abstract_unstemmed	The chemical looping steam reforming (CLSR) of bioethanol is an energy-efficient and carbon-neutral approach of hydrogen production. This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. The design of this solid-solution OC provides a versatile strategy for manipulating the chemical looping process.
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title_short	Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production
url	https://doi.org/10.1016/j.eng.2020.08.029 https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249 http://www.sciencedirect.com/science/article/pii/S2095809922000777 https://doaj.org/toc/2095-8099
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This paper describes the use of a NixMg1−xO solid solution as the oxygen carrier (OC) in the CLSR of bioethanol. Due to the regulation effect of Mg2+ in NixMg1−xO, a three-stage reaction mechanism of the CLSR process is proposed. The surface oxygen of NixMg1−xO initially causes complete oxidation of the ethanol. Subsequently, H2O and bulk oxygen confined by Mg2+ react with ethanol to form CH3COO* followed by H2 over partially reduced NixMg1−xO. Once the bulk oxygen is consumed, the ethanol steam reforming process is promoted by the metallic nickel in the stage III. As a result, Ni0.4Mg0.6O exhibits a high H2 selectivity (4.72 mol H2 per mole ethanol) with a low steam-to-carbon molar ratio of 1, and remains stable over 30 CLSR cycles. 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Civil engineering (General)</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Chunlei Pei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Sai Chen</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Yang Wu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Zhijian Zhao</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Jinlong Gong</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">In</subfield><subfield code="t">Engineering</subfield><subfield code="d">Elsevier, 2016</subfield><subfield code="g">12(2022), Seite 62-69</subfield><subfield code="w">(DE-627)88146578X</subfield><subfield code="w">(DE-600)2886869-9</subfield><subfield code="x">20960026</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:12</subfield><subfield code="g">year:2022</subfield><subfield code="g">pages:62-69</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://doi.org/10.1016/j.eng.2020.08.029</subfield><subfield code="z">kostenfrei</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://doaj.org/article/1c6f9c1b1d1f40f19a2f177f5b7ec249</subfield><subfield code="z">kostenfrei</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">http://www.sciencedirect.com/science/article/pii/S2095809922000777</subfield><subfield code="z">kostenfrei</subfield></datafield><datafield tag="856" ind1="4" 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Regulation of Oxygen Activity by Lattice Confinement over NixMg1−xO Catalysts for Renewable Hydrogen Production

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