The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction

Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The ther...
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Autor*in:	Jian Feng [verfasserIn] Xia Ran [verfasserIn] Li Wang [verfasserIn] Bo Xiao [verfasserIn] Li Lei [verfasserIn] Jinming Zhu [verfasserIn] Zuoji Liu [verfasserIn] Xiaolan Xi [verfasserIn] Guangwei Feng [verfasserIn] Zeqin Dai [verfasserIn] Rong Li [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Cu adsorption photocatalysis degradation Z-scheme

Übergeordnetes Werk:	In: International Journal of Molecular Sciences - MDPI AG, 2003, 23(2022), 22, p 14264
Übergeordnetes Werk:	volume:23 ; year:2022 ; number:22, p 14264

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc Journal toc

DOI / URN:	10.3390/ijms232214264

Katalog-ID:	DOAJ025802097

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spelling	10.3390/ijms232214264 doi (DE-627)DOAJ025802097 (DE-599)DOAJ67ae055241964f628274cb99788b8f40 DE-627 ger DE-627 rakwb eng QH301-705.5 QD1-999 Jian Feng verfasserin aut The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process. Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme Biology (General) Chemistry Xia Ran verfasserin aut Li Wang verfasserin aut Bo Xiao verfasserin aut Li Lei verfasserin aut Jinming Zhu verfasserin aut Zuoji Liu verfasserin aut Xiaolan Xi verfasserin aut Guangwei Feng verfasserin aut Zeqin Dai verfasserin aut Rong Li verfasserin aut In International Journal of Molecular Sciences MDPI AG, 2003 23(2022), 22, p 14264 (DE-627)316340715 (DE-600)2019364-6 14220067 nnns volume:23 year:2022 number:22, p 14264 https://doi.org/10.3390/ijms232214264 kostenfrei https://doaj.org/article/67ae055241964f628274cb99788b8f40 kostenfrei https://www.mdpi.com/1422-0067/23/22/14264 kostenfrei https://doaj.org/toc/1661-6596 Journal toc kostenfrei https://doaj.org/toc/1422-0067 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 23 2022 22, p 14264
allfields_unstemmed	10.3390/ijms232214264 doi (DE-627)DOAJ025802097 (DE-599)DOAJ67ae055241964f628274cb99788b8f40 DE-627 ger DE-627 rakwb eng QH301-705.5 QD1-999 Jian Feng verfasserin aut The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process. Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme Biology (General) Chemistry Xia Ran verfasserin aut Li Wang verfasserin aut Bo Xiao verfasserin aut Li Lei verfasserin aut Jinming Zhu verfasserin aut Zuoji Liu verfasserin aut Xiaolan Xi verfasserin aut Guangwei Feng verfasserin aut Zeqin Dai verfasserin aut Rong Li verfasserin aut In International Journal of Molecular Sciences MDPI AG, 2003 23(2022), 22, p 14264 (DE-627)316340715 (DE-600)2019364-6 14220067 nnns volume:23 year:2022 number:22, p 14264 https://doi.org/10.3390/ijms232214264 kostenfrei https://doaj.org/article/67ae055241964f628274cb99788b8f40 kostenfrei https://www.mdpi.com/1422-0067/23/22/14264 kostenfrei https://doaj.org/toc/1661-6596 Journal toc kostenfrei https://doaj.org/toc/1422-0067 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 23 2022 22, p 14264
allfieldsGer	10.3390/ijms232214264 doi (DE-627)DOAJ025802097 (DE-599)DOAJ67ae055241964f628274cb99788b8f40 DE-627 ger DE-627 rakwb eng QH301-705.5 QD1-999 Jian Feng verfasserin aut The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process. Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme Biology (General) Chemistry Xia Ran verfasserin aut Li Wang verfasserin aut Bo Xiao verfasserin aut Li Lei verfasserin aut Jinming Zhu verfasserin aut Zuoji Liu verfasserin aut Xiaolan Xi verfasserin aut Guangwei Feng verfasserin aut Zeqin Dai verfasserin aut Rong Li verfasserin aut In International Journal of Molecular Sciences MDPI AG, 2003 23(2022), 22, p 14264 (DE-627)316340715 (DE-600)2019364-6 14220067 nnns volume:23 year:2022 number:22, p 14264 https://doi.org/10.3390/ijms232214264 kostenfrei https://doaj.org/article/67ae055241964f628274cb99788b8f40 kostenfrei https://www.mdpi.com/1422-0067/23/22/14264 kostenfrei https://doaj.org/toc/1661-6596 Journal toc kostenfrei https://doaj.org/toc/1422-0067 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 23 2022 22, p 14264
allfieldsSound	10.3390/ijms232214264 doi (DE-627)DOAJ025802097 (DE-599)DOAJ67ae055241964f628274cb99788b8f40 DE-627 ger DE-627 rakwb eng QH301-705.5 QD1-999 Jian Feng verfasserin aut The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process. Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme Biology (General) Chemistry Xia Ran verfasserin aut Li Wang verfasserin aut Bo Xiao verfasserin aut Li Lei verfasserin aut Jinming Zhu verfasserin aut Zuoji Liu verfasserin aut Xiaolan Xi verfasserin aut Guangwei Feng verfasserin aut Zeqin Dai verfasserin aut Rong Li verfasserin aut In International Journal of Molecular Sciences MDPI AG, 2003 23(2022), 22, p 14264 (DE-627)316340715 (DE-600)2019364-6 14220067 nnns volume:23 year:2022 number:22, p 14264 https://doi.org/10.3390/ijms232214264 kostenfrei https://doaj.org/article/67ae055241964f628274cb99788b8f40 kostenfrei https://www.mdpi.com/1422-0067/23/22/14264 kostenfrei https://doaj.org/toc/1661-6596 Journal toc kostenfrei https://doaj.org/toc/1422-0067 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 23 2022 22, p 14264
language	English
source	In International Journal of Molecular Sciences 23(2022), 22, p 14264 volume:23 year:2022 number:22, p 14264
sourceStr	In International Journal of Molecular Sciences 23(2022), 22, p 14264 volume:23 year:2022 number:22, p 14264
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme Biology (General) Chemistry
isfreeaccess_bool	true
container_title	International Journal of Molecular Sciences
authorswithroles_txt_mv	Jian Feng @@aut@@ Xia Ran @@aut@@ Li Wang @@aut@@ Bo Xiao @@aut@@ Li Lei @@aut@@ Jinming Zhu @@aut@@ Zuoji Liu @@aut@@ Xiaolan Xi @@aut@@ Guangwei Feng @@aut@@ Zeqin Dai @@aut@@ Rong Li @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	316340715
id	DOAJ025802097
language_de	englisch
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callnumber-first	Q - Science
author	Jian Feng
spellingShingle	Jian Feng misc QH301-705.5 misc QD1-999 misc Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions misc adsorption misc photocatalysis misc degradation misc Z-scheme misc Biology (General) misc Chemistry The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction
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topic_title	QH301-705.5 QD1-999 The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions adsorption photocatalysis degradation Z-scheme
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topic_unstemmed	misc QH301-705.5 misc QD1-999 misc Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions misc adsorption misc photocatalysis misc degradation misc Z-scheme misc Biology (General) misc Chemistry
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title	The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction
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title_full	The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction
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author_browse	Jian Feng Xia Ran Li Wang Bo Xiao Li Lei Jinming Zhu Zuoji Liu Xiaolan Xi Guangwei Feng Zeqin Dai Rong Li
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author-letter	Jian Feng
doi_str_mv	10.3390/ijms232214264
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title_sort	synergistic effect of adsorption-photocatalysis for removal of organic pollutants on mesoporous cu<sub<2</sub<v<sub<2</sub<o<sub<7</sub</cu<sub<3</sub<v<sub<2</sub<o<sub<8</sub</g-c<sub<3</sub<n<sub<4</sub< heterojunction
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title_auth	The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction
abstract	Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process.
abstractGer	Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process.
abstract_unstemmed	Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< heterojunctions (CVCs) were prepared successfully by the reheating synthesis method. The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. For photocatalytic degradation of CIP, TC and OTC, it was 3.6, 1.8 and 6.1 times that of CN. DRS, XPS VB and ESR results suggested that CVCs had the characteristics of a Z-scheme photocatalytic system. This study provides a reliable reference for the treatment of real wastewater by the adsorption and photocatalysis synergistic process.
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title_short	The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction
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The thermal etching process increased the specific surface area. The formation of heterojunctions enhanced the visible light absorption and improved the separation efficiency of photoinduced charge carriers. Therefore, CVCs exhibited superior adsorption capacity and photocatalytic performance in comparison with pristine g-C<sub<3</sub<N<sub<4</sub< (CN). CVC-2 (containing 2 wt% of Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub<) possessed the best synergistic removal efficiency for removal of dyes and antibiotics, in which 96.2% of methylene blue (MB), 97.3% of rhodamine B (RhB), 83.0% of ciprofloxacin (CIP), 86.0% of tetracycline (TC) and 80.5% of oxytetracycline (OTC) were eliminated by the adsorption and photocatalysis synergistic effect under visible light irradiation. The pseudo first order rate constants of MB and RhB photocatalytic degradation on CVC-2 were 3 times and 10 times that of pristine CN. 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The Synergistic Effect of Adsorption-Photocatalysis for Removal of Organic Pollutants on Mesoporous Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub</Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub</g-C<sub<3</sub<N<sub<4</sub< Heterojunction

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