Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development

Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This re...
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Autor*in:	Chenqian Xu [verfasserIn] Zhenmin Cheng [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	ionic liquid thermal stability thermal decomposition kinetics dicationic ionic liquid

Übergeordnetes Werk:	In: Processes - MDPI AG, 2013, 9(2021), 337, p 337
Übergeordnetes Werk:	volume:9 ; year:2021 ; number:337, p 337

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DOI / URN:	10.3390/pr9020337

Katalog-ID:	DOAJ029913128

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520			\|a Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript.
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allfields	10.3390/pr9020337 doi (DE-627)DOAJ029913128 (DE-599)DOAJdb4778518e264c829bff0169b638dddb DE-627 ger DE-627 rakwb eng TP1-1185 QD1-999 Chenqian Xu verfasserin aut Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript. ionic liquid thermal stability thermal decomposition kinetics dicationic ionic liquid Chemical technology Chemistry Zhenmin Cheng verfasserin aut In Processes MDPI AG, 2013 9(2021), 337, p 337 (DE-627)750371439 (DE-600)2720994-5 22279717 nnns volume:9 year:2021 number:337, p 337 https://doi.org/10.3390/pr9020337 kostenfrei https://doaj.org/article/db4778518e264c829bff0169b638dddb kostenfrei https://www.mdpi.com/2227-9717/9/2/337 kostenfrei https://doaj.org/toc/2227-9717 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2021 337, p 337
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allfieldsSound	10.3390/pr9020337 doi (DE-627)DOAJ029913128 (DE-599)DOAJdb4778518e264c829bff0169b638dddb DE-627 ger DE-627 rakwb eng TP1-1185 QD1-999 Chenqian Xu verfasserin aut Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript. ionic liquid thermal stability thermal decomposition kinetics dicationic ionic liquid Chemical technology Chemistry Zhenmin Cheng verfasserin aut In Processes MDPI AG, 2013 9(2021), 337, p 337 (DE-627)750371439 (DE-600)2720994-5 22279717 nnns volume:9 year:2021 number:337, p 337 https://doi.org/10.3390/pr9020337 kostenfrei https://doaj.org/article/db4778518e264c829bff0169b638dddb kostenfrei https://www.mdpi.com/2227-9717/9/2/337 kostenfrei https://doaj.org/toc/2227-9717 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2021 337, p 337
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callnumber-first	T - Technology
author	Chenqian Xu
spellingShingle	Chenqian Xu misc TP1-1185 misc QD1-999 misc ionic liquid misc thermal stability misc thermal decomposition kinetics misc dicationic ionic liquid misc Chemical technology misc Chemistry Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development
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topic	misc TP1-1185 misc QD1-999 misc ionic liquid misc thermal stability misc thermal decomposition kinetics misc dicationic ionic liquid misc Chemical technology misc Chemistry
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title	Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development
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title_full	Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development
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title_sort	thermal stability of ionic liquids: current status and prospects for future development
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title_auth	Thermal Stability of Ionic Liquids: Current Status and Prospects for Future Development
abstract	Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript.
abstractGer	Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript.
abstract_unstemmed	Ionic liquids (ILs) are the safest solvent in various high-temperature applications due to their non-flammable properties. In order to obtain their thermal stability properties, thermogravimetric analysis (TGA) is extensively used to analyze the kinetics of the thermal decomposition process. This review summarizes the different kinetics analysis methods and finds the isoconversional methods are superior to the Arrhenius methods in calculating the activation energy, and two tools—the compensation effect and master plots—are suggested for the calculation of the pre-exponential factor. With both parameters, the maximum operating temperature (MOT) can be calculated to predict the thermal stability in long-term runnings. The collection of thermal stability data of ILs with divergent cations and anions shows the structure of cations such as alkyl side chains, functional groups, and alkyl substituents will affect the thermal stability, but their influence is less than that of anions. To develop ILs with superior thermal stability, dicationic ILs (DILs) are recommended, and typically, [C<sub<4</sub<(MIM)<sub<2</sub<][NTf<sub<2</sub<]<sub<2</sub< has a decomposition temperature as high as 468.1 °C. For the convenience of application, thermal stability on the decomposition temperature and thermal decomposition activation energy of 130 ILs are summarized at the end of this manuscript.
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