XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes

We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance chang...
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Gespeichert in:

Autor*in:	Chen-Ting Liao [verfasserIn] Arvinder Sandhu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2017

Schlagwörter:	XUV attosecond transient absorption Fano lineshape strong ﬁeld atomic molecular

Übergeordnetes Werk:	In: Photonics - MDPI AG, 2014, 4(2017), 1, p 17
Übergeordnetes Werk:	volume:4 ; year:2017 ; number:1, p 17

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/photonics4010017

Katalog-ID:	DOAJ031179851

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allfieldsSound	10.3390/photonics4010017 doi (DE-627)DOAJ031179851 (DE-599)DOAJ46b4ae41272b40539a56528008cec932 DE-627 ger DE-627 rakwb eng TA1501-1820 Chen-Ting Liao verfasserin aut XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexaﬂuoride (SF6) molecules. We observe and quantify the time-dependence of various transient phenomena in helium atoms,includinglaser-inducedphase(LIP),time-varying(AC)Starkshift,quantumpathinterference, and laser-induced continuum structure. In the case of dense helium targets, we discuss nonlinear macroscopic propagation effects pertaining to LIP and resonant pulse propagation, which accoun tfor the appearance of new spectral features in transient lineshapes. We then use tunable NIR photons to demonstrate the wavelength dependence of the transient laser induced effects. In the case of molecular polarization experiment in SF6, we show suppression of XUV photoabsorption corresponding to inter-valence transitions in the presence of a strong NIR ﬁeld. In each case, the temporal evolution of transient absorption spectra allows us to observe and understand the transient laser induced modiﬁcations of the electronic structure of atoms and molecules. XUV attosecond transient absorption Fano lineshape strong ﬁeld atomic molecular Applied optics. Photonics Arvinder Sandhu verfasserin aut In Photonics MDPI AG, 2014 4(2017), 1, p 17 (DE-627)786192763 (DE-600)2770002-1 23046732 nnns volume:4 year:2017 number:1, p 17 https://doi.org/10.3390/photonics4010017 kostenfrei https://doaj.org/article/46b4ae41272b40539a56528008cec932 kostenfrei http://www.mdpi.com/2304-6732/4/1/17 kostenfrei https://doaj.org/toc/2304-6732 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 4 2017 1, p 17
language	English
source	In Photonics 4(2017), 1, p 17 volume:4 year:2017 number:1, p 17
sourceStr	In Photonics 4(2017), 1, p 17 volume:4 year:2017 number:1, p 17
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topic_facet	XUV attosecond transient absorption Fano lineshape strong ﬁeld atomic molecular Applied optics. Photonics
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container_title	Photonics
authorswithroles_txt_mv	Chen-Ting Liao @@aut@@ Arvinder Sandhu @@aut@@
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callnumber-first	T - Technology
author	Chen-Ting Liao
spellingShingle	Chen-Ting Liao misc TA1501-1820 misc XUV misc attosecond misc transient absorption misc Fano misc lineshape misc strong ﬁeld misc atomic misc molecular misc Applied optics. Photonics XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
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topic_title	TA1501-1820 XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes XUV attosecond transient absorption Fano lineshape strong ﬁeld atomic molecular
topic	misc TA1501-1820 misc XUV misc attosecond misc transient absorption misc Fano misc lineshape misc strong ﬁeld misc atomic misc molecular misc Applied optics. Photonics
topic_unstemmed	misc TA1501-1820 misc XUV misc attosecond misc transient absorption misc Fano misc lineshape misc strong ﬁeld misc atomic misc molecular misc Applied optics. Photonics
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title	XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
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title_full	XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
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title_sort	xuv transient absorption spectroscopy: probing laser-perturbed dipole polarization in single atom, macroscopic, and molecular regimes
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title_auth	XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
abstract	We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexaﬂuoride (SF6) molecules. We observe and quantify the time-dependence of various transient phenomena in helium atoms,includinglaser-inducedphase(LIP),time-varying(AC)Starkshift,quantumpathinterference, and laser-induced continuum structure. In the case of dense helium targets, we discuss nonlinear macroscopic propagation effects pertaining to LIP and resonant pulse propagation, which accoun tfor the appearance of new spectral features in transient lineshapes. We then use tunable NIR photons to demonstrate the wavelength dependence of the transient laser induced effects. In the case of molecular polarization experiment in SF6, we show suppression of XUV photoabsorption corresponding to inter-valence transitions in the presence of a strong NIR ﬁeld. In each case, the temporal evolution of transient absorption spectra allows us to observe and understand the transient laser induced modiﬁcations of the electronic structure of atoms and molecules.
abstractGer	We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexaﬂuoride (SF6) molecules. We observe and quantify the time-dependence of various transient phenomena in helium atoms,includinglaser-inducedphase(LIP),time-varying(AC)Starkshift,quantumpathinterference, and laser-induced continuum structure. In the case of dense helium targets, we discuss nonlinear macroscopic propagation effects pertaining to LIP and resonant pulse propagation, which accoun tfor the appearance of new spectral features in transient lineshapes. We then use tunable NIR photons to demonstrate the wavelength dependence of the transient laser induced effects. In the case of molecular polarization experiment in SF6, we show suppression of XUV photoabsorption corresponding to inter-valence transitions in the presence of a strong NIR ﬁeld. In each case, the temporal evolution of transient absorption spectra allows us to observe and understand the transient laser induced modiﬁcations of the electronic structure of atoms and molecules.
abstract_unstemmed	We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexaﬂuoride (SF6) molecules. We observe and quantify the time-dependence of various transient phenomena in helium atoms,includinglaser-inducedphase(LIP),time-varying(AC)Starkshift,quantumpathinterference, and laser-induced continuum structure. In the case of dense helium targets, we discuss nonlinear macroscopic propagation effects pertaining to LIP and resonant pulse propagation, which accoun tfor the appearance of new spectral features in transient lineshapes. We then use tunable NIR photons to demonstrate the wavelength dependence of the transient laser induced effects. In the case of molecular polarization experiment in SF6, we show suppression of XUV photoabsorption corresponding to inter-valence transitions in the presence of a strong NIR ﬁeld. In each case, the temporal evolution of transient absorption spectra allows us to observe and understand the transient laser induced modiﬁcations of the electronic structure of atoms and molecules.
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title_short	XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
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up_date	2024-07-03T19:10:58.070Z
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XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes

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