Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing

Covalent organic frameworks (COFs) are a new type of metal-free porous architecture with a well-designed pore structure and high stability. Here an efficient electrochemical sensing platform was demonstrated based on COFs TpPa-1 constructed by 1,3,5-triformylphloroglucinol (Tp) with p-phenylenediami...
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Autor*in:	Gang Li [verfasserIn] Baiqing Yuan [verfasserIn] Sidi Chen [verfasserIn] Liju Gan [verfasserIn] Chunying Xu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	covalent organic frameworks electrochemical sensor hydrazine nitrophenol nitrogen doped carbon reduced glutathione

Übergeordnetes Werk:	In: Nanomaterials - MDPI AG, 2012, 12(2022), 17, p 2953
Übergeordnetes Werk:	volume:12 ; year:2022 ; number:17, p 2953

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/nano12172953

Katalog-ID:	DOAJ033478856

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520			\|a Covalent organic frameworks (COFs) are a new type of metal-free porous architecture with a well-designed pore structure and high stability. Here an efficient electrochemical sensing platform was demonstrated based on COFs TpPa-1 constructed by 1,3,5-triformylphloroglucinol (Tp) with p-phenylenediamine (Pa-1), which possesses abundant nitrogen and oxo-functionalities. COFs TpPa-1 exhibited good water dispersibility and strong adsorption affinities for Pd<sup<2+</sup< and thus was used as loading support to modify Pd<sup<2+</sup<. The Pd<sup<2+</sup<-modified COFs TpPa-1 electrode (Pd<sup<2+</sup</COFs) showed high electrocatalytic activity for both hydrazine oxidation reaction and nitrophenol reduction reaction. In addition, TpPa-1-derived nitrogen-doped carbon presented high activity for the electro-oxidation of reduced glutathione (GSH), and sensitive electrochemical detection of GSH was achieved. The presented COFs TpPa-1 can be utilized as a precursor as well as support for anchoring electro-active molecules and nanoparticles, which will be useful for electrochemical sensing and electrocatalysis.
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language	English
source	In Nanomaterials 12(2022), 17, p 2953 volume:12 year:2022 number:17, p 2953
sourceStr	In Nanomaterials 12(2022), 17, p 2953 volume:12 year:2022 number:17, p 2953
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	covalent organic frameworks electrochemical sensor hydrazine nitrophenol nitrogen doped carbon reduced glutathione Chemistry
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container_title	Nanomaterials
authorswithroles_txt_mv	Gang Li @@aut@@ Baiqing Yuan @@aut@@ Sidi Chen @@aut@@ Liju Gan @@aut@@ Chunying Xu @@aut@@
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callnumber-first	Q - Science
author	Gang Li
spellingShingle	Gang Li misc QD1-999 misc covalent organic frameworks misc electrochemical sensor misc hydrazine misc nitrophenol misc nitrogen doped carbon misc reduced glutathione misc Chemistry Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing
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topic_title	QD1-999 Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing covalent organic frameworks electrochemical sensor hydrazine nitrophenol nitrogen doped carbon reduced glutathione
topic	misc QD1-999 misc covalent organic frameworks misc electrochemical sensor misc hydrazine misc nitrophenol misc nitrogen doped carbon misc reduced glutathione misc Chemistry
topic_unstemmed	misc QD1-999 misc covalent organic frameworks misc electrochemical sensor misc hydrazine misc nitrophenol misc nitrogen doped carbon misc reduced glutathione misc Chemistry
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title	Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing
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title_full	Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing
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author_browse	Gang Li Baiqing Yuan Sidi Chen Liju Gan Chunying Xu
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title_sort	covalent organic frameworks-tppa-1 as an emerging platform for electrochemical sensing
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title_auth	Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing
abstract	Covalent organic frameworks (COFs) are a new type of metal-free porous architecture with a well-designed pore structure and high stability. Here an efficient electrochemical sensing platform was demonstrated based on COFs TpPa-1 constructed by 1,3,5-triformylphloroglucinol (Tp) with p-phenylenediamine (Pa-1), which possesses abundant nitrogen and oxo-functionalities. COFs TpPa-1 exhibited good water dispersibility and strong adsorption affinities for Pd<sup<2+</sup< and thus was used as loading support to modify Pd<sup<2+</sup<. The Pd<sup<2+</sup<-modified COFs TpPa-1 electrode (Pd<sup<2+</sup</COFs) showed high electrocatalytic activity for both hydrazine oxidation reaction and nitrophenol reduction reaction. In addition, TpPa-1-derived nitrogen-doped carbon presented high activity for the electro-oxidation of reduced glutathione (GSH), and sensitive electrochemical detection of GSH was achieved. The presented COFs TpPa-1 can be utilized as a precursor as well as support for anchoring electro-active molecules and nanoparticles, which will be useful for electrochemical sensing and electrocatalysis.
abstractGer	Covalent organic frameworks (COFs) are a new type of metal-free porous architecture with a well-designed pore structure and high stability. Here an efficient electrochemical sensing platform was demonstrated based on COFs TpPa-1 constructed by 1,3,5-triformylphloroglucinol (Tp) with p-phenylenediamine (Pa-1), which possesses abundant nitrogen and oxo-functionalities. COFs TpPa-1 exhibited good water dispersibility and strong adsorption affinities for Pd<sup<2+</sup< and thus was used as loading support to modify Pd<sup<2+</sup<. The Pd<sup<2+</sup<-modified COFs TpPa-1 electrode (Pd<sup<2+</sup</COFs) showed high electrocatalytic activity for both hydrazine oxidation reaction and nitrophenol reduction reaction. In addition, TpPa-1-derived nitrogen-doped carbon presented high activity for the electro-oxidation of reduced glutathione (GSH), and sensitive electrochemical detection of GSH was achieved. The presented COFs TpPa-1 can be utilized as a precursor as well as support for anchoring electro-active molecules and nanoparticles, which will be useful for electrochemical sensing and electrocatalysis.
abstract_unstemmed	Covalent organic frameworks (COFs) are a new type of metal-free porous architecture with a well-designed pore structure and high stability. Here an efficient electrochemical sensing platform was demonstrated based on COFs TpPa-1 constructed by 1,3,5-triformylphloroglucinol (Tp) with p-phenylenediamine (Pa-1), which possesses abundant nitrogen and oxo-functionalities. COFs TpPa-1 exhibited good water dispersibility and strong adsorption affinities for Pd<sup<2+</sup< and thus was used as loading support to modify Pd<sup<2+</sup<. The Pd<sup<2+</sup<-modified COFs TpPa-1 electrode (Pd<sup<2+</sup</COFs) showed high electrocatalytic activity for both hydrazine oxidation reaction and nitrophenol reduction reaction. In addition, TpPa-1-derived nitrogen-doped carbon presented high activity for the electro-oxidation of reduced glutathione (GSH), and sensitive electrochemical detection of GSH was achieved. The presented COFs TpPa-1 can be utilized as a precursor as well as support for anchoring electro-active molecules and nanoparticles, which will be useful for electrochemical sensing and electrocatalysis.
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title_short	Covalent Organic Frameworks-TpPa-1 as an Emerging Platform for Electrochemical Sensing
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