Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode

Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending th...
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Autor*in:	He Zhu [verfasserIn] Zhenpeng Yao [verfasserIn] Hekang Zhu [verfasserIn] Yalan Huang [verfasserIn] Jian Zhang [verfasserIn] Cheng Chao Li [verfasserIn] Kamila M. Wiaderek [verfasserIn] Yang Ren [verfasserIn] Cheng‐Jun Sun [verfasserIn] Hua Zhou [verfasserIn] Longlong Fan [verfasserIn] Yanan Chen [verfasserIn] Hui Xia [verfasserIn] Lin Gu [verfasserIn] Si Lan [verfasserIn] Qi Liu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery

Übergeordnetes Werk:	In: Advanced Science - Wiley, 2015, 9(2022), 16, Seite n/a-n/a
Übergeordnetes Werk:	volume:9 ; year:2022 ; number:16 ; pages:n/a-n/a

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1002/advs.202200498

Katalog-ID:	DOAJ043158811

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245	1	0	\|a Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
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520			\|a Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches.
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spelling	10.1002/advs.202200498 doi (DE-627)DOAJ043158811 (DE-599)DOAJc91f77917b554a8e8032ded59bbcb59b DE-627 ger DE-627 rakwb eng He Zhu verfasserin aut Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches. high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery Science Q Zhenpeng Yao verfasserin aut Hekang Zhu verfasserin aut Yalan Huang verfasserin aut Jian Zhang verfasserin aut Cheng Chao Li verfasserin aut Kamila M. Wiaderek verfasserin aut Yang Ren verfasserin aut Cheng‐Jun Sun verfasserin aut Hua Zhou verfasserin aut Longlong Fan verfasserin aut Yanan Chen verfasserin aut Hui Xia verfasserin aut Lin Gu verfasserin aut Si Lan verfasserin aut Qi Liu verfasserin aut In Advanced Science Wiley, 2015 9(2022), 16, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:9 year:2022 number:16 pages:n/a-n/a https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/article/c91f77917b554a8e8032ded59bbcb59b kostenfrei https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2022 16 n/a-n/a
allfields_unstemmed	10.1002/advs.202200498 doi (DE-627)DOAJ043158811 (DE-599)DOAJc91f77917b554a8e8032ded59bbcb59b DE-627 ger DE-627 rakwb eng He Zhu verfasserin aut Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches. high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery Science Q Zhenpeng Yao verfasserin aut Hekang Zhu verfasserin aut Yalan Huang verfasserin aut Jian Zhang verfasserin aut Cheng Chao Li verfasserin aut Kamila M. Wiaderek verfasserin aut Yang Ren verfasserin aut Cheng‐Jun Sun verfasserin aut Hua Zhou verfasserin aut Longlong Fan verfasserin aut Yanan Chen verfasserin aut Hui Xia verfasserin aut Lin Gu verfasserin aut Si Lan verfasserin aut Qi Liu verfasserin aut In Advanced Science Wiley, 2015 9(2022), 16, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:9 year:2022 number:16 pages:n/a-n/a https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/article/c91f77917b554a8e8032ded59bbcb59b kostenfrei https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2022 16 n/a-n/a
allfieldsGer	10.1002/advs.202200498 doi (DE-627)DOAJ043158811 (DE-599)DOAJc91f77917b554a8e8032ded59bbcb59b DE-627 ger DE-627 rakwb eng He Zhu verfasserin aut Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches. high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery Science Q Zhenpeng Yao verfasserin aut Hekang Zhu verfasserin aut Yalan Huang verfasserin aut Jian Zhang verfasserin aut Cheng Chao Li verfasserin aut Kamila M. Wiaderek verfasserin aut Yang Ren verfasserin aut Cheng‐Jun Sun verfasserin aut Hua Zhou verfasserin aut Longlong Fan verfasserin aut Yanan Chen verfasserin aut Hui Xia verfasserin aut Lin Gu verfasserin aut Si Lan verfasserin aut Qi Liu verfasserin aut In Advanced Science Wiley, 2015 9(2022), 16, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:9 year:2022 number:16 pages:n/a-n/a https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/article/c91f77917b554a8e8032ded59bbcb59b kostenfrei https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2022 16 n/a-n/a
allfieldsSound	10.1002/advs.202200498 doi (DE-627)DOAJ043158811 (DE-599)DOAJc91f77917b554a8e8032ded59bbcb59b DE-627 ger DE-627 rakwb eng He Zhu verfasserin aut Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches. high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery Science Q Zhenpeng Yao verfasserin aut Hekang Zhu verfasserin aut Yalan Huang verfasserin aut Jian Zhang verfasserin aut Cheng Chao Li verfasserin aut Kamila M. Wiaderek verfasserin aut Yang Ren verfasserin aut Cheng‐Jun Sun verfasserin aut Hua Zhou verfasserin aut Longlong Fan verfasserin aut Yanan Chen verfasserin aut Hui Xia verfasserin aut Lin Gu verfasserin aut Si Lan verfasserin aut Qi Liu verfasserin aut In Advanced Science Wiley, 2015 9(2022), 16, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:9 year:2022 number:16 pages:n/a-n/a https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/article/c91f77917b554a8e8032ded59bbcb59b kostenfrei https://doi.org/10.1002/advs.202200498 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2022 16 n/a-n/a
language	English
source	In Advanced Science 9(2022), 16, Seite n/a-n/a volume:9 year:2022 number:16 pages:n/a-n/a
sourceStr	In Advanced Science 9(2022), 16, Seite n/a-n/a volume:9 year:2022 number:16 pages:n/a-n/a
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery Science Q
isfreeaccess_bool	true
container_title	Advanced Science
authorswithroles_txt_mv	He Zhu @@aut@@ Zhenpeng Yao @@aut@@ Hekang Zhu @@aut@@ Yalan Huang @@aut@@ Jian Zhang @@aut@@ Cheng Chao Li @@aut@@ Kamila M. Wiaderek @@aut@@ Yang Ren @@aut@@ Cheng‐Jun Sun @@aut@@ Hua Zhou @@aut@@ Longlong Fan @@aut@@ Yanan Chen @@aut@@ Hui Xia @@aut@@ Lin Gu @@aut@@ Si Lan @@aut@@ Qi Liu @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	817357777
id	DOAJ043158811
language_de	englisch
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author	He Zhu
spellingShingle	He Zhu misc high‐voltage structural stability misc in situ synchrotron characterizations misc layered transition‐metal oxide cathodes misc oxygen charge compensation misc sodium‐ion battery misc Science misc Q Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
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topic_title	Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode high‐voltage structural stability in situ synchrotron characterizations layered transition‐metal oxide cathodes oxygen charge compensation sodium‐ion battery
topic	misc high‐voltage structural stability misc in situ synchrotron characterizations misc layered transition‐metal oxide cathodes misc oxygen charge compensation misc sodium‐ion battery misc Science misc Q
topic_unstemmed	misc high‐voltage structural stability misc in situ synchrotron characterizations misc layered transition‐metal oxide cathodes misc oxygen charge compensation misc sodium‐ion battery misc Science misc Q
topic_browse	misc high‐voltage structural stability misc in situ synchrotron characterizations misc layered transition‐metal oxide cathodes misc oxygen charge compensation misc sodium‐ion battery misc Science misc Q
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title	Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
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title_full	Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
author_sort	He Zhu
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author_browse	He Zhu Zhenpeng Yao Hekang Zhu Yalan Huang Jian Zhang Cheng Chao Li Kamila M. Wiaderek Yang Ren Cheng‐Jun Sun Hua Zhou Longlong Fan Yanan Chen Hui Xia Lin Gu Si Lan Qi Liu
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title_sort	unblocking oxygen charge compensation for stabilized high‐voltage structure in p2‐type sodium‐ion cathode
title_auth	Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
abstract	Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches.
abstractGer	Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches.
abstract_unstemmed	Abstract Layered transition‐metal (TM) oxides are ideal hosts for Li+ charge carriers largely due to the occurrence of oxygen charge compensation that stabilizes the layered structure at high voltage. Hence, enabling charge compensation in sodium layered oxides is a fascinating task for extending the cycle life of sodium‐ion batteries. Herein a Ti/Mg co‐doping strategy for a model P2‐Na2/3Ni1/3Mn2/3O2 cathode material is put forward to activate charge compensation through highly hybridized O2pTM3d covalent bonds. In this way, the interlayer OO electrostatic repulsion is weakened upon deeply charging, which strongly affects the systematic total energy that transforms the striking P2–O2 interlayer contraction into a moderate solid‐solution‐type evolution. Accordingly, the cycling stability of the codoped cathode material is improved superiorly over the pristine sample. This study starts a perspective way of optimizing the sodium layered cathodes by rational structural design coupling electrochemical reactions, which can be extended to widespread battery researches.
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title_short	Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode
url	https://doi.org/10.1002/advs.202200498 https://doaj.org/article/c91f77917b554a8e8032ded59bbcb59b https://doaj.org/toc/2198-3844
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Unblocking Oxygen Charge Compensation for Stabilized High‐Voltage Structure in P2‐Type Sodium‐Ion Cathode

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