Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water

Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global product...
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Autor*in:	Mingxin Liu [verfasserIn] Yichen Wang [verfasserIn] Xianghua Kong [verfasserIn] Lida Tan [verfasserIn] Lu Li [verfasserIn] Shaobo Cheng [verfasserIn] Gianluigi Botton [verfasserIn] Hong Guo [verfasserIn] Zetian Mi [verfasserIn] Chao-Jun Li [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	In: iScience - Elsevier, 2019, 17(2019), Seite 208-216
Übergeordnetes Werk:	volume:17 ; year:2019 ; pages:208-216

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.isci.2019.06.032

Katalog-ID:	DOAJ046304746

Internformat


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publishDate	2019
allfields	10.1016/j.isci.2019.06.032 doi (DE-627)DOAJ046304746 (DE-599)DOAJ99b3b906ba154cedbf906fffc36f377c DE-627 ger DE-627 rakwb eng Mingxin Liu verfasserin aut Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure Science Q Yichen Wang verfasserin aut Xianghua Kong verfasserin aut Lida Tan verfasserin aut Lu Li verfasserin aut Shaobo Cheng verfasserin aut Gianluigi Botton verfasserin aut Hong Guo verfasserin aut Zetian Mi verfasserin aut Chao-Jun Li verfasserin aut In iScience Elsevier, 2019 17(2019), Seite 208-216 (DE-627)1019532106 25890042 nnns volume:17 year:2019 pages:208-216 https://doi.org/10.1016/j.isci.2019.06.032 kostenfrei https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219302159 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 17 2019 208-216
spelling	10.1016/j.isci.2019.06.032 doi (DE-627)DOAJ046304746 (DE-599)DOAJ99b3b906ba154cedbf906fffc36f377c DE-627 ger DE-627 rakwb eng Mingxin Liu verfasserin aut Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure Science Q Yichen Wang verfasserin aut Xianghua Kong verfasserin aut Lida Tan verfasserin aut Lu Li verfasserin aut Shaobo Cheng verfasserin aut Gianluigi Botton verfasserin aut Hong Guo verfasserin aut Zetian Mi verfasserin aut Chao-Jun Li verfasserin aut In iScience Elsevier, 2019 17(2019), Seite 208-216 (DE-627)1019532106 25890042 nnns volume:17 year:2019 pages:208-216 https://doi.org/10.1016/j.isci.2019.06.032 kostenfrei https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219302159 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 17 2019 208-216
allfields_unstemmed	10.1016/j.isci.2019.06.032 doi (DE-627)DOAJ046304746 (DE-599)DOAJ99b3b906ba154cedbf906fffc36f377c DE-627 ger DE-627 rakwb eng Mingxin Liu verfasserin aut Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure Science Q Yichen Wang verfasserin aut Xianghua Kong verfasserin aut Lida Tan verfasserin aut Lu Li verfasserin aut Shaobo Cheng verfasserin aut Gianluigi Botton verfasserin aut Hong Guo verfasserin aut Zetian Mi verfasserin aut Chao-Jun Li verfasserin aut In iScience Elsevier, 2019 17(2019), Seite 208-216 (DE-627)1019532106 25890042 nnns volume:17 year:2019 pages:208-216 https://doi.org/10.1016/j.isci.2019.06.032 kostenfrei https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219302159 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 17 2019 208-216
allfieldsGer	10.1016/j.isci.2019.06.032 doi (DE-627)DOAJ046304746 (DE-599)DOAJ99b3b906ba154cedbf906fffc36f377c DE-627 ger DE-627 rakwb eng Mingxin Liu verfasserin aut Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure Science Q Yichen Wang verfasserin aut Xianghua Kong verfasserin aut Lida Tan verfasserin aut Lu Li verfasserin aut Shaobo Cheng verfasserin aut Gianluigi Botton verfasserin aut Hong Guo verfasserin aut Zetian Mi verfasserin aut Chao-Jun Li verfasserin aut In iScience Elsevier, 2019 17(2019), Seite 208-216 (DE-627)1019532106 25890042 nnns volume:17 year:2019 pages:208-216 https://doi.org/10.1016/j.isci.2019.06.032 kostenfrei https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219302159 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 17 2019 208-216
allfieldsSound	10.1016/j.isci.2019.06.032 doi (DE-627)DOAJ046304746 (DE-599)DOAJ99b3b906ba154cedbf906fffc36f377c DE-627 ger DE-627 rakwb eng Mingxin Liu verfasserin aut Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure Science Q Yichen Wang verfasserin aut Xianghua Kong verfasserin aut Lida Tan verfasserin aut Lu Li verfasserin aut Shaobo Cheng verfasserin aut Gianluigi Botton verfasserin aut Hong Guo verfasserin aut Zetian Mi verfasserin aut Chao-Jun Li verfasserin aut In iScience Elsevier, 2019 17(2019), Seite 208-216 (DE-627)1019532106 25890042 nnns volume:17 year:2019 pages:208-216 https://doi.org/10.1016/j.isci.2019.06.032 kostenfrei https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004219302159 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 17 2019 208-216
language	English
source	In iScience 17(2019), Seite 208-216 volume:17 year:2019 pages:208-216
sourceStr	In iScience 17(2019), Seite 208-216 volume:17 year:2019 pages:208-216
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Science Q
isfreeaccess_bool	true
container_title	iScience
authorswithroles_txt_mv	Mingxin Liu @@aut@@ Yichen Wang @@aut@@ Xianghua Kong @@aut@@ Lida Tan @@aut@@ Lu Li @@aut@@ Shaobo Cheng @@aut@@ Gianluigi Botton @@aut@@ Hong Guo @@aut@@ Zetian Mi @@aut@@ Chao-Jun Li @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	1019532106
id	DOAJ046304746
language_de	englisch
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author	Mingxin Liu
spellingShingle	Mingxin Liu misc Science misc Q Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
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topic_title	Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
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title	Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
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title_full	Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
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author_browse	Mingxin Liu Yichen Wang Xianghua Kong Lida Tan Lu Li Shaobo Cheng Gianluigi Botton Hong Guo Zetian Mi Chao-Jun Li
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doi_str_mv	10.1016/j.isci.2019.06.032
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title_sort	efficient nitrogen fixation catalyzed by gallium nitride nanowire using nitrogen and water
title_auth	Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
abstract	Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure
abstractGer	Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure
abstract_unstemmed	Summary: Ammonia is one of the most important bulk chemicals in modern society. However, the highly energy-extensive contemporary industrial production of ammonia was developed in the early 20th century and requires extensive heating of highly pressurized flammable hydrogen gas, whose global production still relies heavily on non-sustainable petroleum. The development of “sustainable” nitrogen fixation process represents a grand aspirational chemical pursuit concerning our future human well-being. Herein, we report an ultra-stable nitride-based photosensitizing semiconductor that enables efficient, sustainable, and mild photochemical nitrogen fixation. The catalyst exhibits strong chemisorption of nitrogen and enables immediate electron donation from its surface vacancy to nitrogen. In addition, it was also demonstrated that the nitride-based semiconductor possesses the potential to minimize electron-hole recombination. : Chemical Reaction; Catalysis; Density Functional Theory (DFT); Nanostructure Subject Areas: Chemical Reaction, Catalysis, Density Functional Theory (DFT), Nanostructure
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title_short	Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water
url	https://doi.org/10.1016/j.isci.2019.06.032 https://doaj.org/article/99b3b906ba154cedbf906fffc36f377c http://www.sciencedirect.com/science/article/pii/S2589004219302159 https://doaj.org/toc/2589-0042
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up_date	2024-07-03T19:54:31.933Z
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Efficient Nitrogen Fixation Catalyzed by Gallium Nitride Nanowire Using Nitrogen and Water

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