Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications
A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions...
Ausführliche Beschreibung
Autor*in: |
Hua Bing Tao [verfasserIn] Hong Bin Yang [verfasserIn] Jiazang Chen [verfasserIn] Jianwei Miao [verfasserIn] Bin Liu [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2014 |
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Übergeordnetes Werk: |
In: Beilstein Journal of Nanotechnology - Beilstein-Institut, 2012, 5(2014), 1, Seite 770-777 |
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Übergeordnetes Werk: |
volume:5 ; year:2014 ; number:1 ; pages:770-777 |
Links: |
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DOI / URN: |
10.3762/bjnano.5.89 |
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Katalog-ID: |
DOAJ047169443 |
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10.3762/bjnano.5.89 doi (DE-627)DOAJ047169443 (DE-599)DOAJ963e7b908ab14bd18049e995d4351699 DE-627 ger DE-627 rakwb eng TP1-1185 QC1-999 Hua Bing Tao verfasserin aut Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. graphitic carbon nitride (g-C3N4) heterojunction photoelectrochemical photocatalysis sulfur doping Technology T Chemical technology Science Q Physics Hong Bin Yang verfasserin aut Jiazang Chen verfasserin aut Jianwei Miao verfasserin aut Bin Liu verfasserin aut In Beilstein Journal of Nanotechnology Beilstein-Institut, 2012 5(2014), 1, Seite 770-777 (DE-627)640860400 (DE-600)2583584-1 21904286 nnns volume:5 year:2014 number:1 pages:770-777 https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/article/963e7b908ab14bd18049e995d4351699 kostenfrei https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/toc/2190-4286 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_267 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 5 2014 1 770-777 |
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10.3762/bjnano.5.89 doi (DE-627)DOAJ047169443 (DE-599)DOAJ963e7b908ab14bd18049e995d4351699 DE-627 ger DE-627 rakwb eng TP1-1185 QC1-999 Hua Bing Tao verfasserin aut Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. graphitic carbon nitride (g-C3N4) heterojunction photoelectrochemical photocatalysis sulfur doping Technology T Chemical technology Science Q Physics Hong Bin Yang verfasserin aut Jiazang Chen verfasserin aut Jianwei Miao verfasserin aut Bin Liu verfasserin aut In Beilstein Journal of Nanotechnology Beilstein-Institut, 2012 5(2014), 1, Seite 770-777 (DE-627)640860400 (DE-600)2583584-1 21904286 nnns volume:5 year:2014 number:1 pages:770-777 https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/article/963e7b908ab14bd18049e995d4351699 kostenfrei https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/toc/2190-4286 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_267 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 5 2014 1 770-777 |
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10.3762/bjnano.5.89 doi (DE-627)DOAJ047169443 (DE-599)DOAJ963e7b908ab14bd18049e995d4351699 DE-627 ger DE-627 rakwb eng TP1-1185 QC1-999 Hua Bing Tao verfasserin aut Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. graphitic carbon nitride (g-C3N4) heterojunction photoelectrochemical photocatalysis sulfur doping Technology T Chemical technology Science Q Physics Hong Bin Yang verfasserin aut Jiazang Chen verfasserin aut Jianwei Miao verfasserin aut Bin Liu verfasserin aut In Beilstein Journal of Nanotechnology Beilstein-Institut, 2012 5(2014), 1, Seite 770-777 (DE-627)640860400 (DE-600)2583584-1 21904286 nnns volume:5 year:2014 number:1 pages:770-777 https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/article/963e7b908ab14bd18049e995d4351699 kostenfrei https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/toc/2190-4286 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_267 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 5 2014 1 770-777 |
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10.3762/bjnano.5.89 doi (DE-627)DOAJ047169443 (DE-599)DOAJ963e7b908ab14bd18049e995d4351699 DE-627 ger DE-627 rakwb eng TP1-1185 QC1-999 Hua Bing Tao verfasserin aut Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. graphitic carbon nitride (g-C3N4) heterojunction photoelectrochemical photocatalysis sulfur doping Technology T Chemical technology Science Q Physics Hong Bin Yang verfasserin aut Jiazang Chen verfasserin aut Jianwei Miao verfasserin aut Bin Liu verfasserin aut In Beilstein Journal of Nanotechnology Beilstein-Institut, 2012 5(2014), 1, Seite 770-777 (DE-627)640860400 (DE-600)2583584-1 21904286 nnns volume:5 year:2014 number:1 pages:770-777 https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/article/963e7b908ab14bd18049e995d4351699 kostenfrei https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/toc/2190-4286 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_267 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 5 2014 1 770-777 |
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10.3762/bjnano.5.89 doi (DE-627)DOAJ047169443 (DE-599)DOAJ963e7b908ab14bd18049e995d4351699 DE-627 ger DE-627 rakwb eng TP1-1185 QC1-999 Hua Bing Tao verfasserin aut Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. graphitic carbon nitride (g-C3N4) heterojunction photoelectrochemical photocatalysis sulfur doping Technology T Chemical technology Science Q Physics Hong Bin Yang verfasserin aut Jiazang Chen verfasserin aut Jianwei Miao verfasserin aut Bin Liu verfasserin aut In Beilstein Journal of Nanotechnology Beilstein-Institut, 2012 5(2014), 1, Seite 770-777 (DE-627)640860400 (DE-600)2583584-1 21904286 nnns volume:5 year:2014 number:1 pages:770-777 https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/article/963e7b908ab14bd18049e995d4351699 kostenfrei https://doi.org/10.3762/bjnano.5.89 kostenfrei https://doaj.org/toc/2190-4286 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_267 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 5 2014 1 770-777 |
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Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications |
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A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. |
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A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. |
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A biomolecule-assisted pyrolysis method has been developed to synthesize sulfur-doped graphitic carbon nitride (CNS) nanosheets. During the synthesis, sulfur could be introduced as a dopant into the lattice of carbon nitride (CN). Sulfur doping changed the texture as well as relative band positions of CN. By growing CN on preformed sulfur-doped CN nanosheets, composite CN/CNS heterojunction nanosheets were constructed, which significantly enhanced the photoelectrochemical performance as compared with various control counterparts including CN, CNS and physically mixed CN and CNS (CN+CNS). The enhanced photoelectrochemical performance of CN/CNS heterojunction nanosheets could be ascribed to the efficient separation of photoexcited charge carriers across the heterojunction interface. The strategy of designing and preparing CN/CNS heterojunction photocatalysts in this work can open up new directions for the construction of all CN-based heterojunction photocatalysts. |
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Biomolecule-assisted synthesis of carbon nitride and sulfur-doped carbon nitride heterojunction nanosheets: An efficient heterojunction photocatalyst for photoelectrochemical applications |
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