Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides

Metallated azomethine ylides are commonly used for the construction of N-heterocycles and α-amino acids. Here, the authors report a synergistic Cu/Ir-catalytic system that converts aldimine esters to a variety of chiral homoallylic amines via a cascade allylation/2-aza-Cope rearrangement.

Gespeichert in:

Autor*in:	Liang Wei [verfasserIn] Qiao Zhu [verfasserIn] Lu Xiao [verfasserIn] Hai-Yan Tao [verfasserIn] Chun-Jiang Wang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	In: Nature Communications - Nature Portfolio, 2016, 10(2019), 1, Seite 12
Übergeordnetes Werk:	volume:10 ; year:2019 ; number:1 ; pages:12

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1038/s41467-019-09563-6

Katalog-ID:	DOAJ052235866

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author	Liang Wei
spellingShingle	Liang Wei misc Science misc Q Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
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topic_title	Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
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title	Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
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title_full	Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
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title_sort	synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
title_auth	Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
abstract	Metallated azomethine ylides are commonly used for the construction of N-heterocycles and α-amino acids. Here, the authors report a synergistic Cu/Ir-catalytic system that converts aldimine esters to a variety of chiral homoallylic amines via a cascade allylation/2-aza-Cope rearrangement.
abstractGer	Metallated azomethine ylides are commonly used for the construction of N-heterocycles and α-amino acids. Here, the authors report a synergistic Cu/Ir-catalytic system that converts aldimine esters to a variety of chiral homoallylic amines via a cascade allylation/2-aza-Cope rearrangement.
abstract_unstemmed	Metallated azomethine ylides are commonly used for the construction of N-heterocycles and α-amino acids. Here, the authors report a synergistic Cu/Ir-catalytic system that converts aldimine esters to a variety of chiral homoallylic amines via a cascade allylation/2-aza-Cope rearrangement.
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title_short	Synergistic catalysis for cascade allylation and 2-aza-cope rearrangement of azomethine ylides
url	https://doi.org/10.1038/s41467-019-09563-6 https://doaj.org/article/d66f8b0ef64849baa3af7b38ea218790 https://doaj.org/toc/2041-1723
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