Investigation on effects of tritium release behavior in Li4SiO4 pebbles

For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investi...
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Autor*in:	Qiang Qi [verfasserIn] Mingzhong Zhao [verfasserIn] Fei Sun [verfasserIn] Yingchun Zhang [verfasserIn] Shouxi Gu [verfasserIn] Baolong Ji [verfasserIn] Hai-Shan Zhou [verfasserIn] Yasuhisa Oya [verfasserIn] Songlin Liu [verfasserIn] Guang-Nan Luo [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity

Übergeordnetes Werk:	In: Nuclear Materials and Energy - Elsevier, 2016, 28(2021), Seite 101036-
Übergeordnetes Werk:	volume:28 ; year:2021 ; pages:101036-

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.nme.2021.101036

Katalog-ID:	DOAJ054596017

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520			\|a For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water.
650		4	\|a Nuclear fusion
650		4	\|a Tritium
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650		4	\|a Li4SiO4
650		4	\|a Porosity
653		0	\|a Nuclear engineering. Atomic power
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700	0		\|a Fei Sun \|e verfasserin \|4 aut
700	0		\|a Yingchun Zhang \|e verfasserin \|4 aut
700	0		\|a Shouxi Gu \|e verfasserin \|4 aut
700	0		\|a Baolong Ji \|e verfasserin \|4 aut
700	0		\|a Hai-Shan Zhou \|e verfasserin \|4 aut
700	0		\|a Yasuhisa Oya \|e verfasserin \|4 aut
700	0		\|a Songlin Liu \|e verfasserin \|4 aut
700	0		\|a Guang-Nan Luo \|e verfasserin \|4 aut
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allfields	10.1016/j.nme.2021.101036 doi (DE-627)DOAJ054596017 (DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd DE-627 ger DE-627 rakwb eng TK9001-9401 Qiang Qi verfasserin aut Investigation on effects of tritium release behavior in Li4SiO4 pebbles 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water. Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power Mingzhong Zhao verfasserin aut Fei Sun verfasserin aut Yingchun Zhang verfasserin aut Shouxi Gu verfasserin aut Baolong Ji verfasserin aut Hai-Shan Zhou verfasserin aut Yasuhisa Oya verfasserin aut Songlin Liu verfasserin aut Guang-Nan Luo verfasserin aut In Nuclear Materials and Energy Elsevier, 2016 28(2021), Seite 101036- (DE-627)817363181 (DE-600)2808888-8 23521791 nnns volume:28 year:2021 pages:101036- https://doi.org/10.1016/j.nme.2021.101036 kostenfrei https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd kostenfrei http://www.sciencedirect.com/science/article/pii/S2352179121001095 kostenfrei https://doaj.org/toc/2352-1791 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 28 2021 101036-
spelling	10.1016/j.nme.2021.101036 doi (DE-627)DOAJ054596017 (DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd DE-627 ger DE-627 rakwb eng TK9001-9401 Qiang Qi verfasserin aut Investigation on effects of tritium release behavior in Li4SiO4 pebbles 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water. Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power Mingzhong Zhao verfasserin aut Fei Sun verfasserin aut Yingchun Zhang verfasserin aut Shouxi Gu verfasserin aut Baolong Ji verfasserin aut Hai-Shan Zhou verfasserin aut Yasuhisa Oya verfasserin aut Songlin Liu verfasserin aut Guang-Nan Luo verfasserin aut In Nuclear Materials and Energy Elsevier, 2016 28(2021), Seite 101036- (DE-627)817363181 (DE-600)2808888-8 23521791 nnns volume:28 year:2021 pages:101036- https://doi.org/10.1016/j.nme.2021.101036 kostenfrei https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd kostenfrei http://www.sciencedirect.com/science/article/pii/S2352179121001095 kostenfrei https://doaj.org/toc/2352-1791 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 28 2021 101036-
allfields_unstemmed	10.1016/j.nme.2021.101036 doi (DE-627)DOAJ054596017 (DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd DE-627 ger DE-627 rakwb eng TK9001-9401 Qiang Qi verfasserin aut Investigation on effects of tritium release behavior in Li4SiO4 pebbles 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water. Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power Mingzhong Zhao verfasserin aut Fei Sun verfasserin aut Yingchun Zhang verfasserin aut Shouxi Gu verfasserin aut Baolong Ji verfasserin aut Hai-Shan Zhou verfasserin aut Yasuhisa Oya verfasserin aut Songlin Liu verfasserin aut Guang-Nan Luo verfasserin aut In Nuclear Materials and Energy Elsevier, 2016 28(2021), Seite 101036- (DE-627)817363181 (DE-600)2808888-8 23521791 nnns volume:28 year:2021 pages:101036- https://doi.org/10.1016/j.nme.2021.101036 kostenfrei https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd kostenfrei http://www.sciencedirect.com/science/article/pii/S2352179121001095 kostenfrei https://doaj.org/toc/2352-1791 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 28 2021 101036-
allfieldsGer	10.1016/j.nme.2021.101036 doi (DE-627)DOAJ054596017 (DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd DE-627 ger DE-627 rakwb eng TK9001-9401 Qiang Qi verfasserin aut Investigation on effects of tritium release behavior in Li4SiO4 pebbles 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water. Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power Mingzhong Zhao verfasserin aut Fei Sun verfasserin aut Yingchun Zhang verfasserin aut Shouxi Gu verfasserin aut Baolong Ji verfasserin aut Hai-Shan Zhou verfasserin aut Yasuhisa Oya verfasserin aut Songlin Liu verfasserin aut Guang-Nan Luo verfasserin aut In Nuclear Materials and Energy Elsevier, 2016 28(2021), Seite 101036- (DE-627)817363181 (DE-600)2808888-8 23521791 nnns volume:28 year:2021 pages:101036- https://doi.org/10.1016/j.nme.2021.101036 kostenfrei https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd kostenfrei http://www.sciencedirect.com/science/article/pii/S2352179121001095 kostenfrei https://doaj.org/toc/2352-1791 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 28 2021 101036-
allfieldsSound	10.1016/j.nme.2021.101036 doi (DE-627)DOAJ054596017 (DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd DE-627 ger DE-627 rakwb eng TK9001-9401 Qiang Qi verfasserin aut Investigation on effects of tritium release behavior in Li4SiO4 pebbles 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water. Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power Mingzhong Zhao verfasserin aut Fei Sun verfasserin aut Yingchun Zhang verfasserin aut Shouxi Gu verfasserin aut Baolong Ji verfasserin aut Hai-Shan Zhou verfasserin aut Yasuhisa Oya verfasserin aut Songlin Liu verfasserin aut Guang-Nan Luo verfasserin aut In Nuclear Materials and Energy Elsevier, 2016 28(2021), Seite 101036- (DE-627)817363181 (DE-600)2808888-8 23521791 nnns volume:28 year:2021 pages:101036- https://doi.org/10.1016/j.nme.2021.101036 kostenfrei https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd kostenfrei http://www.sciencedirect.com/science/article/pii/S2352179121001095 kostenfrei https://doaj.org/toc/2352-1791 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 28 2021 101036-
language	English
source	In Nuclear Materials and Energy 28(2021), Seite 101036- volume:28 year:2021 pages:101036-
sourceStr	In Nuclear Materials and Energy 28(2021), Seite 101036- volume:28 year:2021 pages:101036-
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity Nuclear engineering. Atomic power
isfreeaccess_bool	true
container_title	Nuclear Materials and Energy
authorswithroles_txt_mv	Qiang Qi @@aut@@ Mingzhong Zhao @@aut@@ Fei Sun @@aut@@ Yingchun Zhang @@aut@@ Shouxi Gu @@aut@@ Baolong Ji @@aut@@ Hai-Shan Zhou @@aut@@ Yasuhisa Oya @@aut@@ Songlin Liu @@aut@@ Guang-Nan Luo @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	817363181
id	DOAJ054596017
language_de	englisch
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Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. 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callnumber-first	T - Technology
author	Qiang Qi
spellingShingle	Qiang Qi misc TK9001-9401 misc Nuclear fusion misc Tritium misc Neutron irradiation misc Li4SiO4 misc Porosity misc Nuclear engineering. Atomic power Investigation on effects of tritium release behavior in Li4SiO4 pebbles
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topic_title	TK9001-9401 Investigation on effects of tritium release behavior in Li4SiO4 pebbles Nuclear fusion Tritium Neutron irradiation Li4SiO4 Porosity
topic	misc TK9001-9401 misc Nuclear fusion misc Tritium misc Neutron irradiation misc Li4SiO4 misc Porosity misc Nuclear engineering. Atomic power
topic_unstemmed	misc TK9001-9401 misc Nuclear fusion misc Tritium misc Neutron irradiation misc Li4SiO4 misc Porosity misc Nuclear engineering. Atomic power
topic_browse	misc TK9001-9401 misc Nuclear fusion misc Tritium misc Neutron irradiation misc Li4SiO4 misc Porosity misc Nuclear engineering. Atomic power
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title	Investigation on effects of tritium release behavior in Li4SiO4 pebbles
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title_full	Investigation on effects of tritium release behavior in Li4SiO4 pebbles
author_sort	Qiang Qi
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author_browse	Qiang Qi Mingzhong Zhao Fei Sun Yingchun Zhang Shouxi Gu Baolong Ji Hai-Shan Zhou Yasuhisa Oya Songlin Liu Guang-Nan Luo
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title_sort	investigation on effects of tritium release behavior in li4sio4 pebbles
callnumber	TK9001-9401
title_auth	Investigation on effects of tritium release behavior in Li4SiO4 pebbles
abstract	For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water.
abstractGer	For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water.
abstract_unstemmed	For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water.
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title_short	Investigation on effects of tritium release behavior in Li4SiO4 pebbles
url	https://doi.org/10.1016/j.nme.2021.101036 https://doaj.org/article/91b401434ec740c6bc3f1755833b81bd http://www.sciencedirect.com/science/article/pii/S2352179121001095 https://doaj.org/toc/2352-1791
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author2Str	Mingzhong Zhao Fei Sun Yingchun Zhang Shouxi Gu Baolong Ji Hai-Shan Zhou Yasuhisa Oya Songlin Liu Guang-Nan Luo
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doi_str	10.1016/j.nme.2021.101036
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up_date	2024-07-03T23:49:37.284Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">DOAJ054596017</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230308183323.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230227s2021 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.nme.2021.101036</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)DOAJ054596017</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-599)DOAJ91b401434ec740c6bc3f1755833b81bd</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="050" ind1=" " ind2="0"><subfield code="a">TK9001-9401</subfield></datafield><datafield tag="100" ind1="0" ind2=" "><subfield code="a">Qiang Qi</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Investigation on effects of tritium release behavior in Li4SiO4 pebbles</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2021</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">For deuterium–tritium fusion reactor, the fuel of tritium is not available naturally. Tritium should be produced by the reaction of Li (n, ɑ) T. Li4SiO4 is one of promising candidates due to its high lithium density. In present work, effects of tritium release behavior from Li4SiO4 have been investigated and compared. The main release peak at lower temperature was attributed to tritium located on/near the grain surface and chemical adsorption on pore surface. The small peak at higher temperature was designated as tritium diffusion from grain including lattice and boundary. The tritium release behavior was simulated by diffusion model and surface reaction model. Tritium behavior is controlled by both diffusion and surface reaction for different stages. Based on the desorption theory, the kinetic parameters were obtained. The effects on tritium release behavior were studied. The porosity has significant effects on tritium release. Higher porosity has large specific surface providing more activation sites and fast channels for tritium release which results in lower temperature of tritium release. The main tritium release form was considered as tritium water. The release peak of deuterium moved towards lower temperature after adsorbing water vapor for 1800 h. It was demonstrated that adsorbing water was beneficial for tritium release due to isotope exchange. Compared the effects of porosity and water vapor, higher porosity has larger effects on tritium release in the present work. Based on the work, the tritium release is controlled by both diffusion and surface reaction at different stage and affected by comprehensive effects including porosity and adsorption water.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Nuclear fusion</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Tritium</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Neutron irradiation</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Li4SiO4</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Porosity</subfield></datafield><datafield tag="653" ind1=" " ind2="0"><subfield code="a">Nuclear engineering. 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Investigation on effects of tritium release behavior in Li4SiO4 pebbles

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