Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite

Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge....
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Autor*in:	Meng‐En Sun [verfasserIn] Ting Geng [verfasserIn] Xue Yong [verfasserIn] Siyu Lu [verfasserIn] Lin Ai [verfasserIn] Guanjun Xiao [verfasserIn] Jinmeng Cai [verfasserIn] Bo Zou [verfasserIn] Shuang‐Quan Zang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites

Übergeordnetes Werk:	In: Advanced Science - Wiley, 2015, 8(2021), 9, Seite n/a-n/a
Übergeordnetes Werk:	volume:8 ; year:2021 ; number:9 ; pages:n/a-n/a

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1002/advs.202004853

Katalog-ID:	DOAJ056762046

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520			\|a Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security.
650		4	\|a blue luminescence
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650		4	\|a high pressure
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allfields	10.1002/advs.202004853 doi (DE-627)DOAJ056762046 (DE-599)DOAJe30c0c13963e49958ad4309d55655b6b DE-627 ger DE-627 rakwb eng Meng‐En Sun verfasserin aut Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security. blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q Ting Geng verfasserin aut Xue Yong verfasserin aut Siyu Lu verfasserin aut Lin Ai verfasserin aut Guanjun Xiao verfasserin aut Jinmeng Cai verfasserin aut Bo Zou verfasserin aut Shuang‐Quan Zang verfasserin aut In Advanced Science Wiley, 2015 8(2021), 9, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:8 year:2021 number:9 pages:n/a-n/a https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b kostenfrei https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2021 9 n/a-n/a
spelling	10.1002/advs.202004853 doi (DE-627)DOAJ056762046 (DE-599)DOAJe30c0c13963e49958ad4309d55655b6b DE-627 ger DE-627 rakwb eng Meng‐En Sun verfasserin aut Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security. blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q Ting Geng verfasserin aut Xue Yong verfasserin aut Siyu Lu verfasserin aut Lin Ai verfasserin aut Guanjun Xiao verfasserin aut Jinmeng Cai verfasserin aut Bo Zou verfasserin aut Shuang‐Quan Zang verfasserin aut In Advanced Science Wiley, 2015 8(2021), 9, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:8 year:2021 number:9 pages:n/a-n/a https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b kostenfrei https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2021 9 n/a-n/a
allfields_unstemmed	10.1002/advs.202004853 doi (DE-627)DOAJ056762046 (DE-599)DOAJe30c0c13963e49958ad4309d55655b6b DE-627 ger DE-627 rakwb eng Meng‐En Sun verfasserin aut Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security. blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q Ting Geng verfasserin aut Xue Yong verfasserin aut Siyu Lu verfasserin aut Lin Ai verfasserin aut Guanjun Xiao verfasserin aut Jinmeng Cai verfasserin aut Bo Zou verfasserin aut Shuang‐Quan Zang verfasserin aut In Advanced Science Wiley, 2015 8(2021), 9, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:8 year:2021 number:9 pages:n/a-n/a https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b kostenfrei https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2021 9 n/a-n/a
allfieldsGer	10.1002/advs.202004853 doi (DE-627)DOAJ056762046 (DE-599)DOAJe30c0c13963e49958ad4309d55655b6b DE-627 ger DE-627 rakwb eng Meng‐En Sun verfasserin aut Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security. blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q Ting Geng verfasserin aut Xue Yong verfasserin aut Siyu Lu verfasserin aut Lin Ai verfasserin aut Guanjun Xiao verfasserin aut Jinmeng Cai verfasserin aut Bo Zou verfasserin aut Shuang‐Quan Zang verfasserin aut In Advanced Science Wiley, 2015 8(2021), 9, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:8 year:2021 number:9 pages:n/a-n/a https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b kostenfrei https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2021 9 n/a-n/a
allfieldsSound	10.1002/advs.202004853 doi (DE-627)DOAJ056762046 (DE-599)DOAJe30c0c13963e49958ad4309d55655b6b DE-627 ger DE-627 rakwb eng Meng‐En Sun verfasserin aut Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security. blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q Ting Geng verfasserin aut Xue Yong verfasserin aut Siyu Lu verfasserin aut Lin Ai verfasserin aut Guanjun Xiao verfasserin aut Jinmeng Cai verfasserin aut Bo Zou verfasserin aut Shuang‐Quan Zang verfasserin aut In Advanced Science Wiley, 2015 8(2021), 9, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:8 year:2021 number:9 pages:n/a-n/a https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b kostenfrei https://doi.org/10.1002/advs.202004853 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2021 9 n/a-n/a
language	English
source	In Advanced Science 8(2021), 9, Seite n/a-n/a volume:8 year:2021 number:9 pages:n/a-n/a
sourceStr	In Advanced Science 8(2021), 9, Seite n/a-n/a volume:8 year:2021 number:9 pages:n/a-n/a
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites Science Q
isfreeaccess_bool	true
container_title	Advanced Science
authorswithroles_txt_mv	Meng‐En Sun @@aut@@ Ting Geng @@aut@@ Xue Yong @@aut@@ Siyu Lu @@aut@@ Lin Ai @@aut@@ Guanjun Xiao @@aut@@ Jinmeng Cai @@aut@@ Bo Zou @@aut@@ Shuang‐Quan Zang @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	817357777
id	DOAJ056762046
language_de	englisch
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author	Meng‐En Sun
spellingShingle	Meng‐En Sun misc blue luminescence misc diamond anvil cell misc high pressure misc pressure‐induced emission misc zero‐dimensional perovskites misc Science misc Q Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite
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topic_title	Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite blue luminescence diamond anvil cell high pressure pressure‐induced emission zero‐dimensional perovskites
topic	misc blue luminescence misc diamond anvil cell misc high pressure misc pressure‐induced emission misc zero‐dimensional perovskites misc Science misc Q
topic_unstemmed	misc blue luminescence misc diamond anvil cell misc high pressure misc pressure‐induced emission misc zero‐dimensional perovskites misc Science misc Q
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title	Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite
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title_sort	pressure‐triggered blue emission of zero‐dimensional organic bismuth bromide perovskite
title_auth	Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite
abstract	Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security.
abstractGer	Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security.
abstract_unstemmed	Abstract Understanding the structure–property relationships in Zero‐dimensional (0D) organic–inorganic metal halide perovskites (OMHPs) is essential for their use in optoelectronic applications. Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. The results may improve potential applications of such materials in the fields of pressure sensing and trademark security.
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title_short	Pressure‐Triggered Blue Emission of Zero‐Dimensional Organic Bismuth Bromide Perovskite
url	https://doi.org/10.1002/advs.202004853 https://doaj.org/article/e30c0c13963e49958ad4309d55655b6b https://doaj.org/toc/2198-3844
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Moreover, increasing the emission intensity, particularly for blue emission, is considerably a challenge. Here, intriguing pressure‐induced emission (PIE) is successfully achieved from an initially nonluminous 0D OMHP [(C6H11NH3)4BiBr6]Br·CH3CN (Cy4BiBr7) upon compression. The emission intensity increases significantly, even reaching high‐efficiency blue luminescence, as the external pressure is increased to 4.9 GPa. Analyses of the in situ high‐pressure experiments and first‐principle calculations indicate that the observed PIE can be attributed to the enhanced exciton binding energy associated with [BiBr6]3– octahedron distortion under pressure. This study of Cy4BiBr7 sheds light on the relationship between the structure and optical properties of OMHPs. 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