Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene

The steric and electronic influence of backbone substitution in IMes-based (IMes = 1,3-bis(2,4,6-trimethylphenyl)imidazol-2-ylidene) N-heterocyclic carbenes (NHC) was probed by synthesizing the [RhCl(CO)2(NHC)] series of complexes to quantify experimentally the Tolman electronic parameter (electroni...
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Autor*in:	César A. Urbina-Blanco [verfasserIn] Xavier Bantreil [verfasserIn] Hervé Clavier [verfasserIn] Alexandra M. Z. Slawin [verfasserIn] Steven P. Nolan [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2010

Schlagwörter:	N-heterocyclic carbene olefin metathesis percent buried volume ruthenium–indenylidene Tolman electronic parameter

Übergeordnetes Werk:	In: Beilstein Journal of Organic Chemistry - Beilstein-Institut, 2005, 6(2010), 1, Seite 1120-1126
Übergeordnetes Werk:	volume:6 ; year:2010 ; number:1 ; pages:1120-1126

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3762/bjoc.6.128

Katalog-ID:	DOAJ066383714

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language	English
source	In Beilstein Journal of Organic Chemistry 6(2010), 1, Seite 1120-1126 volume:6 year:2010 number:1 pages:1120-1126
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topic_facet	N-heterocyclic carbene olefin metathesis percent buried volume ruthenium–indenylidene Tolman electronic parameter Science Q Organic chemistry
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spellingShingle	César A. Urbina-Blanco misc QD241-441 misc N-heterocyclic carbene misc olefin metathesis misc percent buried volume misc ruthenium–indenylidene misc Tolman electronic parameter misc Science misc Q misc Organic chemistry Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene
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topic_title	QD241-441 Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene N-heterocyclic carbene olefin metathesis percent buried volume ruthenium–indenylidene Tolman electronic parameter
topic	misc QD241-441 misc N-heterocyclic carbene misc olefin metathesis misc percent buried volume misc ruthenium–indenylidene misc Tolman electronic parameter misc Science misc Q misc Organic chemistry
topic_unstemmed	misc QD241-441 misc N-heterocyclic carbene misc olefin metathesis misc percent buried volume misc ruthenium–indenylidene misc Tolman electronic parameter misc Science misc Q misc Organic chemistry
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title	Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene
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title_full	Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene
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title_sort	backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated n-heterocyclic carbene
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title_auth	Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene
abstract	The steric and electronic influence of backbone substitution in IMes-based (IMes = 1,3-bis(2,4,6-trimethylphenyl)imidazol-2-ylidene) N-heterocyclic carbenes (NHC) was probed by synthesizing the [RhCl(CO)2(NHC)] series of complexes to quantify experimentally the Tolman electronic parameter (electronic) and the percent buried volume (%Vbur, steric) parameters. The corresponding ruthenium–indenylidene complexes were also synthesized and tested in benchmark metathesis transformations to establish possible correlations between reactivity and NHC electronic and steric parameters.
abstractGer	The steric and electronic influence of backbone substitution in IMes-based (IMes = 1,3-bis(2,4,6-trimethylphenyl)imidazol-2-ylidene) N-heterocyclic carbenes (NHC) was probed by synthesizing the [RhCl(CO)2(NHC)] series of complexes to quantify experimentally the Tolman electronic parameter (electronic) and the percent buried volume (%Vbur, steric) parameters. The corresponding ruthenium–indenylidene complexes were also synthesized and tested in benchmark metathesis transformations to establish possible correlations between reactivity and NHC electronic and steric parameters.
abstract_unstemmed	The steric and electronic influence of backbone substitution in IMes-based (IMes = 1,3-bis(2,4,6-trimethylphenyl)imidazol-2-ylidene) N-heterocyclic carbenes (NHC) was probed by synthesizing the [RhCl(CO)2(NHC)] series of complexes to quantify experimentally the Tolman electronic parameter (electronic) and the percent buried volume (%Vbur, steric) parameters. The corresponding ruthenium–indenylidene complexes were also synthesized and tested in benchmark metathesis transformations to establish possible correlations between reactivity and NHC electronic and steric parameters.
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title_short	Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene
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Backbone tuning in indenylidene–ruthenium complexes bearing an unsaturated N-heterocyclic carbene

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