Temperature-gradient effects on heterogeneous ice nucleation from supercooled water

Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at...
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Autor*in:	Liping Wang [verfasserIn] Weiliang Kong [verfasserIn] Fuxin Wang [verfasserIn] Hong Liu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	In: AIP Advances - AIP Publishing LLC, 2011, 9(2019), 12, Seite 125122-125122-6
Übergeordnetes Werk:	volume:9 ; year:2019 ; number:12 ; pages:125122-125122-6

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1063/1.5133459

Katalog-ID:	DOAJ06805663X

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520			\|a Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at two sides can be controlled to present a temperature difference. The experimental results show that the nucleation temperature under temperature differences will be lower than that under isothermal conditions. In addition, an increase in the temperature difference is shown to linearly increase the supercooling needed for ice nucleation. The temperature gradient is capable of suppressing heterogeneous ice nucleation. Based on the classical nucleation theory, the free energy barrier for heterogeneous nucleation is attributed to the main factor to affect the nucleation rate. By comparing theoretical evaluations with experimental results, correction on the free energy barrier was conducted to predict the nucleation rate in the temperature gradient. Our experimental research and theoretical correction reveal the nucleation behavior of supercooled water under nonequilibrium conditions.
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allfieldsSound	10.1063/1.5133459 doi (DE-627)DOAJ06805663X (DE-599)DOAJ9755a63e48fd4f3c9d72d8b83c1fea09 DE-627 ger DE-627 rakwb eng QC1-999 Liping Wang verfasserin aut Temperature-gradient effects on heterogeneous ice nucleation from supercooled water 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at two sides can be controlled to present a temperature difference. The experimental results show that the nucleation temperature under temperature differences will be lower than that under isothermal conditions. In addition, an increase in the temperature difference is shown to linearly increase the supercooling needed for ice nucleation. The temperature gradient is capable of suppressing heterogeneous ice nucleation. Based on the classical nucleation theory, the free energy barrier for heterogeneous nucleation is attributed to the main factor to affect the nucleation rate. By comparing theoretical evaluations with experimental results, correction on the free energy barrier was conducted to predict the nucleation rate in the temperature gradient. Our experimental research and theoretical correction reveal the nucleation behavior of supercooled water under nonequilibrium conditions. Physics Weiliang Kong verfasserin aut Fuxin Wang verfasserin aut Hong Liu verfasserin aut In AIP Advances AIP Publishing LLC, 2011 9(2019), 12, Seite 125122-125122-6 (DE-627)641391706 (DE-600)2583909-3 21583226 nnns volume:9 year:2019 number:12 pages:125122-125122-6 https://doi.org/10.1063/1.5133459 kostenfrei https://doaj.org/article/9755a63e48fd4f3c9d72d8b83c1fea09 kostenfrei http://dx.doi.org/10.1063/1.5133459 kostenfrei https://doaj.org/toc/2158-3226 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 9 2019 12 125122-125122-6
language	English
source	In AIP Advances 9(2019), 12, Seite 125122-125122-6 volume:9 year:2019 number:12 pages:125122-125122-6
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callnumber-first	Q - Science
author	Liping Wang
spellingShingle	Liping Wang misc QC1-999 misc Physics Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
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topic_title	QC1-999 Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
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title	Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
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title_full	Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
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title_sort	temperature-gradient effects on heterogeneous ice nucleation from supercooled water
callnumber	QC1-999
title_auth	Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
abstract	Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at two sides can be controlled to present a temperature difference. The experimental results show that the nucleation temperature under temperature differences will be lower than that under isothermal conditions. In addition, an increase in the temperature difference is shown to linearly increase the supercooling needed for ice nucleation. The temperature gradient is capable of suppressing heterogeneous ice nucleation. Based on the classical nucleation theory, the free energy barrier for heterogeneous nucleation is attributed to the main factor to affect the nucleation rate. By comparing theoretical evaluations with experimental results, correction on the free energy barrier was conducted to predict the nucleation rate in the temperature gradient. Our experimental research and theoretical correction reveal the nucleation behavior of supercooled water under nonequilibrium conditions.
abstractGer	Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at two sides can be controlled to present a temperature difference. The experimental results show that the nucleation temperature under temperature differences will be lower than that under isothermal conditions. In addition, an increase in the temperature difference is shown to linearly increase the supercooling needed for ice nucleation. The temperature gradient is capable of suppressing heterogeneous ice nucleation. Based on the classical nucleation theory, the free energy barrier for heterogeneous nucleation is attributed to the main factor to affect the nucleation rate. By comparing theoretical evaluations with experimental results, correction on the free energy barrier was conducted to predict the nucleation rate in the temperature gradient. Our experimental research and theoretical correction reveal the nucleation behavior of supercooled water under nonequilibrium conditions.
abstract_unstemmed	Investigating the nucleation and freezing behavior of supercooled water under temperature gradients is of significance for theoretical research and practical application. This paper focuses on the freezing temperature of bulk supercooled water in a rectangular container for which the temperature at two sides can be controlled to present a temperature difference. The experimental results show that the nucleation temperature under temperature differences will be lower than that under isothermal conditions. In addition, an increase in the temperature difference is shown to linearly increase the supercooling needed for ice nucleation. The temperature gradient is capable of suppressing heterogeneous ice nucleation. Based on the classical nucleation theory, the free energy barrier for heterogeneous nucleation is attributed to the main factor to affect the nucleation rate. By comparing theoretical evaluations with experimental results, correction on the free energy barrier was conducted to predict the nucleation rate in the temperature gradient. Our experimental research and theoretical correction reveal the nucleation behavior of supercooled water under nonequilibrium conditions.
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title_short	Temperature-gradient effects on heterogeneous ice nucleation from supercooled water
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