Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation

To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studi...
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Gespeichert in:

Autor*in:	Muhammad Zubair [verfasserIn] Estelle Marie M. Vanhaecke [verfasserIn] Ingeborg-Helene Svenum [verfasserIn] Magnus Rønning [verfasserIn] Jia Yang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	C-doped CdS@G Core-shell nanostructure Photocatalytic H2 generation Graphene Carbon doping in CdS Bandgap narrowing

Übergeordnetes Werk:	In: Green Energy & Environment - KeAi Communications Co., Ltd., 2017, 5(2020), 4, Seite 461-472
Übergeordnetes Werk:	volume:5 ; year:2020 ; number:4 ; pages:461-472

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.gee.2020.10.017

Katalog-ID:	DOAJ071691057

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spelling	10.1016/j.gee.2020.10.017 doi (DE-627)DOAJ071691057 (DE-599)DOAJ1684671a33974d34905f2044c893d541 DE-627 ger DE-627 rakwb eng TJ807-830 QH540-549.5 Muhammad Zubair verfasserin aut Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studied for photocatalytic H2 generation. The most active sample consists of CdS and graphene (CdS-0.15G) exhibits promising photocatalytic activity, producing 3.12 mmol g−1 h−1 of H2 under simulated solar light which is ~4.6 times superior than pure CdS nanoparticles giving an apparent quantum efficiency (AQY) of 11.7%. The enhanced photocatalytic activity for H2 generation is associated to the narrowing of the bandgap, enhanced light absorption, fast interfacial charge transfer, and higher carrier density (ND) in C-doped CdS@G samples. This is achieved by C doping in CdS nanoparticles and the formation of a graphene shell over the C-doped CdS nanoparticles. After stability test, the spent catalysts sample was also characterized to investigate the nanostructure. C-doped CdS@G Core-shell nanostructure Photocatalytic H2 generation Graphene Carbon doping in CdS Bandgap narrowing Renewable energy sources Ecology Estelle Marie M. Vanhaecke verfasserin aut Ingeborg-Helene Svenum verfasserin aut Magnus Rønning verfasserin aut Jia Yang verfasserin aut In Green Energy & Environment KeAi Communications Co., Ltd., 2017 5(2020), 4, Seite 461-472 (DE-627)880047542 (DE-600)2884200-5 24680257 nnns volume:5 year:2020 number:4 pages:461-472 https://doi.org/10.1016/j.gee.2020.10.017 kostenfrei https://doaj.org/article/1684671a33974d34905f2044c893d541 kostenfrei http://www.sciencedirect.com/science/article/pii/S2468025720301746 kostenfrei https://doaj.org/toc/2468-0257 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4367 GBV_ILN_4700 AR 5 2020 4 461-472
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allfieldsSound	10.1016/j.gee.2020.10.017 doi (DE-627)DOAJ071691057 (DE-599)DOAJ1684671a33974d34905f2044c893d541 DE-627 ger DE-627 rakwb eng TJ807-830 QH540-549.5 Muhammad Zubair verfasserin aut Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studied for photocatalytic H2 generation. The most active sample consists of CdS and graphene (CdS-0.15G) exhibits promising photocatalytic activity, producing 3.12 mmol g−1 h−1 of H2 under simulated solar light which is ~4.6 times superior than pure CdS nanoparticles giving an apparent quantum efficiency (AQY) of 11.7%. The enhanced photocatalytic activity for H2 generation is associated to the narrowing of the bandgap, enhanced light absorption, fast interfacial charge transfer, and higher carrier density (ND) in C-doped CdS@G samples. This is achieved by C doping in CdS nanoparticles and the formation of a graphene shell over the C-doped CdS nanoparticles. After stability test, the spent catalysts sample was also characterized to investigate the nanostructure. C-doped CdS@G Core-shell nanostructure Photocatalytic H2 generation Graphene Carbon doping in CdS Bandgap narrowing Renewable energy sources Ecology Estelle Marie M. Vanhaecke verfasserin aut Ingeborg-Helene Svenum verfasserin aut Magnus Rønning verfasserin aut Jia Yang verfasserin aut In Green Energy & Environment KeAi Communications Co., Ltd., 2017 5(2020), 4, Seite 461-472 (DE-627)880047542 (DE-600)2884200-5 24680257 nnns volume:5 year:2020 number:4 pages:461-472 https://doi.org/10.1016/j.gee.2020.10.017 kostenfrei https://doaj.org/article/1684671a33974d34905f2044c893d541 kostenfrei http://www.sciencedirect.com/science/article/pii/S2468025720301746 kostenfrei https://doaj.org/toc/2468-0257 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4367 GBV_ILN_4700 AR 5 2020 4 461-472
language	English
source	In Green Energy & Environment 5(2020), 4, Seite 461-472 volume:5 year:2020 number:4 pages:461-472
sourceStr	In Green Energy & Environment 5(2020), 4, Seite 461-472 volume:5 year:2020 number:4 pages:461-472
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	C-doped CdS@G Core-shell nanostructure Photocatalytic H2 generation Graphene Carbon doping in CdS Bandgap narrowing Renewable energy sources Ecology
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container_title	Green Energy & Environment
authorswithroles_txt_mv	Muhammad Zubair @@aut@@ Estelle Marie M. Vanhaecke @@aut@@ Ingeborg-Helene Svenum @@aut@@ Magnus Rønning @@aut@@ Jia Yang @@aut@@
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callnumber-first	T - Technology
author	Muhammad Zubair
spellingShingle	Muhammad Zubair misc TJ807-830 misc QH540-549.5 misc C-doped CdS@G misc Core-shell nanostructure misc Photocatalytic H2 generation misc Graphene misc Carbon doping in CdS misc Bandgap narrowing misc Renewable energy sources misc Ecology Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation
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topic_title	TJ807-830 QH540-549.5 Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation C-doped CdS@G Core-shell nanostructure Photocatalytic H2 generation Graphene Carbon doping in CdS Bandgap narrowing
topic	misc TJ807-830 misc QH540-549.5 misc C-doped CdS@G misc Core-shell nanostructure misc Photocatalytic H2 generation misc Graphene misc Carbon doping in CdS misc Bandgap narrowing misc Renewable energy sources misc Ecology
topic_unstemmed	misc TJ807-830 misc QH540-549.5 misc C-doped CdS@G misc Core-shell nanostructure misc Photocatalytic H2 generation misc Graphene misc Carbon doping in CdS misc Bandgap narrowing misc Renewable energy sources misc Ecology
topic_browse	misc TJ807-830 misc QH540-549.5 misc C-doped CdS@G misc Core-shell nanostructure misc Photocatalytic H2 generation misc Graphene misc Carbon doping in CdS misc Bandgap narrowing misc Renewable energy sources misc Ecology
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title	Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation
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title_full	Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation
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author_browse	Muhammad Zubair Estelle Marie M. Vanhaecke Ingeborg-Helene Svenum Magnus Rønning Jia Yang
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title_sort	core-shell particles of c-doped cds and graphene: a noble metal-free approach for efficient photocatalytic h2 generation
callnumber	TJ807-830
title_auth	Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation
abstract	To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studied for photocatalytic H2 generation. The most active sample consists of CdS and graphene (CdS-0.15G) exhibits promising photocatalytic activity, producing 3.12 mmol g−1 h−1 of H2 under simulated solar light which is ~4.6 times superior than pure CdS nanoparticles giving an apparent quantum efficiency (AQY) of 11.7%. The enhanced photocatalytic activity for H2 generation is associated to the narrowing of the bandgap, enhanced light absorption, fast interfacial charge transfer, and higher carrier density (ND) in C-doped CdS@G samples. This is achieved by C doping in CdS nanoparticles and the formation of a graphene shell over the C-doped CdS nanoparticles. After stability test, the spent catalysts sample was also characterized to investigate the nanostructure.
abstractGer	To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studied for photocatalytic H2 generation. The most active sample consists of CdS and graphene (CdS-0.15G) exhibits promising photocatalytic activity, producing 3.12 mmol g−1 h−1 of H2 under simulated solar light which is ~4.6 times superior than pure CdS nanoparticles giving an apparent quantum efficiency (AQY) of 11.7%. The enhanced photocatalytic activity for H2 generation is associated to the narrowing of the bandgap, enhanced light absorption, fast interfacial charge transfer, and higher carrier density (ND) in C-doped CdS@G samples. This is achieved by C doping in CdS nanoparticles and the formation of a graphene shell over the C-doped CdS nanoparticles. After stability test, the spent catalysts sample was also characterized to investigate the nanostructure.
abstract_unstemmed	To achieve efficient photocatalytic H2 generation from water using earth-abundant and cost-effective materials, a simple synthesis method for carbon-doped CdS particles wrapped with graphene (C-doped CdSG) is reported. The doping effect and the application of graphene as co-catalyst for CdS is studied for photocatalytic H2 generation. The most active sample consists of CdS and graphene (CdS-0.15G) exhibits promising photocatalytic activity, producing 3.12 mmol g−1 h−1 of H2 under simulated solar light which is ~4.6 times superior than pure CdS nanoparticles giving an apparent quantum efficiency (AQY) of 11.7%. The enhanced photocatalytic activity for H2 generation is associated to the narrowing of the bandgap, enhanced light absorption, fast interfacial charge transfer, and higher carrier density (ND) in C-doped CdS@G samples. This is achieved by C doping in CdS nanoparticles and the formation of a graphene shell over the C-doped CdS nanoparticles. After stability test, the spent catalysts sample was also characterized to investigate the nanostructure.
collection_details	GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4367 GBV_ILN_4700
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title_short	Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation
url	https://doi.org/10.1016/j.gee.2020.10.017 https://doaj.org/article/1684671a33974d34905f2044c893d541 http://www.sciencedirect.com/science/article/pii/S2468025720301746 https://doaj.org/toc/2468-0257
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author2	Estelle Marie M. Vanhaecke Ingeborg-Helene Svenum Magnus Rønning Jia Yang
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up_date	2024-07-03T21:40:03.079Z
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Core-shell particles of C-doped CdS and graphene: A noble metal-free approach for efficient photocatalytic H2 generation

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