Validation of ACE-FTS N2O measurements

The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Ausführliche Beschreibung

Gespeichert in:

Autor*in:	G. P. Stiller [verfasserIn] C. Senten [verfasserIn] O. Schrems [verfasserIn] K. Semeniuk [verfasserIn] M. Schneider [verfasserIn] C. Robert [verfasserIn] M. Ridolfi [verfasserIn] P. Raspollini [verfasserIn] C. Piccolo [verfasserIn] J. Notholt [verfasserIn] D. P. Murtagh [verfasserIn] S. Mikuteit [verfasserIn] J. Mellqvist [verfasserIn] J. C. McConnell [verfasserIn] E. Mahieu [verfasserIn] A. Lambert [verfasserIn] H. Kuellmann [verfasserIn] J. Kuttippurath [verfasserIn] K. Jucks [verfasserIn] N. Jones [verfasserIn] J. J. Jin [verfasserIn] D. W. T. Griffith [verfasserIn] N. Glatthor [verfasserIn] M. Höpfner [verfasserIn] J. Hannigan [verfasserIn] E. Dupuy [verfasserIn] P. Duchatelet [verfasserIn] M. De Mazière [verfasserIn] P. Demoulin [verfasserIn] M. Coffey [verfasserIn] V. Catoire [verfasserIn] C. Boone [verfasserIn] T. Blumenstock [verfasserIn] P. F. Bernath [verfasserIn] K. A. Walker [verfasserIn] T. E. Kerzenmacher [verfasserIn] M. A. Wolff [verfasserIn] K. Strong [verfasserIn] A. Strandberg [verfasserIn] J. Taylor [verfasserIn] C. Tétard [verfasserIn] M. Toohey [verfasserIn] J. Urban [verfasserIn] T. Warneke [verfasserIn] S. Wood [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2008

Übergeordnetes Werk:	In: Atmospheric Chemistry and Physics - Copernicus Publications, 2003, 8(2008), 16, Seite 4759-4786
Übergeordnetes Werk:	volume:8 ; year:2008 ; number:16 ; pages:4759-4786

Links:	Link aufrufen Link aufrufen Journal toc Journal toc

Katalog-ID:	DOAJ073691321

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520			\|a The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data.
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allfields	(DE-627)DOAJ073691321 (DE-599)DOAJa072b29df2754870b9c5e22adcb7bd79 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 G. P. Stiller verfasserin aut Validation of ACE-FTS N2O measurements 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Physics Chemistry C. Senten verfasserin aut O. Schrems verfasserin aut K. Semeniuk verfasserin aut M. Schneider verfasserin aut C. Robert verfasserin aut M. Ridolfi verfasserin aut P. Raspollini verfasserin aut C. Piccolo verfasserin aut J. Notholt verfasserin aut D. P. Murtagh verfasserin aut S. Mikuteit verfasserin aut J. Mellqvist verfasserin aut J. C. McConnell verfasserin aut E. Mahieu verfasserin aut A. Lambert verfasserin aut H. Kuellmann verfasserin aut J. Kuttippurath verfasserin aut K. Jucks verfasserin aut N. Jones verfasserin aut J. J. Jin verfasserin aut D. W. T. Griffith verfasserin aut N. Glatthor verfasserin aut M. Höpfner verfasserin aut J. Hannigan verfasserin aut E. Dupuy verfasserin aut P. Duchatelet verfasserin aut M. De Mazière verfasserin aut P. Demoulin verfasserin aut M. Coffey verfasserin aut V. Catoire verfasserin aut C. Boone verfasserin aut T. Blumenstock verfasserin aut P. F. Bernath verfasserin aut K. A. Walker verfasserin aut T. E. Kerzenmacher verfasserin aut M. A. Wolff verfasserin aut K. Strong verfasserin aut A. Strandberg verfasserin aut J. Taylor verfasserin aut C. Tétard verfasserin aut M. Toohey verfasserin aut J. Urban verfasserin aut T. Warneke verfasserin aut S. Wood verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 16, Seite 4759-4786 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:16 pages:4759-4786 https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 kostenfrei http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 16 4759-4786
spelling	(DE-627)DOAJ073691321 (DE-599)DOAJa072b29df2754870b9c5e22adcb7bd79 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 G. P. Stiller verfasserin aut Validation of ACE-FTS N2O measurements 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Physics Chemistry C. Senten verfasserin aut O. Schrems verfasserin aut K. Semeniuk verfasserin aut M. Schneider verfasserin aut C. Robert verfasserin aut M. Ridolfi verfasserin aut P. Raspollini verfasserin aut C. Piccolo verfasserin aut J. Notholt verfasserin aut D. P. Murtagh verfasserin aut S. Mikuteit verfasserin aut J. Mellqvist verfasserin aut J. C. McConnell verfasserin aut E. Mahieu verfasserin aut A. Lambert verfasserin aut H. Kuellmann verfasserin aut J. Kuttippurath verfasserin aut K. Jucks verfasserin aut N. Jones verfasserin aut J. J. Jin verfasserin aut D. W. T. Griffith verfasserin aut N. Glatthor verfasserin aut M. Höpfner verfasserin aut J. Hannigan verfasserin aut E. Dupuy verfasserin aut P. Duchatelet verfasserin aut M. De Mazière verfasserin aut P. Demoulin verfasserin aut M. Coffey verfasserin aut V. Catoire verfasserin aut C. Boone verfasserin aut T. Blumenstock verfasserin aut P. F. Bernath verfasserin aut K. A. Walker verfasserin aut T. E. Kerzenmacher verfasserin aut M. A. Wolff verfasserin aut K. Strong verfasserin aut A. Strandberg verfasserin aut J. Taylor verfasserin aut C. Tétard verfasserin aut M. Toohey verfasserin aut J. Urban verfasserin aut T. Warneke verfasserin aut S. Wood verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 16, Seite 4759-4786 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:16 pages:4759-4786 https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 kostenfrei http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 16 4759-4786
allfields_unstemmed	(DE-627)DOAJ073691321 (DE-599)DOAJa072b29df2754870b9c5e22adcb7bd79 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 G. P. Stiller verfasserin aut Validation of ACE-FTS N2O measurements 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Physics Chemistry C. Senten verfasserin aut O. Schrems verfasserin aut K. Semeniuk verfasserin aut M. Schneider verfasserin aut C. Robert verfasserin aut M. Ridolfi verfasserin aut P. Raspollini verfasserin aut C. Piccolo verfasserin aut J. Notholt verfasserin aut D. P. Murtagh verfasserin aut S. Mikuteit verfasserin aut J. Mellqvist verfasserin aut J. C. McConnell verfasserin aut E. Mahieu verfasserin aut A. Lambert verfasserin aut H. Kuellmann verfasserin aut J. Kuttippurath verfasserin aut K. Jucks verfasserin aut N. Jones verfasserin aut J. J. Jin verfasserin aut D. W. T. Griffith verfasserin aut N. Glatthor verfasserin aut M. Höpfner verfasserin aut J. Hannigan verfasserin aut E. Dupuy verfasserin aut P. Duchatelet verfasserin aut M. De Mazière verfasserin aut P. Demoulin verfasserin aut M. Coffey verfasserin aut V. Catoire verfasserin aut C. Boone verfasserin aut T. Blumenstock verfasserin aut P. F. Bernath verfasserin aut K. A. Walker verfasserin aut T. E. Kerzenmacher verfasserin aut M. A. Wolff verfasserin aut K. Strong verfasserin aut A. Strandberg verfasserin aut J. Taylor verfasserin aut C. Tétard verfasserin aut M. Toohey verfasserin aut J. Urban verfasserin aut T. Warneke verfasserin aut S. Wood verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 16, Seite 4759-4786 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:16 pages:4759-4786 https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 kostenfrei http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 16 4759-4786
allfieldsGer	(DE-627)DOAJ073691321 (DE-599)DOAJa072b29df2754870b9c5e22adcb7bd79 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 G. P. Stiller verfasserin aut Validation of ACE-FTS N2O measurements 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Physics Chemistry C. Senten verfasserin aut O. Schrems verfasserin aut K. Semeniuk verfasserin aut M. Schneider verfasserin aut C. Robert verfasserin aut M. Ridolfi verfasserin aut P. Raspollini verfasserin aut C. Piccolo verfasserin aut J. Notholt verfasserin aut D. P. Murtagh verfasserin aut S. Mikuteit verfasserin aut J. Mellqvist verfasserin aut J. C. McConnell verfasserin aut E. Mahieu verfasserin aut A. Lambert verfasserin aut H. Kuellmann verfasserin aut J. Kuttippurath verfasserin aut K. Jucks verfasserin aut N. Jones verfasserin aut J. J. Jin verfasserin aut D. W. T. Griffith verfasserin aut N. Glatthor verfasserin aut M. Höpfner verfasserin aut J. Hannigan verfasserin aut E. Dupuy verfasserin aut P. Duchatelet verfasserin aut M. De Mazière verfasserin aut P. Demoulin verfasserin aut M. Coffey verfasserin aut V. Catoire verfasserin aut C. Boone verfasserin aut T. Blumenstock verfasserin aut P. F. Bernath verfasserin aut K. A. Walker verfasserin aut T. E. Kerzenmacher verfasserin aut M. A. Wolff verfasserin aut K. Strong verfasserin aut A. Strandberg verfasserin aut J. Taylor verfasserin aut C. Tétard verfasserin aut M. Toohey verfasserin aut J. Urban verfasserin aut T. Warneke verfasserin aut S. Wood verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 16, Seite 4759-4786 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:16 pages:4759-4786 https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 kostenfrei http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 16 4759-4786
allfieldsSound	(DE-627)DOAJ073691321 (DE-599)DOAJa072b29df2754870b9c5e22adcb7bd79 DE-627 ger DE-627 rakwb eng QC1-999 QD1-999 G. P. Stiller verfasserin aut Validation of ACE-FTS N2O measurements 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data. Physics Chemistry C. Senten verfasserin aut O. Schrems verfasserin aut K. Semeniuk verfasserin aut M. Schneider verfasserin aut C. Robert verfasserin aut M. Ridolfi verfasserin aut P. Raspollini verfasserin aut C. Piccolo verfasserin aut J. Notholt verfasserin aut D. P. Murtagh verfasserin aut S. Mikuteit verfasserin aut J. Mellqvist verfasserin aut J. C. McConnell verfasserin aut E. Mahieu verfasserin aut A. Lambert verfasserin aut H. Kuellmann verfasserin aut J. Kuttippurath verfasserin aut K. Jucks verfasserin aut N. Jones verfasserin aut J. J. Jin verfasserin aut D. W. T. Griffith verfasserin aut N. Glatthor verfasserin aut M. Höpfner verfasserin aut J. Hannigan verfasserin aut E. Dupuy verfasserin aut P. Duchatelet verfasserin aut M. De Mazière verfasserin aut P. Demoulin verfasserin aut M. Coffey verfasserin aut V. Catoire verfasserin aut C. Boone verfasserin aut T. Blumenstock verfasserin aut P. F. Bernath verfasserin aut K. A. Walker verfasserin aut T. E. Kerzenmacher verfasserin aut M. A. Wolff verfasserin aut K. Strong verfasserin aut A. Strandberg verfasserin aut J. Taylor verfasserin aut C. Tétard verfasserin aut M. Toohey verfasserin aut J. Urban verfasserin aut T. Warneke verfasserin aut S. Wood verfasserin aut In Atmospheric Chemistry and Physics Copernicus Publications, 2003 8(2008), 16, Seite 4759-4786 (DE-627)092499996 16807324 nnns volume:8 year:2008 number:16 pages:4759-4786 https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 kostenfrei http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf kostenfrei https://doaj.org/toc/1680-7316 Journal toc kostenfrei https://doaj.org/toc/1680-7324 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_381 AR 8 2008 16 4759-4786
language	English
source	In Atmospheric Chemistry and Physics 8(2008), 16, Seite 4759-4786 volume:8 year:2008 number:16 pages:4759-4786
sourceStr	In Atmospheric Chemistry and Physics 8(2008), 16, Seite 4759-4786 volume:8 year:2008 number:16 pages:4759-4786
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Physics Chemistry
isfreeaccess_bool	true
container_title	Atmospheric Chemistry and Physics
authorswithroles_txt_mv	G. P. Stiller @@aut@@ C. Senten @@aut@@ O. Schrems @@aut@@ K. Semeniuk @@aut@@ M. Schneider @@aut@@ C. Robert @@aut@@ M. Ridolfi @@aut@@ P. Raspollini @@aut@@ C. Piccolo @@aut@@ J. Notholt @@aut@@ D. P. Murtagh @@aut@@ S. Mikuteit @@aut@@ J. Mellqvist @@aut@@ J. C. McConnell @@aut@@ E. Mahieu @@aut@@ A. Lambert @@aut@@ H. Kuellmann @@aut@@ J. Kuttippurath @@aut@@ K. Jucks @@aut@@ N. Jones @@aut@@ J. J. Jin @@aut@@ D. W. T. Griffith @@aut@@ N. Glatthor @@aut@@ M. Höpfner @@aut@@ J. Hannigan @@aut@@ E. Dupuy @@aut@@ P. Duchatelet @@aut@@ M. De Mazière @@aut@@ P. Demoulin @@aut@@ M. Coffey @@aut@@ V. Catoire @@aut@@ C. Boone @@aut@@ T. Blumenstock @@aut@@ P. F. Bernath @@aut@@ K. A. Walker @@aut@@ T. E. Kerzenmacher @@aut@@ M. A. Wolff @@aut@@ K. Strong @@aut@@ A. Strandberg @@aut@@ J. Taylor @@aut@@ C. Tétard @@aut@@ M. Toohey @@aut@@ J. Urban @@aut@@ T. Warneke @@aut@@ S. Wood @@aut@@
publishDateDaySort_date	2008-01-01T00:00:00Z
hierarchy_top_id	092499996
id	DOAJ073691321
language_de	englisch
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Stiller</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Validation of ACE-FTS N2O measurements</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2008</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. 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callnumber-first	Q - Science
author	G. P. Stiller
spellingShingle	G. P. Stiller misc QC1-999 misc QD1-999 misc Physics misc Chemistry Validation of ACE-FTS N2O measurements
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topic_title	QC1-999 QD1-999 Validation of ACE-FTS N2O measurements
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title	Validation of ACE-FTS N2O measurements
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title_full	Validation of ACE-FTS N2O measurements
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author_browse	G. P. Stiller C. Senten O. Schrems K. Semeniuk M. Schneider C. Robert M. Ridolfi P. Raspollini C. Piccolo J. Notholt D. P. Murtagh S. Mikuteit J. Mellqvist J. C. McConnell E. Mahieu A. Lambert H. Kuellmann J. Kuttippurath K. Jucks N. Jones J. J. Jin D. W. T. Griffith N. Glatthor M. Höpfner J. Hannigan E. Dupuy P. Duchatelet M. De Mazière P. Demoulin M. Coffey V. Catoire C. Boone T. Blumenstock P. F. Bernath K. A. Walker T. E. Kerzenmacher M. A. Wolff K. Strong A. Strandberg J. Taylor C. Tétard M. Toohey J. Urban T. Warneke S. Wood
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author-letter	G. P. Stiller
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title_sort	validation of ace-fts n2o measurements
callnumber	QC1-999
title_auth	Validation of ACE-FTS N2O measurements
abstract	The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data.
abstractGer	The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data.
abstract_unstemmed	The Atmospheric Chemistry Experiment (ACE), also known as SCISAT, was launched on 12 August 2003, carrying two instruments that measure vertical profiles of atmospheric constituents using the solar occultation technique. One of these instruments, the ACE Fourier Transform Spectrometer (ACE-FTS), is measuring volume mixing ratio (VMR) profiles of nitrous oxide (N<sub<2</sub<O) from the upper troposphere to the lower mesosphere at a vertical resolution of about 3–4 km. In this study, the quality of the ACE-FTS version 2.2 N<sub<2</sub<O data is assessed through comparisons with coincident measurements made by other satellite, balloon-borne, aircraft, and ground-based instruments. These consist of vertical profile comparisons with the SMR, MLS, and MIPAS satellite instruments, multiple aircraft flights of ASUR, and single balloon flights of SPIRALE and FIRS-2, and partial column comparisons with a network of ground-based Fourier Transform InfraRed spectrometers (FTIRs). Between 6 and 30 km, the mean absolute differences for the satellite comparisons lie between -42 ppbv and +17 ppbv, with most within +-20 ppbv. This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. Excellent correlation (<i<R</i<=0.964) is observed between the ACE-FTS and FTIR partial columns, with a slope of 1.01 and an intercept of -0.20 on the line fitted to the data.
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title_short	Validation of ACE-FTS N2O measurements
url	https://doaj.org/article/a072b29df2754870b9c5e22adcb7bd79 http://www.atmos-chem-phys.net/8/4759/2008/acp-8-4759-2008.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324
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author2	C. Senten O. Schrems K. Semeniuk M. Schneider C. Robert M. Ridolfi P. Raspollini C. Piccolo J. Notholt D. P. Murtagh S. Mikuteit J. Mellqvist J. C. McConnell E. Mahieu A. Lambert H. Kuellmann J. Kuttippurath K. Jucks N. Jones J. J. Jin D. W. T. Griffith N. Glatthor M. Höpfner J. Hannigan E. Dupuy P. Duchatelet M. De Mazière P. Demoulin M. Coffey V. Catoire C. Boone T. Blumenstock P. F. Bernath K. A. Walker T. E. Kerzenmacher M. A. Wolff K. Strong A. Strandberg J. Taylor C. Tétard M. Toohey J. Urban T. Warneke S. Wood
author2Str	C. Senten O. Schrems K. Semeniuk M. Schneider C. Robert M. Ridolfi P. Raspollini C. Piccolo J. Notholt D. P. Murtagh S. Mikuteit J. Mellqvist J. C. McConnell E. Mahieu A. Lambert H. Kuellmann J. Kuttippurath K. Jucks N. Jones J. J. Jin D. W. T. Griffith N. Glatthor M. Höpfner J. Hannigan E. Dupuy P. Duchatelet M. De Mazière P. Demoulin M. Coffey V. Catoire C. Boone T. Blumenstock P. F. Bernath K. A. Walker T. E. Kerzenmacher M. A. Wolff K. Strong A. Strandberg J. Taylor C. Tétard M. Toohey J. Urban T. Warneke S. Wood
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This corresponds to relative deviations from the mean that are within +-15%, except for comparisons with MIPAS near 30 km, for which they are as large as 22.5%. Between 18 and 30 km, the mean absolute differences for the satellite comparisons are generally within +-10 ppbv. From 30 to 60 km, the mean absolute differences are within +-4 ppbv, and are mostly between -2 and +1 ppbv. Given the small N<sub<2</sub<O VMR in this region, the relative deviations from the mean are therefore large at these altitudes, with most suggesting a negative bias in the ACE-FTS data between 30 and 50 km. In the comparisons with the FTIRs, the mean relative differences between the ACE-FTS and FTIR partial columns (which cover a mean altitude range of 14 to 27 km) are within +-5.6% for eleven of the twelve contributing stations. This mean relative difference is negative at ten stations, suggesting a small negative bias in the ACE-FTS partial columns over the altitude regions compared. 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Validation of ACE-FTS N2O measurements

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