A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects

Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 na...
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Autor*in:	Yi Tian [verfasserIn] Hanfu Wang [verfasserIn] Lanqin Yan [verfasserIn] Xianfeng Zhang [verfasserIn] Attia Falak [verfasserIn] Yanjun Guo [verfasserIn] Peipei Chen [verfasserIn] Fengliang Dong [verfasserIn] Lianfeng Sun [verfasserIn] Weiguo Chu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection

Übergeordnetes Werk:	In: Advanced Science - Wiley, 2015, 6(2019), 11, Seite n/a-n/a
Übergeordnetes Werk:	volume:6 ; year:2019 ; number:11 ; pages:n/a-n/a

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1002/advs.201900177

Katalog-ID:	DOAJ074096915

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520			\|a Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition.
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700	0		\|a Fengliang Dong \|e verfasserin \|4 aut
700	0		\|a Lianfeng Sun \|e verfasserin \|4 aut
700	0		\|a Weiguo Chu \|e verfasserin \|4 aut
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allfields	10.1002/advs.201900177 doi (DE-627)DOAJ074096915 (DE-599)DOAJ5d32f82a6e674bfdb9b2e1c4ee269ddf DE-627 ger DE-627 rakwb eng Yi Tian verfasserin aut A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition. localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q Hanfu Wang verfasserin aut Lanqin Yan verfasserin aut Xianfeng Zhang verfasserin aut Attia Falak verfasserin aut Yanjun Guo verfasserin aut Peipei Chen verfasserin aut Fengliang Dong verfasserin aut Lianfeng Sun verfasserin aut Weiguo Chu verfasserin aut In Advanced Science Wiley, 2015 6(2019), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:6 year:2019 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf kostenfrei https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 6 2019 11 n/a-n/a
spelling	10.1002/advs.201900177 doi (DE-627)DOAJ074096915 (DE-599)DOAJ5d32f82a6e674bfdb9b2e1c4ee269ddf DE-627 ger DE-627 rakwb eng Yi Tian verfasserin aut A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition. localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q Hanfu Wang verfasserin aut Lanqin Yan verfasserin aut Xianfeng Zhang verfasserin aut Attia Falak verfasserin aut Yanjun Guo verfasserin aut Peipei Chen verfasserin aut Fengliang Dong verfasserin aut Lianfeng Sun verfasserin aut Weiguo Chu verfasserin aut In Advanced Science Wiley, 2015 6(2019), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:6 year:2019 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf kostenfrei https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 6 2019 11 n/a-n/a
allfields_unstemmed	10.1002/advs.201900177 doi (DE-627)DOAJ074096915 (DE-599)DOAJ5d32f82a6e674bfdb9b2e1c4ee269ddf DE-627 ger DE-627 rakwb eng Yi Tian verfasserin aut A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition. localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q Hanfu Wang verfasserin aut Lanqin Yan verfasserin aut Xianfeng Zhang verfasserin aut Attia Falak verfasserin aut Yanjun Guo verfasserin aut Peipei Chen verfasserin aut Fengliang Dong verfasserin aut Lianfeng Sun verfasserin aut Weiguo Chu verfasserin aut In Advanced Science Wiley, 2015 6(2019), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:6 year:2019 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf kostenfrei https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 6 2019 11 n/a-n/a
allfieldsGer	10.1002/advs.201900177 doi (DE-627)DOAJ074096915 (DE-599)DOAJ5d32f82a6e674bfdb9b2e1c4ee269ddf DE-627 ger DE-627 rakwb eng Yi Tian verfasserin aut A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition. localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q Hanfu Wang verfasserin aut Lanqin Yan verfasserin aut Xianfeng Zhang verfasserin aut Attia Falak verfasserin aut Yanjun Guo verfasserin aut Peipei Chen verfasserin aut Fengliang Dong verfasserin aut Lianfeng Sun verfasserin aut Weiguo Chu verfasserin aut In Advanced Science Wiley, 2015 6(2019), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:6 year:2019 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf kostenfrei https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 6 2019 11 n/a-n/a
allfieldsSound	10.1002/advs.201900177 doi (DE-627)DOAJ074096915 (DE-599)DOAJ5d32f82a6e674bfdb9b2e1c4ee269ddf DE-627 ger DE-627 rakwb eng Yi Tian verfasserin aut A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition. localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q Hanfu Wang verfasserin aut Lanqin Yan verfasserin aut Xianfeng Zhang verfasserin aut Attia Falak verfasserin aut Yanjun Guo verfasserin aut Peipei Chen verfasserin aut Fengliang Dong verfasserin aut Lianfeng Sun verfasserin aut Weiguo Chu verfasserin aut In Advanced Science Wiley, 2015 6(2019), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:6 year:2019 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf kostenfrei https://doi.org/10.1002/advs.201900177 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 6 2019 11 n/a-n/a
language	English
source	In Advanced Science 6(2019), 11, Seite n/a-n/a volume:6 year:2019 number:11 pages:n/a-n/a
sourceStr	In Advanced Science 6(2019), 11, Seite n/a-n/a volume:6 year:2019 number:11 pages:n/a-n/a
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection Science Q
isfreeaccess_bool	true
container_title	Advanced Science
authorswithroles_txt_mv	Yi Tian @@aut@@ Hanfu Wang @@aut@@ Lanqin Yan @@aut@@ Xianfeng Zhang @@aut@@ Attia Falak @@aut@@ Yanjun Guo @@aut@@ Peipei Chen @@aut@@ Fengliang Dong @@aut@@ Lianfeng Sun @@aut@@ Weiguo Chu @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	817357777
id	DOAJ074096915
language_de	englisch
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author	Yi Tian
spellingShingle	Yi Tian misc localized surface plasmon resonance (LSPR) misc quantification of multiple coupling effects misc SERS probe design misc surface plasmon polariton (SPP) misc trace detection misc Science misc Q A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects
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topic_title	A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects localized surface plasmon resonance (LSPR) quantification of multiple coupling effects SERS probe design surface plasmon polariton (SPP) trace detection
topic	misc localized surface plasmon resonance (LSPR) misc quantification of multiple coupling effects misc SERS probe design misc surface plasmon polariton (SPP) misc trace detection misc Science misc Q
topic_unstemmed	misc localized surface plasmon resonance (LSPR) misc quantification of multiple coupling effects misc SERS probe design misc surface plasmon polariton (SPP) misc trace detection misc Science misc Q
topic_browse	misc localized surface plasmon resonance (LSPR) misc quantification of multiple coupling effects misc SERS probe design misc surface plasmon polariton (SPP) misc trace detection misc Science misc Q
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title	A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects
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title_full	A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects
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author_browse	Yi Tian Hanfu Wang Lanqin Yan Xianfeng Zhang Attia Falak Yanjun Guo Peipei Chen Fengliang Dong Lianfeng Sun Weiguo Chu
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title_sort	generalized methodology of designing 3d sers probes with superior detection limit and uniformity by maximizing multiple coupling effects
title_auth	A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects
abstract	Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition.
abstractGer	Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition.
abstract_unstemmed	Abstract Accurate design of high‐performance 3D surface‐enhanced Raman scattering (SERS) probes is the desired target, which is possibly implemented with a prerequisite of quantifying formidable multiple coupling effects involved. Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition.
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title_short	A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects
url	https://doi.org/10.1002/advs.201900177 https://doaj.org/article/5d32f82a6e674bfdb9b2e1c4ee269ddf https://doaj.org/toc/2198-3844
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up_date	2024-07-03T21:19:03.047Z
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Herein, by combining theory and experiments on 3D periodic Au/SiO2 nanogrid models, a generalized methodology of accurately designing high performance 3D SERS probes is developed. Structural symmetry, dimensions, Au roughness, and polarization are successfully correlated quantitatively to intrinsic localized electromagnetic field (EMF) enhancements by calculating surface plasmon polariton (SPP), localized surface plasmon resonance (LSPR), optical standing wave effects, and their couplings theoretically, which is experimentally verified. The hexagonal SERS probes optimized by this methodology realize over two orders of magnitudes (405 times) improvement of detection limit for Rhodamine 6G model molecules (2.17 × 10−11 m) compared to the unoptimized probes with the same number density of hot spots, an enhancement factor of 3.4 × 108, a uniformity of 5.52%, and are successfully applied to the detection of 5 × 10−11 m Hg ions in water. This unambiguously results from the Au roughness‐independent extra 144% contribution of LSPR effects excited by SPP interference waves as secondary sources, which is very unusual to be beyond the conventional recognition.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">localized surface plasmon resonance (LSPR)</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">quantification of multiple coupling effects</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">SERS probe design</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">surface plasmon polariton (SPP)</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">trace detection</subfield></datafield><datafield tag="653" ind1=" " ind2="0"><subfield code="a">Science</subfield></datafield><datafield tag="653" ind1=" " ind2="0"><subfield code="a">Q</subfield></datafield><datafield tag="700" ind1="0" 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A Generalized Methodology of Designing 3D SERS Probes with Superior Detection Limit and Uniformity by Maximizing Multiple Coupling Effects

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