Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach
Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead hali...
Ausführliche Beschreibung
Autor*in: |
Yu Sun [verfasserIn] Jin Chen [verfasserIn] Fengchao Wang [verfasserIn] Yi Yin [verfasserIn] Yan Jin [verfasserIn] Jun Wang [verfasserIn] Xiaogai Peng [verfasserIn] Ruiyi Han [verfasserIn] Canyun Zhang [verfasserIn] Jinfang Kong [verfasserIn] Jing Yang [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2021 |
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In: Nanomaterials - MDPI AG, 2012, 11(2021), 12, p 3242 |
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Übergeordnetes Werk: |
volume:11 ; year:2021 ; number:12, p 3242 |
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DOI / URN: |
10.3390/nano11123242 |
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Katalog-ID: |
DOAJ074352946 |
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520 | |a Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. | ||
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10.3390/nano11123242 doi (DE-627)DOAJ074352946 (DE-599)DOAJef57581bcf75463384c1dd8580f0ab13 DE-627 ger DE-627 rakwb eng QD1-999 Yu Sun verfasserin aut Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. MnCl<sub<2</sub< doping CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< thin films solution spraying Chemistry Jin Chen verfasserin aut Fengchao Wang verfasserin aut Yi Yin verfasserin aut Yan Jin verfasserin aut Jun Wang verfasserin aut Xiaogai Peng verfasserin aut Ruiyi Han verfasserin aut Canyun Zhang verfasserin aut Jinfang Kong verfasserin aut Jing Yang verfasserin aut In Nanomaterials MDPI AG, 2012 11(2021), 12, p 3242 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:11 year:2021 number:12, p 3242 https://doi.org/10.3390/nano11123242 kostenfrei https://doaj.org/article/ef57581bcf75463384c1dd8580f0ab13 kostenfrei https://www.mdpi.com/2079-4991/11/12/3242 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 11 2021 12, p 3242 |
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10.3390/nano11123242 doi (DE-627)DOAJ074352946 (DE-599)DOAJef57581bcf75463384c1dd8580f0ab13 DE-627 ger DE-627 rakwb eng QD1-999 Yu Sun verfasserin aut Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. MnCl<sub<2</sub< doping CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< thin films solution spraying Chemistry Jin Chen verfasserin aut Fengchao Wang verfasserin aut Yi Yin verfasserin aut Yan Jin verfasserin aut Jun Wang verfasserin aut Xiaogai Peng verfasserin aut Ruiyi Han verfasserin aut Canyun Zhang verfasserin aut Jinfang Kong verfasserin aut Jing Yang verfasserin aut In Nanomaterials MDPI AG, 2012 11(2021), 12, p 3242 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:11 year:2021 number:12, p 3242 https://doi.org/10.3390/nano11123242 kostenfrei https://doaj.org/article/ef57581bcf75463384c1dd8580f0ab13 kostenfrei https://www.mdpi.com/2079-4991/11/12/3242 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 11 2021 12, p 3242 |
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10.3390/nano11123242 doi (DE-627)DOAJ074352946 (DE-599)DOAJef57581bcf75463384c1dd8580f0ab13 DE-627 ger DE-627 rakwb eng QD1-999 Yu Sun verfasserin aut Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. MnCl<sub<2</sub< doping CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< thin films solution spraying Chemistry Jin Chen verfasserin aut Fengchao Wang verfasserin aut Yi Yin verfasserin aut Yan Jin verfasserin aut Jun Wang verfasserin aut Xiaogai Peng verfasserin aut Ruiyi Han verfasserin aut Canyun Zhang verfasserin aut Jinfang Kong verfasserin aut Jing Yang verfasserin aut In Nanomaterials MDPI AG, 2012 11(2021), 12, p 3242 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:11 year:2021 number:12, p 3242 https://doi.org/10.3390/nano11123242 kostenfrei https://doaj.org/article/ef57581bcf75463384c1dd8580f0ab13 kostenfrei https://www.mdpi.com/2079-4991/11/12/3242 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 11 2021 12, p 3242 |
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10.3390/nano11123242 doi (DE-627)DOAJ074352946 (DE-599)DOAJef57581bcf75463384c1dd8580f0ab13 DE-627 ger DE-627 rakwb eng QD1-999 Yu Sun verfasserin aut Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. MnCl<sub<2</sub< doping CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< thin films solution spraying Chemistry Jin Chen verfasserin aut Fengchao Wang verfasserin aut Yi Yin verfasserin aut Yan Jin verfasserin aut Jun Wang verfasserin aut Xiaogai Peng verfasserin aut Ruiyi Han verfasserin aut Canyun Zhang verfasserin aut Jinfang Kong verfasserin aut Jing Yang verfasserin aut In Nanomaterials MDPI AG, 2012 11(2021), 12, p 3242 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:11 year:2021 number:12, p 3242 https://doi.org/10.3390/nano11123242 kostenfrei https://doaj.org/article/ef57581bcf75463384c1dd8580f0ab13 kostenfrei https://www.mdpi.com/2079-4991/11/12/3242 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 11 2021 12, p 3242 |
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Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach |
abstract |
Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. |
abstractGer |
Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. |
abstract_unstemmed |
Nowadays, Mn-doping is considered as a promising dissolution for the heavy usage of toxic lead in CsPbX<sub<3</sub< perovskite material. Interestingly, Mn-doping also introduces an additional photoluminescence band, which is favorable to enrich the emission gamut of this cesium lead halide. Here, a solution spraying strategy was employed for the direct preparation of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< film through MnCl<sub<2</sub< doping in host CsPbBr<sub<3</sub< material. The possible fabrication mechanism of the provided approach and the dependences of material properties on Mn-doping were investigated in detail. As the results shown, Pb was partially substituted by Mn as expected. With the ratio of PbBr<sub<2</sub<:MnCl<sub<2</sub< increasing from 3:0 to 1:1, the obtained film separately featured green, cyan, orange-red and pink-red emission, which was caused by the energy transferring process. Moreover, the combining energy of Cs, Pb, and Mn gradually red-shifted resulted from the formation of Cs-Cl, Pb-Cl and Mn-Br coordination bonding as MnCl<sub<2</sub< doping increased. In addition, the weight of short decay lifetime of prepared samples increased with the doping rising, which indicated a better exciton emission and less defect-related transition. The aiming of current work is to provide a new possibility for the facile preparation of Mn-doping CsPbX<sub<3</sub< film material. |
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container_issue |
12, p 3242 |
title_short |
Direct Fabrication of CsPb<sub<x</sub<Mn<sub<1−x</sub<(Br,Cl)<sub<3</sub< Thin Film by a Facile Solution Spraying Approach |
url |
https://doi.org/10.3390/nano11123242 https://doaj.org/article/ef57581bcf75463384c1dd8580f0ab13 https://www.mdpi.com/2079-4991/11/12/3242 https://doaj.org/toc/2079-4991 |
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author2 |
Jin Chen Fengchao Wang Yi Yin Yan Jin Jun Wang Xiaogai Peng Ruiyi Han Canyun Zhang Jinfang Kong Jing Yang |
author2Str |
Jin Chen Fengchao Wang Yi Yin Yan Jin Jun Wang Xiaogai Peng Ruiyi Han Canyun Zhang Jinfang Kong Jing Yang |
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doi_str |
10.3390/nano11123242 |
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up_date |
2024-07-03T22:40:46.162Z |
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