Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis

Automobile shredder residue (ASR) pyrolysis produces solid, liquid, and gaseous products, particularly pyrolysis oil and gas, which could be used as renewable alternative energy resources. Due to the primary pyrolysis reaction not being complete, the yield of gaseous product is low. The pyrolysis ta...
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Gespeichert in:

Autor*in:	Bin Yang [verfasserIn] Ming Chen [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	automobile shredder residue (ASR) pyrolysis thermogravimetric analysis gas chromatograph gas chromatography mass spectrometry Fourier transform infrared spectrometry

Übergeordnetes Werk:	In: Polymers - MDPI AG, 2011, 12(2020), 11, p 2734
Übergeordnetes Werk:	volume:12 ; year:2020 ; number:11, p 2734

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/polym12112734

Katalog-ID:	DOAJ076575314

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520			\|a Automobile shredder residue (ASR) pyrolysis produces solid, liquid, and gaseous products, particularly pyrolysis oil and gas, which could be used as renewable alternative energy resources. Due to the primary pyrolysis reaction not being complete, the yield of gaseous product is low. The pyrolysis tar comprises chemically unstable volatiles before condensing into liquid. Understanding the characteristics of volatile products will aid the design and improvement of subsequent processes. In order to accurately analyze the chemical characteristics and yields of volatile products of ASR primary pyrolysis, TG–FTIR–GC/MS analysis technology was used. According to the analysis results of the Gram–Schmidt profiles, the 3D stack plots, and GC/MS chromatograms of MixASR, ASR, and its main components, the major pyrolytic products of ASR included alkanes, olefins, and alcohols, and both had dense and indistinguishable weak peaks in the wavenumber range of 1900–1400 cm<sup<−1</sup<. Many of these products have unstable or weaker chemical bonds, such as =CH–, =CH2, –C=C–, and –C=CH2. Hence, more syngas with higher heating values can be obtained with further catalytic pyrolysis gasification, steam gasification, or higher temperature pyrolysis.
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callnumber-first	Q - Science
author	Bin Yang
spellingShingle	Bin Yang misc QD241-441 misc automobile shredder residue (ASR) misc pyrolysis misc thermogravimetric analysis misc gas chromatograph misc gas chromatography mass spectrometry misc Fourier transform infrared spectrometry misc Organic chemistry Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis
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topic_title	QD241-441 Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis automobile shredder residue (ASR) pyrolysis thermogravimetric analysis gas chromatograph gas chromatography mass spectrometry Fourier transform infrared spectrometry
topic	misc QD241-441 misc automobile shredder residue (ASR) misc pyrolysis misc thermogravimetric analysis misc gas chromatograph misc gas chromatography mass spectrometry misc Fourier transform infrared spectrometry misc Organic chemistry
topic_unstemmed	misc QD241-441 misc automobile shredder residue (ASR) misc pyrolysis misc thermogravimetric analysis misc gas chromatograph misc gas chromatography mass spectrometry misc Fourier transform infrared spectrometry misc Organic chemistry
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title	Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis
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title_full	Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis
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title_sort	py–ftir–gc/ms analysis of volatile products of automobile shredder residue pyrolysis
callnumber	QD241-441
title_auth	Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis
abstract	Automobile shredder residue (ASR) pyrolysis produces solid, liquid, and gaseous products, particularly pyrolysis oil and gas, which could be used as renewable alternative energy resources. Due to the primary pyrolysis reaction not being complete, the yield of gaseous product is low. The pyrolysis tar comprises chemically unstable volatiles before condensing into liquid. Understanding the characteristics of volatile products will aid the design and improvement of subsequent processes. In order to accurately analyze the chemical characteristics and yields of volatile products of ASR primary pyrolysis, TG–FTIR–GC/MS analysis technology was used. According to the analysis results of the Gram–Schmidt profiles, the 3D stack plots, and GC/MS chromatograms of MixASR, ASR, and its main components, the major pyrolytic products of ASR included alkanes, olefins, and alcohols, and both had dense and indistinguishable weak peaks in the wavenumber range of 1900–1400 cm<sup<−1</sup<. Many of these products have unstable or weaker chemical bonds, such as =CH–, =CH2, –C=C–, and –C=CH2. Hence, more syngas with higher heating values can be obtained with further catalytic pyrolysis gasification, steam gasification, or higher temperature pyrolysis.
abstractGer	Automobile shredder residue (ASR) pyrolysis produces solid, liquid, and gaseous products, particularly pyrolysis oil and gas, which could be used as renewable alternative energy resources. Due to the primary pyrolysis reaction not being complete, the yield of gaseous product is low. The pyrolysis tar comprises chemically unstable volatiles before condensing into liquid. Understanding the characteristics of volatile products will aid the design and improvement of subsequent processes. In order to accurately analyze the chemical characteristics and yields of volatile products of ASR primary pyrolysis, TG–FTIR–GC/MS analysis technology was used. According to the analysis results of the Gram–Schmidt profiles, the 3D stack plots, and GC/MS chromatograms of MixASR, ASR, and its main components, the major pyrolytic products of ASR included alkanes, olefins, and alcohols, and both had dense and indistinguishable weak peaks in the wavenumber range of 1900–1400 cm<sup<−1</sup<. Many of these products have unstable or weaker chemical bonds, such as =CH–, =CH2, –C=C–, and –C=CH2. Hence, more syngas with higher heating values can be obtained with further catalytic pyrolysis gasification, steam gasification, or higher temperature pyrolysis.
abstract_unstemmed	Automobile shredder residue (ASR) pyrolysis produces solid, liquid, and gaseous products, particularly pyrolysis oil and gas, which could be used as renewable alternative energy resources. Due to the primary pyrolysis reaction not being complete, the yield of gaseous product is low. The pyrolysis tar comprises chemically unstable volatiles before condensing into liquid. Understanding the characteristics of volatile products will aid the design and improvement of subsequent processes. In order to accurately analyze the chemical characteristics and yields of volatile products of ASR primary pyrolysis, TG–FTIR–GC/MS analysis technology was used. According to the analysis results of the Gram–Schmidt profiles, the 3D stack plots, and GC/MS chromatograms of MixASR, ASR, and its main components, the major pyrolytic products of ASR included alkanes, olefins, and alcohols, and both had dense and indistinguishable weak peaks in the wavenumber range of 1900–1400 cm<sup<−1</sup<. Many of these products have unstable or weaker chemical bonds, such as =CH–, =CH2, –C=C–, and –C=CH2. Hence, more syngas with higher heating values can be obtained with further catalytic pyrolysis gasification, steam gasification, or higher temperature pyrolysis.
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title_short	Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis
url	https://doi.org/10.3390/polym12112734 https://doaj.org/article/1f6459156786436686c46ca8a84d7dc6 https://www.mdpi.com/2073-4360/12/11/2734 https://doaj.org/toc/2073-4360
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up_date	2024-07-03T21:16:30.472Z
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Py–FTIR–GC/MS Analysis of Volatile Products of Automobile Shredder Residue Pyrolysis

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