High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors

Abstract With the development of the non-fullerene acceptors (NFAs), the use of ternary organic photovoltaic devices based on a fullerene acceptor and a NFA is now widespread, and the merits of both acceptor types can be fully utilized. However, the effective approach of enhancing device performance...
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Autor*in:	Yuanyuan Jiang [verfasserIn] Xiaozhang Zhu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	ternary organic solar cells fullerene acceptors non-fullerene acceptors power conversion efficiency

Übergeordnetes Werk:	In: Organic Materials - Georg Thieme Verlag, 2020, 03(2021), 02, Seite 254-276
Übergeordnetes Werk:	volume:03 ; year:2021 ; number:02 ; pages:254-276

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1055/a-1472-3989

Katalog-ID:	DOAJ078992494

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520			\|a Abstract With the development of the non-fullerene acceptors (NFAs), the use of ternary organic photovoltaic devices based on a fullerene acceptor and a NFA is now widespread, and the merits of both acceptor types can be fully utilized. However, the effective approach of enhancing device performance is adjusting the charge dynamics and the thin-film morphology of the active layer via introducing the second acceptor, which would significantly impact the open-circuit voltage, the short-circuit current, and the fill factor, thus strongly affecting device efficiency. The functions of the second acceptor in a ternary organic solar cell with a fullerene acceptor and a NFA are summarized here. These include a broader absorption spectrum; formation of a cascade energy level or energy transfer; modified thin-film morphology including phase separation, effects on crystallinity, size, and purity of domain; and vertical distribution along with improved charge dynamics like exciton dissociation and charge transport, collection, and recombination. Then, we discuss the hierarchical morphology in ternary solar cells, which may benefit device performance, and the outlook of the ternary device.
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callnumber-first	Q - Science
author	Yuanyuan Jiang
spellingShingle	Yuanyuan Jiang misc QD1-999 misc ternary organic solar cells misc fullerene acceptors misc non-fullerene acceptors misc power conversion efficiency misc Chemistry High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors
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topic_title	QD1-999 High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors ternary organic solar cells fullerene acceptors non-fullerene acceptors power conversion efficiency
topic	misc QD1-999 misc ternary organic solar cells misc fullerene acceptors misc non-fullerene acceptors misc power conversion efficiency misc Chemistry
topic_unstemmed	misc QD1-999 misc ternary organic solar cells misc fullerene acceptors misc non-fullerene acceptors misc power conversion efficiency misc Chemistry
topic_browse	misc QD1-999 misc ternary organic solar cells misc fullerene acceptors misc non-fullerene acceptors misc power conversion efficiency misc Chemistry
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title	High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors
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title_sort	high-performance ternary organic solar cells enabled by synergizing fullerene and non-fullerene acceptors
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title_auth	High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors
abstract	Abstract With the development of the non-fullerene acceptors (NFAs), the use of ternary organic photovoltaic devices based on a fullerene acceptor and a NFA is now widespread, and the merits of both acceptor types can be fully utilized. However, the effective approach of enhancing device performance is adjusting the charge dynamics and the thin-film morphology of the active layer via introducing the second acceptor, which would significantly impact the open-circuit voltage, the short-circuit current, and the fill factor, thus strongly affecting device efficiency. The functions of the second acceptor in a ternary organic solar cell with a fullerene acceptor and a NFA are summarized here. These include a broader absorption spectrum; formation of a cascade energy level or energy transfer; modified thin-film morphology including phase separation, effects on crystallinity, size, and purity of domain; and vertical distribution along with improved charge dynamics like exciton dissociation and charge transport, collection, and recombination. Then, we discuss the hierarchical morphology in ternary solar cells, which may benefit device performance, and the outlook of the ternary device.
abstractGer	Abstract With the development of the non-fullerene acceptors (NFAs), the use of ternary organic photovoltaic devices based on a fullerene acceptor and a NFA is now widespread, and the merits of both acceptor types can be fully utilized. However, the effective approach of enhancing device performance is adjusting the charge dynamics and the thin-film morphology of the active layer via introducing the second acceptor, which would significantly impact the open-circuit voltage, the short-circuit current, and the fill factor, thus strongly affecting device efficiency. The functions of the second acceptor in a ternary organic solar cell with a fullerene acceptor and a NFA are summarized here. These include a broader absorption spectrum; formation of a cascade energy level or energy transfer; modified thin-film morphology including phase separation, effects on crystallinity, size, and purity of domain; and vertical distribution along with improved charge dynamics like exciton dissociation and charge transport, collection, and recombination. Then, we discuss the hierarchical morphology in ternary solar cells, which may benefit device performance, and the outlook of the ternary device.
abstract_unstemmed	Abstract With the development of the non-fullerene acceptors (NFAs), the use of ternary organic photovoltaic devices based on a fullerene acceptor and a NFA is now widespread, and the merits of both acceptor types can be fully utilized. However, the effective approach of enhancing device performance is adjusting the charge dynamics and the thin-film morphology of the active layer via introducing the second acceptor, which would significantly impact the open-circuit voltage, the short-circuit current, and the fill factor, thus strongly affecting device efficiency. The functions of the second acceptor in a ternary organic solar cell with a fullerene acceptor and a NFA are summarized here. These include a broader absorption spectrum; formation of a cascade energy level or energy transfer; modified thin-film morphology including phase separation, effects on crystallinity, size, and purity of domain; and vertical distribution along with improved charge dynamics like exciton dissociation and charge transport, collection, and recombination. Then, we discuss the hierarchical morphology in ternary solar cells, which may benefit device performance, and the outlook of the ternary device.
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title_short	High-Performance Ternary Organic Solar Cells Enabled by Synergizing Fullerene and Non-fullerene Acceptors
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