Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction

Producing chemical fuels from sunlight is a sustainable way to utilize solar energy and reduce carbon emissions. Within the current photovoltaic-electrolysis or photoelectrochemical-based solar fuel generation system, electrochemical CO<sub<2</sub< reduction is the key step. Although the...
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Autor*in:	Ya Liu [verfasserIn] Dan Lei [verfasserIn] Xiaoqi Guo [verfasserIn] Tengfei Ma [verfasserIn] Feng Wang [verfasserIn] Yubin Chen [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	electrochemical CO CO formate fuel

Übergeordnetes Werk:	In: Energies - MDPI AG, 2008, 15(2022), 1, p 335
Übergeordnetes Werk:	volume:15 ; year:2022 ; number:1, p 335

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/en15010335

Katalog-ID:	DOAJ079385389

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allfieldsSound	10.3390/en15010335 doi (DE-627)DOAJ079385389 (DE-599)DOAJd74b18f09fcc44eb95cc946b4547f684 DE-627 ger DE-627 rakwb eng Ya Liu verfasserin aut Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Producing chemical fuels from sunlight is a sustainable way to utilize solar energy and reduce carbon emissions. Within the current photovoltaic-electrolysis or photoelectrochemical-based solar fuel generation system, electrochemical CO<sub<2</sub< reduction is the key step. Although there has been important progress in developing new materials and devices, scaling up electrochemical CO<sub<2</sub< reduction is essential to promote the industrial application of this technology. In this work, we use Ag and In as the representative electrocatalyst for producing gas and liquid products in both small and big electrochemical cells. We find that gas production is blocked more easily than liquid products when scaling up the electrochemical cell. Simulation results show that the generated gas product, CO, forms bubbles on the surface of the electrocatalyst, thus blocking the transport of CO<sub<2</sub<, while there is no such trouble for producing the liquid product such as formate. This work provides methods for studying the mass transfer of CO, and it is also an important reference for scaling up solar fuel generation devices that are constructed based on electrochemical CO<sub<2</sub< reduction. electrochemical CO<sub<2</sub< CO formate fuel Technology T Dan Lei verfasserin aut Xiaoqi Guo verfasserin aut Tengfei Ma verfasserin aut Feng Wang verfasserin aut Yubin Chen verfasserin aut In Energies MDPI AG, 2008 15(2022), 1, p 335 (DE-627)572083742 (DE-600)2437446-5 19961073 nnns volume:15 year:2022 number:1, p 335 https://doi.org/10.3390/en15010335 kostenfrei https://doaj.org/article/d74b18f09fcc44eb95cc946b4547f684 kostenfrei https://www.mdpi.com/1996-1073/15/1/335 kostenfrei https://doaj.org/toc/1996-1073 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 15 2022 1, p 335
language	English
source	In Energies 15(2022), 1, p 335 volume:15 year:2022 number:1, p 335
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authorswithroles_txt_mv	Ya Liu @@aut@@ Dan Lei @@aut@@ Xiaoqi Guo @@aut@@ Tengfei Ma @@aut@@ Feng Wang @@aut@@ Yubin Chen @@aut@@
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author	Ya Liu
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topic_title	Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction electrochemical CO<sub<2</sub< CO formate fuel
topic	misc electrochemical misc CO<sub<2</sub< misc CO misc formate misc fuel misc Technology misc T
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title	Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction
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title_sort	scale effect on producing gaseous and liquid chemical fuels via co<sub<2</sub< reduction
title_auth	Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction
abstract	Producing chemical fuels from sunlight is a sustainable way to utilize solar energy and reduce carbon emissions. Within the current photovoltaic-electrolysis or photoelectrochemical-based solar fuel generation system, electrochemical CO<sub<2</sub< reduction is the key step. Although there has been important progress in developing new materials and devices, scaling up electrochemical CO<sub<2</sub< reduction is essential to promote the industrial application of this technology. In this work, we use Ag and In as the representative electrocatalyst for producing gas and liquid products in both small and big electrochemical cells. We find that gas production is blocked more easily than liquid products when scaling up the electrochemical cell. Simulation results show that the generated gas product, CO, forms bubbles on the surface of the electrocatalyst, thus blocking the transport of CO<sub<2</sub<, while there is no such trouble for producing the liquid product such as formate. This work provides methods for studying the mass transfer of CO, and it is also an important reference for scaling up solar fuel generation devices that are constructed based on electrochemical CO<sub<2</sub< reduction.
abstractGer	Producing chemical fuels from sunlight is a sustainable way to utilize solar energy and reduce carbon emissions. Within the current photovoltaic-electrolysis or photoelectrochemical-based solar fuel generation system, electrochemical CO<sub<2</sub< reduction is the key step. Although there has been important progress in developing new materials and devices, scaling up electrochemical CO<sub<2</sub< reduction is essential to promote the industrial application of this technology. In this work, we use Ag and In as the representative electrocatalyst for producing gas and liquid products in both small and big electrochemical cells. We find that gas production is blocked more easily than liquid products when scaling up the electrochemical cell. Simulation results show that the generated gas product, CO, forms bubbles on the surface of the electrocatalyst, thus blocking the transport of CO<sub<2</sub<, while there is no such trouble for producing the liquid product such as formate. This work provides methods for studying the mass transfer of CO, and it is also an important reference for scaling up solar fuel generation devices that are constructed based on electrochemical CO<sub<2</sub< reduction.
abstract_unstemmed	Producing chemical fuels from sunlight is a sustainable way to utilize solar energy and reduce carbon emissions. Within the current photovoltaic-electrolysis or photoelectrochemical-based solar fuel generation system, electrochemical CO<sub<2</sub< reduction is the key step. Although there has been important progress in developing new materials and devices, scaling up electrochemical CO<sub<2</sub< reduction is essential to promote the industrial application of this technology. In this work, we use Ag and In as the representative electrocatalyst for producing gas and liquid products in both small and big electrochemical cells. We find that gas production is blocked more easily than liquid products when scaling up the electrochemical cell. Simulation results show that the generated gas product, CO, forms bubbles on the surface of the electrocatalyst, thus blocking the transport of CO<sub<2</sub<, while there is no such trouble for producing the liquid product such as formate. This work provides methods for studying the mass transfer of CO, and it is also an important reference for scaling up solar fuel generation devices that are constructed based on electrochemical CO<sub<2</sub< reduction.
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title_short	Scale Effect on Producing Gaseous and Liquid Chemical Fuels via CO<sub<2</sub< Reduction
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