One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery

Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling...
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Autor*in:	Shi Chen [verfasserIn] Yifeng Huang [verfasserIn] Haoran Li [verfasserIn] Fuxin Wang [verfasserIn] Wei Xu [verfasserIn] Dezhou Zheng [verfasserIn] Xihong Lu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Ni-Zn battery NiSe one-pot synthesis cathode

Übergeordnetes Werk:	In: Molecules - MDPI AG, 2003, 28(2023), 3, p 1098
Übergeordnetes Werk:	volume:28 ; year:2023 ; number:3, p 1098

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/molecules28031098

Katalog-ID:	DOAJ080615511

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520			\|a Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. This work provides a simple attempt to design a high-performance layered cathode material for aqueous Ni-Zn batteries.
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spelling	10.3390/molecules28031098 doi (DE-627)DOAJ080615511 (DE-599)DOAJe92c620e6af74f1983cb43bb0da7e04a DE-627 ger DE-627 rakwb eng QD241-441 Shi Chen verfasserin aut One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. This work provides a simple attempt to design a high-performance layered cathode material for aqueous Ni-Zn batteries. Ni-Zn battery NiSe<sub<2</sub< one-pot synthesis cathode Organic chemistry Yifeng Huang verfasserin aut Haoran Li verfasserin aut Fuxin Wang verfasserin aut Wei Xu verfasserin aut Dezhou Zheng verfasserin aut Xihong Lu verfasserin aut In Molecules MDPI AG, 2003 28(2023), 3, p 1098 (DE-627)311313132 (DE-600)2008644-1 14203049 nnns volume:28 year:2023 number:3, p 1098 https://doi.org/10.3390/molecules28031098 kostenfrei https://doaj.org/article/e92c620e6af74f1983cb43bb0da7e04a kostenfrei https://www.mdpi.com/1420-3049/28/3/1098 kostenfrei https://doaj.org/toc/1420-3049 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 28 2023 3, p 1098
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callnumber-first	Q - Science
author	Shi Chen
spellingShingle	Shi Chen misc QD241-441 misc Ni-Zn battery misc NiSe<sub<2</sub< misc one-pot synthesis misc cathode misc Organic chemistry One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery
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topic_title	QD241-441 One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery Ni-Zn battery NiSe<sub<2</sub< one-pot synthesis cathode
topic	misc QD241-441 misc Ni-Zn battery misc NiSe<sub<2</sub< misc one-pot synthesis misc cathode misc Organic chemistry
topic_unstemmed	misc QD241-441 misc Ni-Zn battery misc NiSe<sub<2</sub< misc one-pot synthesis misc cathode misc Organic chemistry
topic_browse	misc QD241-441 misc Ni-Zn battery misc NiSe<sub<2</sub< misc one-pot synthesis misc cathode misc Organic chemistry
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title	One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery
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title_full	One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery
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author_browse	Shi Chen Yifeng Huang Haoran Li Fuxin Wang Wei Xu Dezhou Zheng Xihong Lu
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title_sort	one-pot synthesis of nise<sub<2</sub< with layered structure for nickel-zinc battery
callnumber	QD241-441
title_auth	One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery
abstract	Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. This work provides a simple attempt to design a high-performance layered cathode material for aqueous Ni-Zn batteries.
abstractGer	Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. This work provides a simple attempt to design a high-performance layered cathode material for aqueous Ni-Zn batteries.
abstract_unstemmed	Transition metal organic framework materials and their selenides are considered to be one of the most promising cathode materials for nickel-zinc (denoted as Ni-Zn) batteries due to their low cost, environmental friendliness, and controllable microstructure. Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. This work provides a simple attempt to design a high-performance layered cathode material for aqueous Ni-Zn batteries.
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container_issue	3, p 1098
title_short	One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery
url	https://doi.org/10.3390/molecules28031098 https://doaj.org/article/e92c620e6af74f1983cb43bb0da7e04a https://www.mdpi.com/1420-3049/28/3/1098 https://doaj.org/toc/1420-3049
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author2	Yifeng Huang Haoran Li Fuxin Wang Wei Xu Dezhou Zheng Xihong Lu
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doi_str	10.3390/molecules28031098
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up_date	2024-07-03T15:37:10.836Z
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Yet, their low capacity and poor cycling performance severely restricts their further development. Herein, we developed a simple one-pot hydrothermal process to directly synthesize NiSe<sub<2</sub< (denotes as NiSe<sub<2</sub<-X based on the molar amount of SeO<sub<2</sub< added) stacked layered sheets. Benefiting from the peculiar architectures, the fabricated NiSe<sub<2</sub<−1//Zn battery based on NiSe<sub<2</sub< and the Zn plate exhibits a high specific capacity of 231.6 mAh g<sup<−1</sup< at 1 A g<sup<−1</sup<, and excellent rate performance (162.8 mAh g<sup<−1</sup< at 10 A g<sup<−1</sup<). In addition, the NiSe<sub<2</sub<//Zn battery also presents a satisfactory cycle life at the high current density of 8 A g<sup<−1</sup< (almost no decay compared to the initial specific capacity after 1000 cycles). Additionally, the battery device also exhibits a satisfactory energy density of 343.2 Wh kg<sup<−1</sup< and a peak power density of 11.7 kW kg<sup<−1</sup<. 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One-Pot Synthesis of NiSe<sub<2</sub< with Layered Structure for Nickel-Zinc Battery

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