Rabi oscillations in a stretching molecule

Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissocia...
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Autor*in:	Shengzhe Pan [verfasserIn] Chenxi Hu [verfasserIn] Wenbin Zhang [verfasserIn] Zhaohan Zhang [verfasserIn] Lianrong Zhou [verfasserIn] Chenxu Lu [verfasserIn] Peifen Lu [verfasserIn] Hongcheng Ni [verfasserIn] Jian Wu [verfasserIn] Feng He [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Übergeordnetes Werk:	In: Light: Science & Applications - Nature Publishing Group, 2014, 12(2023), 1, Seite 9
Übergeordnetes Werk:	volume:12 ; year:2023 ; number:1 ; pages:9

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1038/s41377-023-01075-9

Katalog-ID:	DOAJ080964060

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allfields	10.1038/s41377-023-01075-9 doi (DE-627)DOAJ080964060 (DE-599)DOAJcea6b7a3612a4b6bb469287b150e43fb DE-627 ger DE-627 rakwb eng TA1501-1820 QC350-467 Shengzhe Pan verfasserin aut Rabi oscillations in a stretching molecule 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules. Applied optics. Photonics Optics. Light Chenxi Hu verfasserin aut Wenbin Zhang verfasserin aut Zhaohan Zhang verfasserin aut Lianrong Zhou verfasserin aut Chenxu Lu verfasserin aut Peifen Lu verfasserin aut Hongcheng Ni verfasserin aut Jian Wu verfasserin aut Feng He verfasserin aut In Light: Science & Applications Nature Publishing Group, 2014 12(2023), 1, Seite 9 (DE-627)718632680 (DE-600)2662628-7 20477538 nnns volume:12 year:2023 number:1 pages:9 https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/article/cea6b7a3612a4b6bb469287b150e43fb kostenfrei https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/toc/2047-7538 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2023 1 9
spelling	10.1038/s41377-023-01075-9 doi (DE-627)DOAJ080964060 (DE-599)DOAJcea6b7a3612a4b6bb469287b150e43fb DE-627 ger DE-627 rakwb eng TA1501-1820 QC350-467 Shengzhe Pan verfasserin aut Rabi oscillations in a stretching molecule 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules. Applied optics. Photonics Optics. Light Chenxi Hu verfasserin aut Wenbin Zhang verfasserin aut Zhaohan Zhang verfasserin aut Lianrong Zhou verfasserin aut Chenxu Lu verfasserin aut Peifen Lu verfasserin aut Hongcheng Ni verfasserin aut Jian Wu verfasserin aut Feng He verfasserin aut In Light: Science & Applications Nature Publishing Group, 2014 12(2023), 1, Seite 9 (DE-627)718632680 (DE-600)2662628-7 20477538 nnns volume:12 year:2023 number:1 pages:9 https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/article/cea6b7a3612a4b6bb469287b150e43fb kostenfrei https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/toc/2047-7538 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2023 1 9
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allfieldsGer	10.1038/s41377-023-01075-9 doi (DE-627)DOAJ080964060 (DE-599)DOAJcea6b7a3612a4b6bb469287b150e43fb DE-627 ger DE-627 rakwb eng TA1501-1820 QC350-467 Shengzhe Pan verfasserin aut Rabi oscillations in a stretching molecule 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules. Applied optics. Photonics Optics. Light Chenxi Hu verfasserin aut Wenbin Zhang verfasserin aut Zhaohan Zhang verfasserin aut Lianrong Zhou verfasserin aut Chenxu Lu verfasserin aut Peifen Lu verfasserin aut Hongcheng Ni verfasserin aut Jian Wu verfasserin aut Feng He verfasserin aut In Light: Science & Applications Nature Publishing Group, 2014 12(2023), 1, Seite 9 (DE-627)718632680 (DE-600)2662628-7 20477538 nnns volume:12 year:2023 number:1 pages:9 https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/article/cea6b7a3612a4b6bb469287b150e43fb kostenfrei https://doi.org/10.1038/s41377-023-01075-9 kostenfrei https://doaj.org/toc/2047-7538 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 12 2023 1 9
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callnumber-first	T - Technology
author	Shengzhe Pan
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title	Rabi oscillations in a stretching molecule
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title_auth	Rabi oscillations in a stretching molecule
abstract	Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules.
abstractGer	Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules.
abstract_unstemmed	Abstract Rabi oscillation is an elementary laser-driven physical process in atoms and artificial atoms from solid-state systems, while it is rarely demonstrated in molecules. Here, we investigate the bond-length-dependent Rabi oscillations with varying Rabi frequencies in strong-laser-field dissociation of H2 +. The coupling of the bond stretching and Rabi oscillations makes the nuclei gain different kinetic energies while the electron is alternatively absorbing and emitting photons. The resulting proton kinetic energy spectra show rich structures beyond the prediction of the Floquet theorem and the well-accepted resonant one-photon dissociation pathway. Our study shows that the laser-driven Rabi oscillations accompanied by nuclear motions are essential to understanding the bond-breaking mechanism and provide a time-resolved perspective to manipulate rich dynamics of the strong-laser-field dissociation of molecules.
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title_short	Rabi oscillations in a stretching molecule
url	https://doi.org/10.1038/s41377-023-01075-9 https://doaj.org/article/cea6b7a3612a4b6bb469287b150e43fb https://doaj.org/toc/2047-7538
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