On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement

In this paper, a novel application of industrial waste, namely red mud (RM), in the abatement of two malodorous and harmful sulfur compounds, dimethyl disulfide (DMDS) and methyl mercaptan (MM), is presented. The effects of calcination and activations with hydrochloric acid or a mixture of hydrochlo...
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Autor*in:	Sanna Päivärinta-Antikainen [verfasserIn] Satu Ojala [verfasserIn] Satu Pitkäaho [verfasserIn] Lenka Matějová [verfasserIn] Riitta L. Keiski [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	circular economy industrial waste red mud volatile organic compound S-VOC malodorous organic compound

Übergeordnetes Werk:	In: Resources - MDPI AG, 2013, 12(2023), 1, p 9
Übergeordnetes Werk:	volume:12 ; year:2023 ; number:1, p 9

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/resources12010009

Katalog-ID:	DOAJ081710739

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authorswithroles_txt_mv	Sanna Päivärinta-Antikainen @@aut@@ Satu Ojala @@aut@@ Satu Pitkäaho @@aut@@ Lenka Matějová @@aut@@ Riitta L. Keiski @@aut@@
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author	Sanna Päivärinta-Antikainen
spellingShingle	Sanna Päivärinta-Antikainen misc circular economy misc industrial waste misc red mud misc volatile organic compound misc S-VOC misc malodorous organic compound misc Science misc Q On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement
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topic_title	On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement circular economy industrial waste red mud volatile organic compound S-VOC malodorous organic compound
topic	misc circular economy misc industrial waste misc red mud misc volatile organic compound misc S-VOC misc malodorous organic compound misc Science misc Q
topic_unstemmed	misc circular economy misc industrial waste misc red mud misc volatile organic compound misc S-VOC misc malodorous organic compound misc Science misc Q
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title	On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement
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title_full	On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement
author_sort	Sanna Päivärinta-Antikainen
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author_browse	Sanna Päivärinta-Antikainen Satu Ojala Satu Pitkäaho Lenka Matějová Riitta L. Keiski
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title_sort	on the utilization of modified red mud in dimethyl disulfide and methyl mercaptan emission abatement
title_auth	On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement
abstract	In this paper, a novel application of industrial waste, namely red mud (RM), in the abatement of two malodorous and harmful sulfur compounds, dimethyl disulfide (DMDS) and methyl mercaptan (MM), is presented. The effects of calcination and activations with hydrochloric acid or a mixture of hydrochloric and orthophosphoric acid on the properties and performance of RM are compared using laboratory-scale experiments. The RM-based materials were characterized by XRF, XRD, FE-SEM, N<sub<2</sub<-physisorption, TGA/DTA, and FTIR analyses. RM exhibits very promising catalytic properties in the abatement of both DMDS and MM. The hydrochloric acid-activated RM was the most active in both cases, which was explained by its rather high specific surface area (144 m<sup<2</sup< g<sup<−1</sup<), higher contents of Fe<sub<2</sub<O<sub<3</sub< and TiO<sub<2,</sub< as well as lower content of phosphorus. For both DMDS and MM, the main oxidation products were sulfur dioxide, carbon monoxide, and carbon dioxide. DMDS was observed as a reaction intermediate in MM oxidation. While the final conversions of DMDS and MM were high, the oxidation was not complete, indicated by the formation of carbon monoxide. Nevertheless, the modified RM appears as a very interesting alternative to the existing DMDS and MM abatement catalysts.
abstractGer	In this paper, a novel application of industrial waste, namely red mud (RM), in the abatement of two malodorous and harmful sulfur compounds, dimethyl disulfide (DMDS) and methyl mercaptan (MM), is presented. The effects of calcination and activations with hydrochloric acid or a mixture of hydrochloric and orthophosphoric acid on the properties and performance of RM are compared using laboratory-scale experiments. The RM-based materials were characterized by XRF, XRD, FE-SEM, N<sub<2</sub<-physisorption, TGA/DTA, and FTIR analyses. RM exhibits very promising catalytic properties in the abatement of both DMDS and MM. The hydrochloric acid-activated RM was the most active in both cases, which was explained by its rather high specific surface area (144 m<sup<2</sup< g<sup<−1</sup<), higher contents of Fe<sub<2</sub<O<sub<3</sub< and TiO<sub<2,</sub< as well as lower content of phosphorus. For both DMDS and MM, the main oxidation products were sulfur dioxide, carbon monoxide, and carbon dioxide. DMDS was observed as a reaction intermediate in MM oxidation. While the final conversions of DMDS and MM were high, the oxidation was not complete, indicated by the formation of carbon monoxide. Nevertheless, the modified RM appears as a very interesting alternative to the existing DMDS and MM abatement catalysts.
abstract_unstemmed	In this paper, a novel application of industrial waste, namely red mud (RM), in the abatement of two malodorous and harmful sulfur compounds, dimethyl disulfide (DMDS) and methyl mercaptan (MM), is presented. The effects of calcination and activations with hydrochloric acid or a mixture of hydrochloric and orthophosphoric acid on the properties and performance of RM are compared using laboratory-scale experiments. The RM-based materials were characterized by XRF, XRD, FE-SEM, N<sub<2</sub<-physisorption, TGA/DTA, and FTIR analyses. RM exhibits very promising catalytic properties in the abatement of both DMDS and MM. The hydrochloric acid-activated RM was the most active in both cases, which was explained by its rather high specific surface area (144 m<sup<2</sup< g<sup<−1</sup<), higher contents of Fe<sub<2</sub<O<sub<3</sub< and TiO<sub<2,</sub< as well as lower content of phosphorus. For both DMDS and MM, the main oxidation products were sulfur dioxide, carbon monoxide, and carbon dioxide. DMDS was observed as a reaction intermediate in MM oxidation. While the final conversions of DMDS and MM were high, the oxidation was not complete, indicated by the formation of carbon monoxide. Nevertheless, the modified RM appears as a very interesting alternative to the existing DMDS and MM abatement catalysts.
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title_short	On the Utilization of Modified Red Mud in Dimethyl Disulfide and Methyl Mercaptan Emission Abatement
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