Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batte...
Ausführliche Beschreibung
Autor*in: |
Xinghua Liang [verfasserIn] Xingtao Jiang [verfasserIn] Linxiao Lan [verfasserIn] Shuaibo Zeng [verfasserIn] Meihong Huang [verfasserIn] Dongxue Huang [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
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2022 |
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Übergeordnetes Werk: |
In: Nanomaterials - MDPI AG, 2012, 12(2022), 17, p 3069 |
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Übergeordnetes Werk: |
volume:12 ; year:2022 ; number:17, p 3069 |
Links: |
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DOI / URN: |
10.3390/nano12173069 |
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Katalog-ID: |
DOAJ084932457 |
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Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air |
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Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse. |
abstractGer |
Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse. |
abstract_unstemmed |
Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse. |
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