Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air

Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batte...
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Autor*in:	Xinghua Liang [verfasserIn] Xingtao Jiang [verfasserIn] Linxiao Lan [verfasserIn] Shuaibo Zeng [verfasserIn] Meihong Huang [verfasserIn] Dongxue Huang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	composite solid electrolyte lithium ion conductivity capacity retention flame retardancy

Übergeordnetes Werk:	In: Nanomaterials - MDPI AG, 2012, 12(2022), 17, p 3069
Übergeordnetes Werk:	volume:12 ; year:2022 ; number:17, p 3069

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DOI / URN:	10.3390/nano12173069

Katalog-ID:	DOAJ084932457

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language	English
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authorswithroles_txt_mv	Xinghua Liang @@aut@@ Xingtao Jiang @@aut@@ Linxiao Lan @@aut@@ Shuaibo Zeng @@aut@@ Meihong Huang @@aut@@ Dongxue Huang @@aut@@
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callnumber-first	Q - Science
author	Xinghua Liang
spellingShingle	Xinghua Liang misc QD1-999 misc composite solid electrolyte misc lithium ion conductivity misc capacity retention misc flame retardancy misc Chemistry Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
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topic_title	QD1-999 Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air composite solid electrolyte lithium ion conductivity capacity retention flame retardancy
topic	misc QD1-999 misc composite solid electrolyte misc lithium ion conductivity misc capacity retention misc flame retardancy misc Chemistry
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title	Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
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title_full	Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
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title_sort	preparation and study of a simple three-matrix solid electrolyte membrane in air
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title_auth	Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
abstract	Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse.
abstractGer	Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse.
abstract_unstemmed	Solid-state lithium batteries have attracted much attention due to their special properties of high safety and high energy density. Among them, the polymer electrolyte membrane with high ionic conductivity and a wide electrochemical window is a key part to achieve stable cycling of solid-state batteries. However, the low ionic conductivity and the high interfacial resistance limit its practical application. This work deals with the preparation of a composite solid electrolyte with high mechanical flexibility and non-flammability. Firstly, the crystallinity of the polymer is reduced, and the fluidity of Li<sup<+</sup< between the polymer segments is improved by tertiary polymer polymerization. Then, lithium salt is added to form a solpolymer solution to provide Li<sup<+</sup< and anion and then an inorganic solid electrolyte is added. As a result, the composite solid electrolyte has a Li<sup<+</sup< conductivity (3.18 × 10<sup<−4</sup< mS cm<sup<−1</sup<). The (LiNi<sub<0.5</sub<Mn<sub<1.5</sub<O<sub<4</sub<)LNMO/SPLL (PES-PVC-PVDF-LiBF<sub<4</sub<-LAZTP)/Li battery has a capacity retention rate of 98.4% after 100 cycles, which is much higher than that without inorganic oxides. This research provides an important reference for developing all-solid-state batteries in the greenhouse.
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title_short	Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air
url	https://doi.org/10.3390/nano12173069 https://doaj.org/article/30b28faed0684c8cafb93b3efe0b509d https://www.mdpi.com/2079-4991/12/17/3069 https://doaj.org/toc/2079-4991
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up_date	2024-07-04T01:09:30.343Z
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Preparation and Study of a Simple Three-Matrix Solid Electrolyte Membrane in Air

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