Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides

The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and fun...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Guannan Qian [verfasserIn] Xiaobiao Huang [verfasserIn] Jun-Sik Lee [verfasserIn] Piero Pianetta [verfasserIn] Yijin Liu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	free-electron laser battery layered cathode

Übergeordnetes Werk:	In: Condensed Matter - MDPI AG, 2017, 8(2023), 1, p 25
Übergeordnetes Werk:	volume:8 ; year:2023 ; number:1, p 25

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/condmat8010025

Katalog-ID:	DOAJ087398184

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spelling	10.3390/condmat8010025 doi (DE-627)DOAJ087398184 (DE-599)DOAJf49cfb12f8da4e458b114f3569d760e7 DE-627 ger DE-627 rakwb eng QC1-999 Guannan Qian verfasserin aut Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential. free-electron laser battery layered cathode Physics Xiaobiao Huang verfasserin aut Jun-Sik Lee verfasserin aut Piero Pianetta verfasserin aut Yijin Liu verfasserin aut In Condensed Matter MDPI AG, 2017 8(2023), 1, p 25 (DE-627)873952502 (DE-600)2877004-3 24103896 nnns volume:8 year:2023 number:1, p 25 https://doi.org/10.3390/condmat8010025 kostenfrei https://doaj.org/article/f49cfb12f8da4e458b114f3569d760e7 kostenfrei https://www.mdpi.com/2410-3896/8/1/25 kostenfrei https://doaj.org/toc/2410-3896 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2023 1, p 25
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allfieldsGer	10.3390/condmat8010025 doi (DE-627)DOAJ087398184 (DE-599)DOAJf49cfb12f8da4e458b114f3569d760e7 DE-627 ger DE-627 rakwb eng QC1-999 Guannan Qian verfasserin aut Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential. free-electron laser battery layered cathode Physics Xiaobiao Huang verfasserin aut Jun-Sik Lee verfasserin aut Piero Pianetta verfasserin aut Yijin Liu verfasserin aut In Condensed Matter MDPI AG, 2017 8(2023), 1, p 25 (DE-627)873952502 (DE-600)2877004-3 24103896 nnns volume:8 year:2023 number:1, p 25 https://doi.org/10.3390/condmat8010025 kostenfrei https://doaj.org/article/f49cfb12f8da4e458b114f3569d760e7 kostenfrei https://www.mdpi.com/2410-3896/8/1/25 kostenfrei https://doaj.org/toc/2410-3896 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2023 1, p 25
allfieldsSound	10.3390/condmat8010025 doi (DE-627)DOAJ087398184 (DE-599)DOAJf49cfb12f8da4e458b114f3569d760e7 DE-627 ger DE-627 rakwb eng QC1-999 Guannan Qian verfasserin aut Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential. free-electron laser battery layered cathode Physics Xiaobiao Huang verfasserin aut Jun-Sik Lee verfasserin aut Piero Pianetta verfasserin aut Yijin Liu verfasserin aut In Condensed Matter MDPI AG, 2017 8(2023), 1, p 25 (DE-627)873952502 (DE-600)2877004-3 24103896 nnns volume:8 year:2023 number:1, p 25 https://doi.org/10.3390/condmat8010025 kostenfrei https://doaj.org/article/f49cfb12f8da4e458b114f3569d760e7 kostenfrei https://www.mdpi.com/2410-3896/8/1/25 kostenfrei https://doaj.org/toc/2410-3896 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 8 2023 1, p 25
language	English
source	In Condensed Matter 8(2023), 1, p 25 volume:8 year:2023 number:1, p 25
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author	Guannan Qian
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topic_title	QC1-999 Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides free-electron laser battery layered cathode
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title	Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides
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title_sort	exploring the ultrafast charge-transfer and redox dynamics in layered transition metal oxides
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title_auth	Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides
abstract	The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential.
abstractGer	The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential.
abstract_unstemmed	The rapid development and broad deployment of rechargeable batteries have fundamentally transformed modern society by revolutionizing the sectors of consumer electronics, transportation, and grid energy storage. Redox reactions in active battery cathode materials are ubiquitous, complicated, and functionally very important. While a lot of effort has been devoted to investigating redox heterogeneity and its progressive evolution upon prolonged battery cycling, the ultrafast dynamics in these systems are largely unexplored. In this article, we discuss the potential significance of understanding redox dynamics in battery cathodes in the ultrafast time regime. Here, we outline a conceptual experimental design for investigating the ultrafast electron transport in an industry-relevant layered transition metal oxide battery cathode using a plasma-acceleration-based X-ray free-electron laser (FEL) facility. Going beyond the proposed experiment, we provide our perspectives on the use of compact FEL sources for applied research, which, in our view, is an area of tremendous potential.
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title_short	Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides
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score	7.401119

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Exploring the Ultrafast Charge-Transfer and Redox Dynamics in Layered Transition Metal Oxides

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Vorhandene Bände

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