PAHs, hydrocarbons, and dimethylsulfides in Asteroid Ryugu samples A0106 and C0107 and the Orgueil (CI1) meteorite
Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the or...
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E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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In: Earth, Planets and Space - SpringerOpen, 2015, 75(2023), 1, Seite 14 |
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| Übergeordnetes Werk: |
volume:75 ; year:2023 ; number:1 ; pages:14 |
| Links: |
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| DOI / URN: |
10.1186/s40623-022-01758-4 |
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| 520 | |a Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract | ||
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10.1186/s40623-022-01758-4 doi (DE-627)DOAJ08776542X (DE-599)DOAJb0a3be3c34224fdc820bb6258c97a711 DE-627 ger DE-627 rakwb eng QB275-343 QE1-996.5 José C. Aponte verfasserin aut PAHs, hydrocarbons, and dimethylsulfides in Asteroid Ryugu samples A0106 and C0107 and the Orgueil (CI1) meteorite 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract Hayabusa2 Ryugu PAHs Aqueous alteration Soluble organics GC×GC Geography. Anthropology. Recreation G Geodesy Geology Jason P. Dworkin verfasserin aut Daniel P. Glavin verfasserin aut Jamie E. Elsila verfasserin aut Eric T. Parker verfasserin aut Hannah L. McLain verfasserin aut Hiroshi Naraoka verfasserin aut Ryuji Okazaki verfasserin aut Yoshinori Takano verfasserin aut Shogo Tachibana verfasserin aut Guannan Dong verfasserin aut Sarah S. Zeichner verfasserin aut John M. Eiler verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Hikaru Yabuta verfasserin aut Fuyuto Terui verfasserin aut Takaaki Noguchi verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Satoru Nakazawa verfasserin aut Yuichi Tsuda verfasserin aut Sei-ichiro Watanabe verfasserin aut The Hayabusa2-initial-analysis SOM team verfasserin aut The Hayabusa2-initial-analysis core team verfasserin aut In Earth, Planets and Space SpringerOpen, 2015 75(2023), 1, Seite 14 (DE-627)353898597 (DE-600)2087663-4 18805981 nnns volume:75 year:2023 number:1 pages:14 https://doi.org/10.1186/s40623-022-01758-4 kostenfrei https://doaj.org/article/b0a3be3c34224fdc820bb6258c97a711 kostenfrei https://doi.org/10.1186/s40623-022-01758-4 kostenfrei https://doaj.org/toc/1880-5981 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 75 2023 1 14 |
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10.1186/s40623-022-01758-4 doi (DE-627)DOAJ08776542X (DE-599)DOAJb0a3be3c34224fdc820bb6258c97a711 DE-627 ger DE-627 rakwb eng QB275-343 QE1-996.5 José C. Aponte verfasserin aut PAHs, hydrocarbons, and dimethylsulfides in Asteroid Ryugu samples A0106 and C0107 and the Orgueil (CI1) meteorite 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract Hayabusa2 Ryugu PAHs Aqueous alteration Soluble organics GC×GC Geography. Anthropology. Recreation G Geodesy Geology Jason P. Dworkin verfasserin aut Daniel P. Glavin verfasserin aut Jamie E. Elsila verfasserin aut Eric T. Parker verfasserin aut Hannah L. McLain verfasserin aut Hiroshi Naraoka verfasserin aut Ryuji Okazaki verfasserin aut Yoshinori Takano verfasserin aut Shogo Tachibana verfasserin aut Guannan Dong verfasserin aut Sarah S. Zeichner verfasserin aut John M. Eiler verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Hikaru Yabuta verfasserin aut Fuyuto Terui verfasserin aut Takaaki Noguchi verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Satoru Nakazawa verfasserin aut Yuichi Tsuda verfasserin aut Sei-ichiro Watanabe verfasserin aut The Hayabusa2-initial-analysis SOM team verfasserin aut The Hayabusa2-initial-analysis core team verfasserin aut In Earth, Planets and Space SpringerOpen, 2015 75(2023), 1, Seite 14 (DE-627)353898597 (DE-600)2087663-4 18805981 nnns volume:75 year:2023 number:1 pages:14 https://doi.org/10.1186/s40623-022-01758-4 kostenfrei https://doaj.org/article/b0a3be3c34224fdc820bb6258c97a711 kostenfrei https://doi.org/10.1186/s40623-022-01758-4 kostenfrei https://doaj.org/toc/1880-5981 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 75 2023 1 14 |
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José C. Aponte @@aut@@ Jason P. Dworkin @@aut@@ Daniel P. Glavin @@aut@@ Jamie E. Elsila @@aut@@ Eric T. Parker @@aut@@ Hannah L. McLain @@aut@@ Hiroshi Naraoka @@aut@@ Ryuji Okazaki @@aut@@ Yoshinori Takano @@aut@@ Shogo Tachibana @@aut@@ Guannan Dong @@aut@@ Sarah S. Zeichner @@aut@@ John M. Eiler @@aut@@ Hisayoshi Yurimoto @@aut@@ Tomoki Nakamura @@aut@@ Hikaru Yabuta @@aut@@ Fuyuto Terui @@aut@@ Takaaki Noguchi @@aut@@ Kanako Sakamoto @@aut@@ Toru Yada @@aut@@ Masahiro Nishimura @@aut@@ Aiko Nakato @@aut@@ Akiko Miyazaki @@aut@@ Kasumi Yogata @@aut@@ Masanao Abe @@aut@@ Tatsuaki Okada @@aut@@ Tomohiro Usui @@aut@@ Makoto Yoshikawa @@aut@@ Takanao Saiki @@aut@@ Satoshi Tanaka @@aut@@ Satoru Nakazawa @@aut@@ Yuichi Tsuda @@aut@@ Sei-ichiro Watanabe @@aut@@ The Hayabusa2-initial-analysis SOM team @@aut@@ The Hayabusa2-initial-analysis core team @@aut@@ |
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José C. Aponte Jason P. Dworkin Daniel P. Glavin Jamie E. Elsila Eric T. Parker Hannah L. McLain Hiroshi Naraoka Ryuji Okazaki Yoshinori Takano Shogo Tachibana Guannan Dong Sarah S. Zeichner John M. Eiler Hisayoshi Yurimoto Tomoki Nakamura Hikaru Yabuta Fuyuto Terui Takaaki Noguchi Kanako Sakamoto Toru Yada Masahiro Nishimura Aiko Nakato Akiko Miyazaki Kasumi Yogata Masanao Abe Tatsuaki Okada Tomohiro Usui Makoto Yoshikawa Takanao Saiki Satoshi Tanaka Satoru Nakazawa Yuichi Tsuda Sei-ichiro Watanabe The Hayabusa2-initial-analysis SOM team The Hayabusa2-initial-analysis core team |
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pahs, hydrocarbons, and dimethylsulfides in asteroid ryugu samples a0106 and c0107 and the orgueil (ci1) meteorite |
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PAHs, hydrocarbons, and dimethylsulfides in Asteroid Ryugu samples A0106 and C0107 and the Orgueil (CI1) meteorite |
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Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract |
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Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract |
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Abstract Evaluating the molecular distribution of organic compounds in pristine extraterrestrial materials is cornerstone to understanding the abiotic synthesis of organics and allows us to better understand the molecular diversity available during the formation of our solar system and before the origins of life on Earth. In this work, we identify multiple organic compounds in solvent extracts of asteroid Ryugu samples A0106 and C0107 and the Orgueil meteorite using two-dimensional gas chromatography and time-of-flight high resolution mass spectrometry (GC×GC–HRMS). Our analyses found similarities between the molecular distribution of organic compounds in Ryugu and the CI carbonaceous chondrite Orgueil. Specifically, several PAHs and organosulfides were found in Ryugu and Orgueil suggesting an interstellar and parent body origin for these compounds. We also evaluated the common relationship between Ryugu, Orgueil, and comets, such as Wild-2; however, until comprehensive compound-specific isotopic analyses for these organic species are undertaken, and until the effects of parent body processes and Earth’s weathering processes on meteoritic organics are better understood, their parent–daughter relationships will remain unanswered. Finally, the study of organic compounds in Ryugu samples and the curation practices for the future preservation of these unvaluable materials are also of special interest for future sample return missions, including NASA’s OSIRIS-REx asteroid sample return mission. Graphical Abstract |
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