Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting

Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low...
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Autor*in:	Bing Wang [verfasserIn] Weigui Liu [verfasserIn] Yecheng Leng [verfasserIn] Xiwen Yu [verfasserIn] Cheng Wang [verfasserIn] Lianghe Hu [verfasserIn] Xi Zhu [verfasserIn] Congping Wu [verfasserIn] Yingfang Yao [verfasserIn] Zhigang Zou [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis

Übergeordnetes Werk:	In: iScience - Elsevier, 2019, 26(2023), 4, Seite 106326-
Übergeordnetes Werk:	volume:26 ; year:2023 ; number:4 ; pages:106326-

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.isci.2023.106326

Katalog-ID:	DOAJ088549445

Internformat


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520			\|a Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting.
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allfields	10.1016/j.isci.2023.106326 doi (DE-627)DOAJ088549445 (DE-599)DOAJ793a9c4c86264f7daad588e5bd948409 DE-627 ger DE-627 rakwb eng Bing Wang verfasserin aut Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting. Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q Weigui Liu verfasserin aut Yecheng Leng verfasserin aut Xiwen Yu verfasserin aut Cheng Wang verfasserin aut Lianghe Hu verfasserin aut Xi Zhu verfasserin aut Congping Wu verfasserin aut Yingfang Yao verfasserin aut Zhigang Zou verfasserin aut In iScience Elsevier, 2019 26(2023), 4, Seite 106326- (DE-627)1019532106 25890042 nnns volume:26 year:2023 number:4 pages:106326- https://doi.org/10.1016/j.isci.2023.106326 kostenfrei https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004223004030 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 26 2023 4 106326-
spelling	10.1016/j.isci.2023.106326 doi (DE-627)DOAJ088549445 (DE-599)DOAJ793a9c4c86264f7daad588e5bd948409 DE-627 ger DE-627 rakwb eng Bing Wang verfasserin aut Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting. Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q Weigui Liu verfasserin aut Yecheng Leng verfasserin aut Xiwen Yu verfasserin aut Cheng Wang verfasserin aut Lianghe Hu verfasserin aut Xi Zhu verfasserin aut Congping Wu verfasserin aut Yingfang Yao verfasserin aut Zhigang Zou verfasserin aut In iScience Elsevier, 2019 26(2023), 4, Seite 106326- (DE-627)1019532106 25890042 nnns volume:26 year:2023 number:4 pages:106326- https://doi.org/10.1016/j.isci.2023.106326 kostenfrei https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004223004030 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 26 2023 4 106326-
allfields_unstemmed	10.1016/j.isci.2023.106326 doi (DE-627)DOAJ088549445 (DE-599)DOAJ793a9c4c86264f7daad588e5bd948409 DE-627 ger DE-627 rakwb eng Bing Wang verfasserin aut Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting. Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q Weigui Liu verfasserin aut Yecheng Leng verfasserin aut Xiwen Yu verfasserin aut Cheng Wang verfasserin aut Lianghe Hu verfasserin aut Xi Zhu verfasserin aut Congping Wu verfasserin aut Yingfang Yao verfasserin aut Zhigang Zou verfasserin aut In iScience Elsevier, 2019 26(2023), 4, Seite 106326- (DE-627)1019532106 25890042 nnns volume:26 year:2023 number:4 pages:106326- https://doi.org/10.1016/j.isci.2023.106326 kostenfrei https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004223004030 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 26 2023 4 106326-
allfieldsGer	10.1016/j.isci.2023.106326 doi (DE-627)DOAJ088549445 (DE-599)DOAJ793a9c4c86264f7daad588e5bd948409 DE-627 ger DE-627 rakwb eng Bing Wang verfasserin aut Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting. Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q Weigui Liu verfasserin aut Yecheng Leng verfasserin aut Xiwen Yu verfasserin aut Cheng Wang verfasserin aut Lianghe Hu verfasserin aut Xi Zhu verfasserin aut Congping Wu verfasserin aut Yingfang Yao verfasserin aut Zhigang Zou verfasserin aut In iScience Elsevier, 2019 26(2023), 4, Seite 106326- (DE-627)1019532106 25890042 nnns volume:26 year:2023 number:4 pages:106326- https://doi.org/10.1016/j.isci.2023.106326 kostenfrei https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004223004030 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 26 2023 4 106326-
allfieldsSound	10.1016/j.isci.2023.106326 doi (DE-627)DOAJ088549445 (DE-599)DOAJ793a9c4c86264f7daad588e5bd948409 DE-627 ger DE-627 rakwb eng Bing Wang verfasserin aut Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting. Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q Weigui Liu verfasserin aut Yecheng Leng verfasserin aut Xiwen Yu verfasserin aut Cheng Wang verfasserin aut Lianghe Hu verfasserin aut Xi Zhu verfasserin aut Congping Wu verfasserin aut Yingfang Yao verfasserin aut Zhigang Zou verfasserin aut In iScience Elsevier, 2019 26(2023), 4, Seite 106326- (DE-627)1019532106 25890042 nnns volume:26 year:2023 number:4 pages:106326- https://doi.org/10.1016/j.isci.2023.106326 kostenfrei https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 kostenfrei http://www.sciencedirect.com/science/article/pii/S2589004223004030 kostenfrei https://doaj.org/toc/2589-0042 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 26 2023 4 106326-
language	English
source	In iScience 26(2023), 4, Seite 106326- volume:26 year:2023 number:4 pages:106326-
sourceStr	In iScience 26(2023), 4, Seite 106326- volume:26 year:2023 number:4 pages:106326-
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis Science Q
isfreeaccess_bool	true
container_title	iScience
authorswithroles_txt_mv	Bing Wang @@aut@@ Weigui Liu @@aut@@ Yecheng Leng @@aut@@ Xiwen Yu @@aut@@ Cheng Wang @@aut@@ Lianghe Hu @@aut@@ Xi Zhu @@aut@@ Congping Wu @@aut@@ Yingfang Yao @@aut@@ Zhigang Zou @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	1019532106
id	DOAJ088549445
language_de	englisch
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author	Bing Wang
spellingShingle	Bing Wang misc Catalysis misc Electrochemistry misc Materials science misc Materials chemistry misc Materials synthesis misc Science misc Q Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
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topic_title	Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting Catalysis Electrochemistry Materials science Materials chemistry Materials synthesis
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title	Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
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title_full	Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
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author_browse	Bing Wang Weigui Liu Yecheng Leng Xiwen Yu Cheng Wang Lianghe Hu Xi Zhu Congping Wu Yingfang Yao Zhigang Zou
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title_sort	strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
title_auth	Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
abstract	Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting.
abstractGer	Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting.
abstract_unstemmed	Summary: Developing active and cost-effective bifunctional electrocatalysts for overall water splitting is challenging but mandatory for renewable energy technologies. We report a high-entropy alloy (HEA) of PtIrCuNiCr as a bifunctional electrocatalyst for overall water splitting, which shows a low overpotential of ca. 190 mV at the current density of 10 mA cm−2. Compared with pure metals, HEAs exhibit remarkable surface strain due to severe lattice distortion in their crystal structures. Theoretical calculations reveal that the strain can regulate the binding energy of intermediates on catalysts by adjusting the metal-metal bonding energy. It pushes the HEA toward the top of volcano plots to achieve superior electrocatalytic activity for both hydrogen and oxygen evolution reactions. The strain effect of HEAs on electrocatalysis can be well engineered by tuning the catalyst radius or configurational entropy. This work renders a systematic strain regulation strategy for designing a high-performance HEA catalyst for overall water splitting.
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title_short	Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting
url	https://doi.org/10.1016/j.isci.2023.106326 https://doaj.org/article/793a9c4c86264f7daad588e5bd948409 http://www.sciencedirect.com/science/article/pii/S2589004223004030 https://doaj.org/toc/2589-0042
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Strain engineering of high-entropy alloy catalysts for electrocatalytic water splitting

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