New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy

Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by ther...
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Autor*in:	Baokang Ren [verfasserIn] Zijing Li [verfasserIn] Yanhui Zhang [verfasserIn] Shidong Feng [verfasserIn] Li‐Min Wang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	glass‐forming ability isomer melting entropy melting point

Übergeordnetes Werk:	In: Advanced Science - Wiley, 2015, 10(2023), 11, Seite n/a-n/a
Übergeordnetes Werk:	volume:10 ; year:2023 ; number:11 ; pages:n/a-n/a

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1002/advs.202206389

Katalog-ID:	DOAJ089278607

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245	1	0	\|a New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
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520			\|a Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances.
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allfields	10.1002/advs.202206389 doi (DE-627)DOAJ089278607 (DE-599)DOAJe90ef2f3653c4a748e5507487cd4f0f6 DE-627 ger DE-627 rakwb eng Baokang Ren verfasserin aut New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances. glass‐forming ability isomer melting entropy melting point Science Q Zijing Li verfasserin aut Yanhui Zhang verfasserin aut Shidong Feng verfasserin aut Li‐Min Wang verfasserin aut In Advanced Science Wiley, 2015 10(2023), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:10 year:2023 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 kostenfrei https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 10 2023 11 n/a-n/a
spelling	10.1002/advs.202206389 doi (DE-627)DOAJ089278607 (DE-599)DOAJe90ef2f3653c4a748e5507487cd4f0f6 DE-627 ger DE-627 rakwb eng Baokang Ren verfasserin aut New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances. glass‐forming ability isomer melting entropy melting point Science Q Zijing Li verfasserin aut Yanhui Zhang verfasserin aut Shidong Feng verfasserin aut Li‐Min Wang verfasserin aut In Advanced Science Wiley, 2015 10(2023), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:10 year:2023 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 kostenfrei https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 10 2023 11 n/a-n/a
allfields_unstemmed	10.1002/advs.202206389 doi (DE-627)DOAJ089278607 (DE-599)DOAJe90ef2f3653c4a748e5507487cd4f0f6 DE-627 ger DE-627 rakwb eng Baokang Ren verfasserin aut New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances. glass‐forming ability isomer melting entropy melting point Science Q Zijing Li verfasserin aut Yanhui Zhang verfasserin aut Shidong Feng verfasserin aut Li‐Min Wang verfasserin aut In Advanced Science Wiley, 2015 10(2023), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:10 year:2023 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 kostenfrei https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 10 2023 11 n/a-n/a
allfieldsGer	10.1002/advs.202206389 doi (DE-627)DOAJ089278607 (DE-599)DOAJe90ef2f3653c4a748e5507487cd4f0f6 DE-627 ger DE-627 rakwb eng Baokang Ren verfasserin aut New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances. glass‐forming ability isomer melting entropy melting point Science Q Zijing Li verfasserin aut Yanhui Zhang verfasserin aut Shidong Feng verfasserin aut Li‐Min Wang verfasserin aut In Advanced Science Wiley, 2015 10(2023), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:10 year:2023 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 kostenfrei https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 10 2023 11 n/a-n/a
allfieldsSound	10.1002/advs.202206389 doi (DE-627)DOAJ089278607 (DE-599)DOAJe90ef2f3653c4a748e5507487cd4f0f6 DE-627 ger DE-627 rakwb eng Baokang Ren verfasserin aut New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances. glass‐forming ability isomer melting entropy melting point Science Q Zijing Li verfasserin aut Yanhui Zhang verfasserin aut Shidong Feng verfasserin aut Li‐Min Wang verfasserin aut In Advanced Science Wiley, 2015 10(2023), 11, Seite n/a-n/a (DE-627)817357777 (DE-600)2808093-2 21983844 nnns volume:10 year:2023 number:11 pages:n/a-n/a https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 kostenfrei https://doi.org/10.1002/advs.202206389 kostenfrei https://doaj.org/toc/2198-3844 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 10 2023 11 n/a-n/a
language	English
source	In Advanced Science 10(2023), 11, Seite n/a-n/a volume:10 year:2023 number:11 pages:n/a-n/a
sourceStr	In Advanced Science 10(2023), 11, Seite n/a-n/a volume:10 year:2023 number:11 pages:n/a-n/a
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	glass‐forming ability isomer melting entropy melting point Science Q
isfreeaccess_bool	true
container_title	Advanced Science
authorswithroles_txt_mv	Baokang Ren @@aut@@ Zijing Li @@aut@@ Yanhui Zhang @@aut@@ Shidong Feng @@aut@@ Li‐Min Wang @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	817357777
id	DOAJ089278607
language_de	englisch
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author	Baokang Ren
spellingShingle	Baokang Ren misc glass‐forming ability misc isomer misc melting entropy misc melting point misc Science misc Q New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
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topic_title	New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy glass‐forming ability isomer melting entropy melting point
topic	misc glass‐forming ability misc isomer misc melting entropy misc melting point misc Science misc Q
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title	New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
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title_full	New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
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title_sort	new interpretation of glass formation in isomeric substances: shifting from melting‐point to melting‐entropy
title_auth	New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
abstract	Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances.
abstractGer	Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances.
abstract_unstemmed	Abstract Revealing the critical thermodynamic parameters determining the glass formation of substances is of great significance for understanding the glass transition and guiding the composition design of glass‐forming materials. Nevertheless, the direct access to glass‐forming ability (GFA) by thermodynamics for various substances remains to be substantiated. The strategy to seek the fundamental properties of glass formation is explored several decades ago, as pioneered by Angell, arguing that the GFA in isomeric xylenes depends on the low lattice energy manifested by the low melting point. Here, an in‐depth study is advanced using two more isomeric systems. Surprisingly, the results do not constantly support the reported relationship between the melting point and glass formation among isomeric molecules. Instead, molecules with enhanced glass formability are featured by the properties of low melting entropy without exception. Comprehensive studies of isomeric molecules find that the low melting entropy is roughly accompanied by the low melting point, explaining the apparent link between melting point and glass formation. Progressively, the viscosity measurements of the isomers uncover a strong dependence of the melting viscosity on melting entropy. These results emphasize the significance of the melting entropy in governing the glass formability of substances.
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title_short	New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy
url	https://doi.org/10.1002/advs.202206389 https://doaj.org/article/e90ef2f3653c4a748e5507487cd4f0f6 https://doaj.org/toc/2198-3844
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New Interpretation of Glass Formation in Isomeric Substances: Shifting from Melting‐Point to Melting‐Entropy

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