Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu
Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fr...
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| Autor*in: |
Toshihiro Yoshimura [verfasserIn] Yoshinori Takano [verfasserIn] Hiroshi Naraoka [verfasserIn] Toshiki Koga [verfasserIn] Daisuke Araoka [verfasserIn] Nanako O. Ogawa [verfasserIn] Philippe Schmitt-Kopplin [verfasserIn] Norbert Hertkorn [verfasserIn] Yasuhiro Oba [verfasserIn] Jason P. Dworkin [verfasserIn] José C. Aponte [verfasserIn] Takaaki Yoshikawa [verfasserIn] Satoru Tanaka [verfasserIn] Naohiko Ohkouchi [verfasserIn] Minako Hashiguchi [verfasserIn] Hannah McLain [verfasserIn] Eric T. Parker [verfasserIn] Saburo Sakai [verfasserIn] Mihoko Yamaguchi [verfasserIn] Takahiro Suzuki [verfasserIn] Tetsuya Yokoyama [verfasserIn] Hisayoshi Yurimoto [verfasserIn] Tomoki Nakamura [verfasserIn] Takaaki Noguchi [verfasserIn] Ryuji Okazaki [verfasserIn] Hikaru Yabuta [verfasserIn] Kanako Sakamoto [verfasserIn] Toru Yada [verfasserIn] Masahiro Nishimura [verfasserIn] Aiko Nakato [verfasserIn] Akiko Miyazaki [verfasserIn] Kasumi Yogata [verfasserIn] Masanao Abe [verfasserIn] Tatsuaki Okada [verfasserIn] Tomohiro Usui [verfasserIn] Makoto Yoshikawa [verfasserIn] Takanao Saiki [verfasserIn] Satoshi Tanaka [verfasserIn] Fuyuto Terui [verfasserIn] Satoru Nakazawa [verfasserIn] Sei-ichiro Watanabe [verfasserIn] Yuichi Tsuda [verfasserIn] Shogo Tachibana [verfasserIn] Hayabusa2-initial-analysis SOM team [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Übergeordnetes Werk: |
In: Nature Communications - Nature Portfolio, 2016, 14(2023), 1, Seite 11 |
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| Übergeordnetes Werk: |
volume:14 ; year:2023 ; number:1 ; pages:11 |
| Links: |
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| DOI / URN: |
10.1038/s41467-023-40871-0 |
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| Katalog-ID: |
DOAJ091754003 |
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| 520 | |a Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. | ||
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10.1038/s41467-023-40871-0 doi (DE-627)DOAJ091754003 (DE-599)DOAJa8365f2b1660426c828fe3e327fedd7e DE-627 ger DE-627 rakwb eng Toshihiro Yoshimura verfasserin aut Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. Science Q Yoshinori Takano verfasserin aut Hiroshi Naraoka verfasserin aut Toshiki Koga verfasserin aut Daisuke Araoka verfasserin aut Nanako O. Ogawa verfasserin aut Philippe Schmitt-Kopplin verfasserin aut Norbert Hertkorn verfasserin aut Yasuhiro Oba verfasserin aut Jason P. Dworkin verfasserin aut José C. Aponte verfasserin aut Takaaki Yoshikawa verfasserin aut Satoru Tanaka verfasserin aut Naohiko Ohkouchi verfasserin aut Minako Hashiguchi verfasserin aut Hannah McLain verfasserin aut Eric T. Parker verfasserin aut Saburo Sakai verfasserin aut Mihoko Yamaguchi verfasserin aut Takahiro Suzuki verfasserin aut Tetsuya Yokoyama verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Takaaki Noguchi verfasserin aut Ryuji Okazaki verfasserin aut Hikaru Yabuta verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Fuyuto Terui verfasserin aut Satoru Nakazawa verfasserin aut Sei-ichiro Watanabe verfasserin aut Yuichi Tsuda verfasserin aut Shogo Tachibana verfasserin aut Hayabusa2-initial-analysis SOM team verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 11 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:11 https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/article/a8365f2b1660426c828fe3e327fedd7e kostenfrei https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 11 |
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10.1038/s41467-023-40871-0 doi (DE-627)DOAJ091754003 (DE-599)DOAJa8365f2b1660426c828fe3e327fedd7e DE-627 ger DE-627 rakwb eng Toshihiro Yoshimura verfasserin aut Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. Science Q Yoshinori Takano verfasserin aut Hiroshi Naraoka verfasserin aut Toshiki Koga verfasserin aut Daisuke Araoka verfasserin aut Nanako O. Ogawa verfasserin aut Philippe Schmitt-Kopplin verfasserin aut Norbert Hertkorn verfasserin aut Yasuhiro Oba verfasserin aut Jason P. Dworkin verfasserin aut José C. Aponte verfasserin aut Takaaki Yoshikawa verfasserin aut Satoru Tanaka verfasserin aut Naohiko Ohkouchi verfasserin aut Minako Hashiguchi verfasserin aut Hannah McLain verfasserin aut Eric T. Parker verfasserin aut Saburo Sakai verfasserin aut Mihoko Yamaguchi verfasserin aut Takahiro Suzuki verfasserin aut Tetsuya Yokoyama verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Takaaki Noguchi verfasserin aut Ryuji Okazaki verfasserin aut Hikaru Yabuta verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Fuyuto Terui verfasserin aut Satoru Nakazawa verfasserin aut Sei-ichiro Watanabe verfasserin aut Yuichi Tsuda verfasserin aut Shogo Tachibana verfasserin aut Hayabusa2-initial-analysis SOM team verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 11 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:11 https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/article/a8365f2b1660426c828fe3e327fedd7e kostenfrei https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 11 |
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10.1038/s41467-023-40871-0 doi (DE-627)DOAJ091754003 (DE-599)DOAJa8365f2b1660426c828fe3e327fedd7e DE-627 ger DE-627 rakwb eng Toshihiro Yoshimura verfasserin aut Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. Science Q Yoshinori Takano verfasserin aut Hiroshi Naraoka verfasserin aut Toshiki Koga verfasserin aut Daisuke Araoka verfasserin aut Nanako O. Ogawa verfasserin aut Philippe Schmitt-Kopplin verfasserin aut Norbert Hertkorn verfasserin aut Yasuhiro Oba verfasserin aut Jason P. Dworkin verfasserin aut José C. Aponte verfasserin aut Takaaki Yoshikawa verfasserin aut Satoru Tanaka verfasserin aut Naohiko Ohkouchi verfasserin aut Minako Hashiguchi verfasserin aut Hannah McLain verfasserin aut Eric T. Parker verfasserin aut Saburo Sakai verfasserin aut Mihoko Yamaguchi verfasserin aut Takahiro Suzuki verfasserin aut Tetsuya Yokoyama verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Takaaki Noguchi verfasserin aut Ryuji Okazaki verfasserin aut Hikaru Yabuta verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Fuyuto Terui verfasserin aut Satoru Nakazawa verfasserin aut Sei-ichiro Watanabe verfasserin aut Yuichi Tsuda verfasserin aut Shogo Tachibana verfasserin aut Hayabusa2-initial-analysis SOM team verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 11 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:11 https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/article/a8365f2b1660426c828fe3e327fedd7e kostenfrei https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 11 |
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10.1038/s41467-023-40871-0 doi (DE-627)DOAJ091754003 (DE-599)DOAJa8365f2b1660426c828fe3e327fedd7e DE-627 ger DE-627 rakwb eng Toshihiro Yoshimura verfasserin aut Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. Science Q Yoshinori Takano verfasserin aut Hiroshi Naraoka verfasserin aut Toshiki Koga verfasserin aut Daisuke Araoka verfasserin aut Nanako O. Ogawa verfasserin aut Philippe Schmitt-Kopplin verfasserin aut Norbert Hertkorn verfasserin aut Yasuhiro Oba verfasserin aut Jason P. Dworkin verfasserin aut José C. Aponte verfasserin aut Takaaki Yoshikawa verfasserin aut Satoru Tanaka verfasserin aut Naohiko Ohkouchi verfasserin aut Minako Hashiguchi verfasserin aut Hannah McLain verfasserin aut Eric T. Parker verfasserin aut Saburo Sakai verfasserin aut Mihoko Yamaguchi verfasserin aut Takahiro Suzuki verfasserin aut Tetsuya Yokoyama verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Takaaki Noguchi verfasserin aut Ryuji Okazaki verfasserin aut Hikaru Yabuta verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Fuyuto Terui verfasserin aut Satoru Nakazawa verfasserin aut Sei-ichiro Watanabe verfasserin aut Yuichi Tsuda verfasserin aut Shogo Tachibana verfasserin aut Hayabusa2-initial-analysis SOM team verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 11 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:11 https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/article/a8365f2b1660426c828fe3e327fedd7e kostenfrei https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 11 |
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10.1038/s41467-023-40871-0 doi (DE-627)DOAJ091754003 (DE-599)DOAJa8365f2b1660426c828fe3e327fedd7e DE-627 ger DE-627 rakwb eng Toshihiro Yoshimura verfasserin aut Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. Science Q Yoshinori Takano verfasserin aut Hiroshi Naraoka verfasserin aut Toshiki Koga verfasserin aut Daisuke Araoka verfasserin aut Nanako O. Ogawa verfasserin aut Philippe Schmitt-Kopplin verfasserin aut Norbert Hertkorn verfasserin aut Yasuhiro Oba verfasserin aut Jason P. Dworkin verfasserin aut José C. Aponte verfasserin aut Takaaki Yoshikawa verfasserin aut Satoru Tanaka verfasserin aut Naohiko Ohkouchi verfasserin aut Minako Hashiguchi verfasserin aut Hannah McLain verfasserin aut Eric T. Parker verfasserin aut Saburo Sakai verfasserin aut Mihoko Yamaguchi verfasserin aut Takahiro Suzuki verfasserin aut Tetsuya Yokoyama verfasserin aut Hisayoshi Yurimoto verfasserin aut Tomoki Nakamura verfasserin aut Takaaki Noguchi verfasserin aut Ryuji Okazaki verfasserin aut Hikaru Yabuta verfasserin aut Kanako Sakamoto verfasserin aut Toru Yada verfasserin aut Masahiro Nishimura verfasserin aut Aiko Nakato verfasserin aut Akiko Miyazaki verfasserin aut Kasumi Yogata verfasserin aut Masanao Abe verfasserin aut Tatsuaki Okada verfasserin aut Tomohiro Usui verfasserin aut Makoto Yoshikawa verfasserin aut Takanao Saiki verfasserin aut Satoshi Tanaka verfasserin aut Fuyuto Terui verfasserin aut Satoru Nakazawa verfasserin aut Sei-ichiro Watanabe verfasserin aut Yuichi Tsuda verfasserin aut Shogo Tachibana verfasserin aut Hayabusa2-initial-analysis SOM team verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 11 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:11 https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/article/a8365f2b1660426c828fe3e327fedd7e kostenfrei https://doi.org/10.1038/s41467-023-40871-0 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 11 |
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Toshihiro Yoshimura @@aut@@ Yoshinori Takano @@aut@@ Hiroshi Naraoka @@aut@@ Toshiki Koga @@aut@@ Daisuke Araoka @@aut@@ Nanako O. Ogawa @@aut@@ Philippe Schmitt-Kopplin @@aut@@ Norbert Hertkorn @@aut@@ Yasuhiro Oba @@aut@@ Jason P. Dworkin @@aut@@ José C. Aponte @@aut@@ Takaaki Yoshikawa @@aut@@ Satoru Tanaka @@aut@@ Naohiko Ohkouchi @@aut@@ Minako Hashiguchi @@aut@@ Hannah McLain @@aut@@ Eric T. Parker @@aut@@ Saburo Sakai @@aut@@ Mihoko Yamaguchi @@aut@@ Takahiro Suzuki @@aut@@ Tetsuya Yokoyama @@aut@@ Hisayoshi Yurimoto @@aut@@ Tomoki Nakamura @@aut@@ Takaaki Noguchi @@aut@@ Ryuji Okazaki @@aut@@ Hikaru Yabuta @@aut@@ Kanako Sakamoto @@aut@@ Toru Yada @@aut@@ Masahiro Nishimura @@aut@@ Aiko Nakato @@aut@@ Akiko Miyazaki @@aut@@ Kasumi Yogata @@aut@@ Masanao Abe @@aut@@ Tatsuaki Okada @@aut@@ Tomohiro Usui @@aut@@ Makoto Yoshikawa @@aut@@ Takanao Saiki @@aut@@ Satoshi Tanaka @@aut@@ Fuyuto Terui @@aut@@ Satoru Nakazawa @@aut@@ Sei-ichiro Watanabe @@aut@@ Yuichi Tsuda @@aut@@ Shogo Tachibana @@aut@@ Hayabusa2-initial-analysis SOM team @@aut@@ |
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Toshihiro Yoshimura Yoshinori Takano Hiroshi Naraoka Toshiki Koga Daisuke Araoka Nanako O. Ogawa Philippe Schmitt-Kopplin Norbert Hertkorn Yasuhiro Oba Jason P. Dworkin José C. Aponte Takaaki Yoshikawa Satoru Tanaka Naohiko Ohkouchi Minako Hashiguchi Hannah McLain Eric T. Parker Saburo Sakai Mihoko Yamaguchi Takahiro Suzuki Tetsuya Yokoyama Hisayoshi Yurimoto Tomoki Nakamura Takaaki Noguchi Ryuji Okazaki Hikaru Yabuta Kanako Sakamoto Toru Yada Masahiro Nishimura Aiko Nakato Akiko Miyazaki Kasumi Yogata Masanao Abe Tatsuaki Okada Tomohiro Usui Makoto Yoshikawa Takanao Saiki Satoshi Tanaka Fuyuto Terui Satoru Nakazawa Sei-ichiro Watanabe Yuichi Tsuda Shogo Tachibana Hayabusa2-initial-analysis SOM team |
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Chemical evolution of primordial salts and organic sulfur molecules in the asteroid 162173 Ryugu |
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Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. |
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Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. |
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Abstract Samples from the carbonaceous asteroid (162173) Ryugu provide information on the chemical evolution of organic molecules in the early solar system. Here we show the element partitioning of the major component ions by sequential extractions of salts, carbonates, and phyllosilicate-bearing fractions to reveal primordial brine composition of the primitive asteroid. Sodium is the dominant electrolyte of the salt fraction extract. Anions and NH4 + are more abundant in the salt fraction than in the carbonate and phyllosilicate fractions, with molar concentrations in the order SO4 2− < Cl− < S2O3 2− < NO3 − < NH4 +. The salt fraction extracts contain anionic soluble sulfur-bearing species such as S n -polythionic acids (n < 6), C n -alkylsulfonates, alkylthiosulfonates, hydroxyalkylsulfonates, and hydroxyalkylthiosulfonates (n < 7). The sulfur-bearing soluble compounds may have driven the molecular evolution of prebiotic organic material transforming simple organic molecules into hydrophilic, amphiphilic, and refractory S allotropes. |
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