State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting

The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal o...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Shankara S. Kalanur [verfasserIn] Jaldappagari Seetharamappa [verfasserIn] Qadeer Akbar Sial [verfasserIn] Bruno G. Pollet [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	photoelectrochemical water splitting CuV Cu Cu Cu Cu

Übergeordnetes Werk:	In: Nanomaterials - MDPI AG, 2012, 13(2023), 2599, p 2599
Übergeordnetes Werk:	volume:13 ; year:2023 ; number:2599, p 2599

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/nano13182599

Katalog-ID:	DOAJ093334206

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allfields	10.3390/nano13182599 doi (DE-627)DOAJ093334206 (DE-599)DOAJ11f253388b2a4fe9a09869990add1911 DE-627 ger DE-627 rakwb eng QD1-999 Shankara S. Kalanur verfasserin aut State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions. photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< Chemistry Jaldappagari Seetharamappa verfasserin aut Qadeer Akbar Sial verfasserin aut Bruno G. Pollet verfasserin aut In Nanomaterials MDPI AG, 2012 13(2023), 2599, p 2599 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:13 year:2023 number:2599, p 2599 https://doi.org/10.3390/nano13182599 kostenfrei https://doaj.org/article/11f253388b2a4fe9a09869990add1911 kostenfrei https://www.mdpi.com/2079-4991/13/18/2599 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2023 2599, p 2599
spelling	10.3390/nano13182599 doi (DE-627)DOAJ093334206 (DE-599)DOAJ11f253388b2a4fe9a09869990add1911 DE-627 ger DE-627 rakwb eng QD1-999 Shankara S. Kalanur verfasserin aut State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions. photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< Chemistry Jaldappagari Seetharamappa verfasserin aut Qadeer Akbar Sial verfasserin aut Bruno G. Pollet verfasserin aut In Nanomaterials MDPI AG, 2012 13(2023), 2599, p 2599 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:13 year:2023 number:2599, p 2599 https://doi.org/10.3390/nano13182599 kostenfrei https://doaj.org/article/11f253388b2a4fe9a09869990add1911 kostenfrei https://www.mdpi.com/2079-4991/13/18/2599 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2023 2599, p 2599
allfields_unstemmed	10.3390/nano13182599 doi (DE-627)DOAJ093334206 (DE-599)DOAJ11f253388b2a4fe9a09869990add1911 DE-627 ger DE-627 rakwb eng QD1-999 Shankara S. Kalanur verfasserin aut State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions. photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< Chemistry Jaldappagari Seetharamappa verfasserin aut Qadeer Akbar Sial verfasserin aut Bruno G. Pollet verfasserin aut In Nanomaterials MDPI AG, 2012 13(2023), 2599, p 2599 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:13 year:2023 number:2599, p 2599 https://doi.org/10.3390/nano13182599 kostenfrei https://doaj.org/article/11f253388b2a4fe9a09869990add1911 kostenfrei https://www.mdpi.com/2079-4991/13/18/2599 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2023 2599, p 2599
allfieldsGer	10.3390/nano13182599 doi (DE-627)DOAJ093334206 (DE-599)DOAJ11f253388b2a4fe9a09869990add1911 DE-627 ger DE-627 rakwb eng QD1-999 Shankara S. Kalanur verfasserin aut State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions. photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< Chemistry Jaldappagari Seetharamappa verfasserin aut Qadeer Akbar Sial verfasserin aut Bruno G. Pollet verfasserin aut In Nanomaterials MDPI AG, 2012 13(2023), 2599, p 2599 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:13 year:2023 number:2599, p 2599 https://doi.org/10.3390/nano13182599 kostenfrei https://doaj.org/article/11f253388b2a4fe9a09869990add1911 kostenfrei https://www.mdpi.com/2079-4991/13/18/2599 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2023 2599, p 2599
allfieldsSound	10.3390/nano13182599 doi (DE-627)DOAJ093334206 (DE-599)DOAJ11f253388b2a4fe9a09869990add1911 DE-627 ger DE-627 rakwb eng QD1-999 Shankara S. Kalanur verfasserin aut State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions. photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< Chemistry Jaldappagari Seetharamappa verfasserin aut Qadeer Akbar Sial verfasserin aut Bruno G. Pollet verfasserin aut In Nanomaterials MDPI AG, 2012 13(2023), 2599, p 2599 (DE-627)718627199 (DE-600)2662255-5 20794991 nnns volume:13 year:2023 number:2599, p 2599 https://doi.org/10.3390/nano13182599 kostenfrei https://doaj.org/article/11f253388b2a4fe9a09869990add1911 kostenfrei https://www.mdpi.com/2079-4991/13/18/2599 kostenfrei https://doaj.org/toc/2079-4991 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2023 2599, p 2599
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callnumber-first	Q - Science
author	Shankara S. Kalanur
spellingShingle	Shankara S. Kalanur misc QD1-999 misc photoelectrochemical water splitting misc CuV<sub<2</sub<O<sub<6</sub< misc Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< misc Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< misc Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< misc Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< misc Chemistry State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting
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topic_title	QD1-999 State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting photoelectrochemical water splitting CuV<sub<2</sub<O<sub<6</sub< Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub<
topic	misc QD1-999 misc photoelectrochemical water splitting misc CuV<sub<2</sub<O<sub<6</sub< misc Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< misc Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< misc Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< misc Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< misc Chemistry
topic_unstemmed	misc QD1-999 misc photoelectrochemical water splitting misc CuV<sub<2</sub<O<sub<6</sub< misc Cu<sub<2</sub<V<sub<2</sub<O<sub<7</sub< misc Cu<sub<3</sub<V<sub<2</sub<O<sub<8</sub< misc Cu<sub<5</sub<V<sub<2</sub<O<sub<10</sub< misc Cu<sub<11</sub<V<sub<6</sub<O<sub<26</sub< misc Chemistry
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title	State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting
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title_full	State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting
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title_sort	state of the art progress in copper vanadate materials for solar water splitting
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title_auth	State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting
abstract	The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions.
abstractGer	The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions.
abstract_unstemmed	The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. Importantly, intense and strategically focused research is vital to overcome the scientific challenges involved in copper vanadates and to explore and exploit new polymorphs to set new efficiency benchmarks and PEC water splitting solutions.
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title_short	State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting
url	https://doi.org/10.3390/nano13182599 https://doaj.org/article/11f253388b2a4fe9a09869990add1911 https://www.mdpi.com/2079-4991/13/18/2599 https://doaj.org/toc/2079-4991
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Kalanur</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The development of a single junction photoelectrode material having specific properties is essential and challenging for the efficient application in solar water splitting for oxygen production and a high value-added product, hydrogen. Moreover, the present material solutions based on binary metal oxides offer limited catalytic activity and hydrogen production efficiency. Therefore, it is paramount to develop and exploit a unique range of materials derived from ternary metal oxides with specifically engineered properties to advance in photoelectrochemical (PEC) water splitting. Among the ternary oxides, copper vanadates offer promising characteristics, such as a narrow bandgap and catalytic surface properties along with favorable band edges for facile oxygen evolution reaction (OER), which is considered the bottleneck step in performing overall water dissociation. Furthermore, the copper vanadates allow the tuning of the stoichiometry through which a wide range of polymorphs and materials could be obtained. This review provides a complete outlook on the range of copper vanadates and the established synthesis approach, morphology, crystal structure, band edge properties, and PEC characterizations. Mainly, the underlying charge dynamic properties, carrier path length, effect of doping, and influence of surface catalysts are discussed. The review concludes that the advancement toward obtaining low-bandgap materials is a main challenge to overcome the limitations for efficient water dissociation to OER and copper vanadates, which offer a promising solution with their unique properties and advantages. 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State of the Art Progress in Copper Vanadate Materials for Solar Water Splitting

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