One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films

To the best of our knowledge, this study reports the first direct electropolymerization of a dicyanobenzene-carbazole dye functionalized with an imidazole group to prepare redox- and photoactive porous organic polymer (POP) films in controlled amounts. The POP films were grown on indium-doped tin ox...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Jinkun Liu [verfasserIn] Octavio Martinez Perez [verfasserIn] Dominic Lavergne [verfasserIn] Loorthuraja Rasu [verfasserIn] Elizabeth Murphy [verfasserIn] Andy Galvez-Rodriguez [verfasserIn] Steven H. Bergens [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	4CzIPN 3CzImIPN photoredox-POP photochemistry polymerization

Übergeordnetes Werk:	In: Polymers - MDPI AG, 2011, 15(2023), 16, p 3340
Übergeordnetes Werk:	volume:15 ; year:2023 ; number:16, p 3340

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/polym15163340

Katalog-ID:	DOAJ093561644

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callnumber-first	Q - Science
author	Jinkun Liu
spellingShingle	Jinkun Liu misc QD241-441 misc 4CzIPN misc 3CzImIPN misc photoredox-POP misc photochemistry misc polymerization misc Organic chemistry One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films
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topic_title	QD241-441 One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films 4CzIPN 3CzImIPN photoredox-POP photochemistry polymerization
topic	misc QD241-441 misc 4CzIPN misc 3CzImIPN misc photoredox-POP misc photochemistry misc polymerization misc Organic chemistry
topic_unstemmed	misc QD241-441 misc 4CzIPN misc 3CzImIPN misc photoredox-POP misc photochemistry misc polymerization misc Organic chemistry
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title	One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films
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title_full	One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films
author_sort	Jinkun Liu
journal	Polymers
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author_browse	Jinkun Liu Octavio Martinez Perez Dominic Lavergne Loorthuraja Rasu Elizabeth Murphy Andy Galvez-Rodriguez Steven H. Bergens
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title_sort	one-step electropolymerization of a dicyanobenzene-carbazole-imidazole dye to prepare photoactive redox polymer films
callnumber	QD241-441
title_auth	One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films
abstract	To the best of our knowledge, this study reports the first direct electropolymerization of a dicyanobenzene-carbazole dye functionalized with an imidazole group to prepare redox- and photoactive porous organic polymer (POP) films in controlled amounts. The POP films were grown on indium-doped tin oxide (ITO) and carbon surfaces using a new monomer, 1-imidazole-2,4,6-tri(carbazol-9-yl)-3,5-dicyanobenzene (<b<1</b<, 3CzImIPN), through a simple one-step process. The structure and activities of the POP films were investigated as photoelectrodes for electrooxidations, as heterogeneous photocatalysts for photosynthetic olefin isomerizations, and for solid-state photoluminescence behavior tunable by lithium-ion concentrations in solution. The results demonstrate that the photoredox-POPs can be used as efficient photocatalysts, and they have potential applications in sensing.
abstractGer	To the best of our knowledge, this study reports the first direct electropolymerization of a dicyanobenzene-carbazole dye functionalized with an imidazole group to prepare redox- and photoactive porous organic polymer (POP) films in controlled amounts. The POP films were grown on indium-doped tin oxide (ITO) and carbon surfaces using a new monomer, 1-imidazole-2,4,6-tri(carbazol-9-yl)-3,5-dicyanobenzene (<b<1</b<, 3CzImIPN), through a simple one-step process. The structure and activities of the POP films were investigated as photoelectrodes for electrooxidations, as heterogeneous photocatalysts for photosynthetic olefin isomerizations, and for solid-state photoluminescence behavior tunable by lithium-ion concentrations in solution. The results demonstrate that the photoredox-POPs can be used as efficient photocatalysts, and they have potential applications in sensing.
abstract_unstemmed	To the best of our knowledge, this study reports the first direct electropolymerization of a dicyanobenzene-carbazole dye functionalized with an imidazole group to prepare redox- and photoactive porous organic polymer (POP) films in controlled amounts. The POP films were grown on indium-doped tin oxide (ITO) and carbon surfaces using a new monomer, 1-imidazole-2,4,6-tri(carbazol-9-yl)-3,5-dicyanobenzene (<b<1</b<, 3CzImIPN), through a simple one-step process. The structure and activities of the POP films were investigated as photoelectrodes for electrooxidations, as heterogeneous photocatalysts for photosynthetic olefin isomerizations, and for solid-state photoluminescence behavior tunable by lithium-ion concentrations in solution. The results demonstrate that the photoredox-POPs can be used as efficient photocatalysts, and they have potential applications in sensing.
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container_issue	16, p 3340
title_short	One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films
url	https://doi.org/10.3390/polym15163340 https://doaj.org/article/d3c8c41d71744f39941ff1c8b5f278c1 https://www.mdpi.com/2073-4360/15/16/3340 https://doaj.org/toc/2073-4360
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author2	Octavio Martinez Perez Dominic Lavergne Loorthuraja Rasu Elizabeth Murphy Andy Galvez-Rodriguez Steven H. Bergens
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doi_str	10.3390/polym15163340
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up_date	2024-07-03T18:03:35.483Z
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One-Step Electropolymerization of a Dicyanobenzene-Carbazole-Imidazole Dye to Prepare Photoactive Redox Polymer Films

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