Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution

Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggrega...
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Autor*in:	Sen Lin [verfasserIn] Shiyong Sun [verfasserIn] Zhengwei Li [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution

Übergeordnetes Werk:	In: Heliyon - Elsevier, 2016, 9(2023), 10, Seite e20520-
Übergeordnetes Werk:	volume:9 ; year:2023 ; number:10 ; pages:e20520-

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1016/j.heliyon.2023.e20520

Katalog-ID:	DOAJ09514367X

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520			\|a Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field.
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allfields	10.1016/j.heliyon.2023.e20520 doi (DE-627)DOAJ09514367X (DE-599)DOAJ92975395daef4a46af3d2251f2802b9d DE-627 ger DE-627 rakwb eng Q1-390 H1-99 Sen Lin verfasserin aut Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field. G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General) Shiyong Sun verfasserin aut Zhengwei Li verfasserin aut In Heliyon Elsevier, 2016 9(2023), 10, Seite e20520- (DE-627)835893197 (DE-600)2835763-2 24058440 nnns volume:9 year:2023 number:10 pages:e20520- https://doi.org/10.1016/j.heliyon.2023.e20520 kostenfrei https://doaj.org/article/92975395daef4a46af3d2251f2802b9d kostenfrei http://www.sciencedirect.com/science/article/pii/S2405844023077289 kostenfrei https://doaj.org/toc/2405-8440 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 9 2023 10 e20520-
spelling	10.1016/j.heliyon.2023.e20520 doi (DE-627)DOAJ09514367X (DE-599)DOAJ92975395daef4a46af3d2251f2802b9d DE-627 ger DE-627 rakwb eng Q1-390 H1-99 Sen Lin verfasserin aut Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field. G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General) Shiyong Sun verfasserin aut Zhengwei Li verfasserin aut In Heliyon Elsevier, 2016 9(2023), 10, Seite e20520- (DE-627)835893197 (DE-600)2835763-2 24058440 nnns volume:9 year:2023 number:10 pages:e20520- https://doi.org/10.1016/j.heliyon.2023.e20520 kostenfrei https://doaj.org/article/92975395daef4a46af3d2251f2802b9d kostenfrei http://www.sciencedirect.com/science/article/pii/S2405844023077289 kostenfrei https://doaj.org/toc/2405-8440 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 9 2023 10 e20520-
allfields_unstemmed	10.1016/j.heliyon.2023.e20520 doi (DE-627)DOAJ09514367X (DE-599)DOAJ92975395daef4a46af3d2251f2802b9d DE-627 ger DE-627 rakwb eng Q1-390 H1-99 Sen Lin verfasserin aut Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field. G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General) Shiyong Sun verfasserin aut Zhengwei Li verfasserin aut In Heliyon Elsevier, 2016 9(2023), 10, Seite e20520- (DE-627)835893197 (DE-600)2835763-2 24058440 nnns volume:9 year:2023 number:10 pages:e20520- https://doi.org/10.1016/j.heliyon.2023.e20520 kostenfrei https://doaj.org/article/92975395daef4a46af3d2251f2802b9d kostenfrei http://www.sciencedirect.com/science/article/pii/S2405844023077289 kostenfrei https://doaj.org/toc/2405-8440 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 9 2023 10 e20520-
allfieldsGer	10.1016/j.heliyon.2023.e20520 doi (DE-627)DOAJ09514367X (DE-599)DOAJ92975395daef4a46af3d2251f2802b9d DE-627 ger DE-627 rakwb eng Q1-390 H1-99 Sen Lin verfasserin aut Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field. G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General) Shiyong Sun verfasserin aut Zhengwei Li verfasserin aut In Heliyon Elsevier, 2016 9(2023), 10, Seite e20520- (DE-627)835893197 (DE-600)2835763-2 24058440 nnns volume:9 year:2023 number:10 pages:e20520- https://doi.org/10.1016/j.heliyon.2023.e20520 kostenfrei https://doaj.org/article/92975395daef4a46af3d2251f2802b9d kostenfrei http://www.sciencedirect.com/science/article/pii/S2405844023077289 kostenfrei https://doaj.org/toc/2405-8440 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 9 2023 10 e20520-
allfieldsSound	10.1016/j.heliyon.2023.e20520 doi (DE-627)DOAJ09514367X (DE-599)DOAJ92975395daef4a46af3d2251f2802b9d DE-627 ger DE-627 rakwb eng Q1-390 H1-99 Sen Lin verfasserin aut Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field. G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General) Shiyong Sun verfasserin aut Zhengwei Li verfasserin aut In Heliyon Elsevier, 2016 9(2023), 10, Seite e20520- (DE-627)835893197 (DE-600)2835763-2 24058440 nnns volume:9 year:2023 number:10 pages:e20520- https://doi.org/10.1016/j.heliyon.2023.e20520 kostenfrei https://doaj.org/article/92975395daef4a46af3d2251f2802b9d kostenfrei http://www.sciencedirect.com/science/article/pii/S2405844023077289 kostenfrei https://doaj.org/toc/2405-8440 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_171 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 9 2023 10 e20520-
language	English
source	In Heliyon 9(2023), 10, Seite e20520- volume:9 year:2023 number:10 pages:e20520-
sourceStr	In Heliyon 9(2023), 10, Seite e20520- volume:9 year:2023 number:10 pages:e20520-
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution Science (General) Social sciences (General)
isfreeaccess_bool	true
container_title	Heliyon
authorswithroles_txt_mv	Sen Lin @@aut@@ Shiyong Sun @@aut@@ Zhengwei Li @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	835893197
id	DOAJ09514367X
language_de	englisch
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author	Sen Lin
spellingShingle	Sen Lin misc Q1-390 misc H1-99 misc G-C3N4 misc Halloysite misc Cell pulverizing misc Electrostatic self-assembly misc H2 evolution misc Science (General) misc Social sciences (General) Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution
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topic_title	Q1-390 H1-99 Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution G-C3N4 Halloysite Cell pulverizing Electrostatic self-assembly H2 evolution
topic	misc Q1-390 misc H1-99 misc G-C3N4 misc Halloysite misc Cell pulverizing misc Electrostatic self-assembly misc H2 evolution misc Science (General) misc Social sciences (General)
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title	Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution
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title_full	Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution
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title_sort	clay-based 1d-2d halloysite&g-c3n4 nanostructured meat floss for photocatalytic hydrogen evolution
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title_auth	Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution
abstract	Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field.
abstractGer	Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field.
abstract_unstemmed	Graphitic carbon nitride (g-C3N4) has drawn extensive attention with some features including visible-light response as non-metallic semiconductor, low cost in raw material and green pollution-free for environment, but suffers from some issues such as fast charge carriers’ recombination, easy aggregation, etc. In this work, the 1D-2D HNTs&g–C3N4–X binary materials similar to meat floss pattern in a series of halloysite loading amounts are designed via a facile electrostatic self-assembly strategy with debris g-C3N4 after cell pulverizing treatment and HNTs that outwardly modified by cetyltrimethylammonium bromide (CTAB) as the building blocks. The halloysite-mediated satellite-core material displays a photocatalytic of H2 evolution performance with the highest evolution rate of 137.0 μmol g−1 h−1 in visible light condition with no co-catalysts, and is ∼3.4 times that of bulk g-C3N4, mainly benefiting from the reduced nanometer size of debris g-C3N4 and enhanced interface dispersion ability by HNTs, resulting in ameliorative separation efficiency of photogenerated charge carriers. This research conclusively provides the new perspective towards the performance enhancement of water splitting of g-C3N4 in raw clay mineral modification mode and broadens the applications of mineral-based composite in the renewable energy utilization field.
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title_short	Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution
url	https://doi.org/10.1016/j.heliyon.2023.e20520 https://doaj.org/article/92975395daef4a46af3d2251f2802b9d http://www.sciencedirect.com/science/article/pii/S2405844023077289 https://doaj.org/toc/2405-8440
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up_date	2024-07-04T02:04:33.203Z
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Clay-based 1D-2D halloysite&g-C3N4 nanostructured meat floss for photocatalytic hydrogen evolution

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