Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries
Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheri...
Ausführliche Beschreibung
Autor*in: |
Xinghua Liang [verfasserIn] Yuying Wang [verfasserIn] Zhida Liang [verfasserIn] Ge Yan [verfasserIn] Lingxiao Lan [verfasserIn] Yujiang Wang [verfasserIn] Xueli Shi [verfasserIn] Shuhong Yun [verfasserIn] Meihong Huang [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Übergeordnetes Werk: |
In: Polymers - MDPI AG, 2011, 16(2023), 1, p 55 |
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Übergeordnetes Werk: |
volume:16 ; year:2023 ; number:1, p 55 |
Links: |
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DOI / URN: |
10.3390/polym16010055 |
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Katalog-ID: |
DOAJ097775339 |
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10.3390/polym16010055 doi (DE-627)DOAJ097775339 (DE-599)DOAJ8acc435fb4204e7297936374ce310228 DE-627 ger DE-627 rakwb eng QD241-441 Xinghua Liang verfasserin aut Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< atmospheric plasma spraying (APS) in situ solid-state batteries ultraviolet curing (UV-curing) Organic chemistry Yuying Wang verfasserin aut Zhida Liang verfasserin aut Ge Yan verfasserin aut Lingxiao Lan verfasserin aut Yujiang Wang verfasserin aut Xueli Shi verfasserin aut Shuhong Yun verfasserin aut Meihong Huang verfasserin aut In Polymers MDPI AG, 2011 16(2023), 1, p 55 (DE-627)61409612X (DE-600)2527146-5 20734360 nnns volume:16 year:2023 number:1, p 55 https://doi.org/10.3390/polym16010055 kostenfrei https://doaj.org/article/8acc435fb4204e7297936374ce310228 kostenfrei https://www.mdpi.com/2073-4360/16/1/55 kostenfrei https://doaj.org/toc/2073-4360 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 16 2023 1, p 55 |
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10.3390/polym16010055 doi (DE-627)DOAJ097775339 (DE-599)DOAJ8acc435fb4204e7297936374ce310228 DE-627 ger DE-627 rakwb eng QD241-441 Xinghua Liang verfasserin aut Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< atmospheric plasma spraying (APS) in situ solid-state batteries ultraviolet curing (UV-curing) Organic chemistry Yuying Wang verfasserin aut Zhida Liang verfasserin aut Ge Yan verfasserin aut Lingxiao Lan verfasserin aut Yujiang Wang verfasserin aut Xueli Shi verfasserin aut Shuhong Yun verfasserin aut Meihong Huang verfasserin aut In Polymers MDPI AG, 2011 16(2023), 1, p 55 (DE-627)61409612X (DE-600)2527146-5 20734360 nnns volume:16 year:2023 number:1, p 55 https://doi.org/10.3390/polym16010055 kostenfrei https://doaj.org/article/8acc435fb4204e7297936374ce310228 kostenfrei https://www.mdpi.com/2073-4360/16/1/55 kostenfrei https://doaj.org/toc/2073-4360 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 16 2023 1, p 55 |
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10.3390/polym16010055 doi (DE-627)DOAJ097775339 (DE-599)DOAJ8acc435fb4204e7297936374ce310228 DE-627 ger DE-627 rakwb eng QD241-441 Xinghua Liang verfasserin aut Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< atmospheric plasma spraying (APS) in situ solid-state batteries ultraviolet curing (UV-curing) Organic chemistry Yuying Wang verfasserin aut Zhida Liang verfasserin aut Ge Yan verfasserin aut Lingxiao Lan verfasserin aut Yujiang Wang verfasserin aut Xueli Shi verfasserin aut Shuhong Yun verfasserin aut Meihong Huang verfasserin aut In Polymers MDPI AG, 2011 16(2023), 1, p 55 (DE-627)61409612X (DE-600)2527146-5 20734360 nnns volume:16 year:2023 number:1, p 55 https://doi.org/10.3390/polym16010055 kostenfrei https://doaj.org/article/8acc435fb4204e7297936374ce310228 kostenfrei https://www.mdpi.com/2073-4360/16/1/55 kostenfrei https://doaj.org/toc/2073-4360 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 16 2023 1, p 55 |
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10.3390/polym16010055 doi (DE-627)DOAJ097775339 (DE-599)DOAJ8acc435fb4204e7297936374ce310228 DE-627 ger DE-627 rakwb eng QD241-441 Xinghua Liang verfasserin aut Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< atmospheric plasma spraying (APS) in situ solid-state batteries ultraviolet curing (UV-curing) Organic chemistry Yuying Wang verfasserin aut Zhida Liang verfasserin aut Ge Yan verfasserin aut Lingxiao Lan verfasserin aut Yujiang Wang verfasserin aut Xueli Shi verfasserin aut Shuhong Yun verfasserin aut Meihong Huang verfasserin aut In Polymers MDPI AG, 2011 16(2023), 1, p 55 (DE-627)61409612X (DE-600)2527146-5 20734360 nnns volume:16 year:2023 number:1, p 55 https://doi.org/10.3390/polym16010055 kostenfrei https://doaj.org/article/8acc435fb4204e7297936374ce310228 kostenfrei https://www.mdpi.com/2073-4360/16/1/55 kostenfrei https://doaj.org/toc/2073-4360 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2119 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 16 2023 1, p 55 |
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Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries |
abstract |
Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. |
abstractGer |
Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. |
abstract_unstemmed |
Lithium-ion solid-state batteries with spinel Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub< (LTO) electrodes have significant advantages, such as stability, long life, and good multiplication performance. In this work, the LTO electrode was obtained by the atmospheric plasma spraying method, and a composite solid electrolyte was prepared by in situ ultraviolet (UV) curing on the LTO electrode. The composite solid electrolyte was designed using a soft–hard combination strategy, and the electrolyte was prepared into a composite of a poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) flexible structure and high-conductivity Li<sub<1.3</sub<Al<sub<0.3</sub<Ti<sub<1.7</sub<(PO<sub<4</sub<)<sub<3</sub< (LATP) hard particles. The composite electrolyte exhibited a good ionic conductivity up to 0.35 mS cm<sup<−1</sup< at 30 °C and an electrochemical window above 4.0 V. In situ and ex situ electrolytes were assembled into LTO//electrolyte//Li solid-state batteries to investigate their impact on the electrochemical performance of the batteries. As a result, the assembled Li<sub<4</sub<Ti<sub<5</sub<O<sub<12</sub<//in situ electrolytes//Li batteries exhibited excellent rate of performance, and their capacity retention rate was 90% at 0.2 mA/cm<sup<2</sup< after 300 cycles. This work provides a new method for the fabrication of novel advanced solid-state electrolytes and electrodes for applications in solid-state batteries. |
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container_issue |
1, p 55 |
title_short |
Long-Cycle Stability of In Situ Ultraviolet Curable Organic/Inorganic Composite Electrolyte for Solid-State Batteries |
url |
https://doi.org/10.3390/polym16010055 https://doaj.org/article/8acc435fb4204e7297936374ce310228 https://www.mdpi.com/2073-4360/16/1/55 https://doaj.org/toc/2073-4360 |
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author2 |
Yuying Wang Zhida Liang Ge Yan Lingxiao Lan Yujiang Wang Xueli Shi Shuhong Yun Meihong Huang |
author2Str |
Yuying Wang Zhida Liang Ge Yan Lingxiao Lan Yujiang Wang Xueli Shi Shuhong Yun Meihong Huang |
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QD - Chemistry |
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doi_str |
10.3390/polym16010055 |
callnumber-a |
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up_date |
2024-07-03T13:42:52.318Z |
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