Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis

Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and io...
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Autor*in:	Hongzheng Dong [verfasserIn] Xiangyu Pan [verfasserIn] Yuancai Gong [verfasserIn] Mengfan Xue [verfasserIn] Pin Wang [verfasserIn] SocMan Ho-Kimura [verfasserIn] Yingfang Yao [verfasserIn] Hao Xin [verfasserIn] Wenjun Luo [verfasserIn] Zhigang Zou [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Übergeordnetes Werk:	In: Nature Communications - Nature Portfolio, 2016, 14(2023), 1, Seite 9
Übergeordnetes Werk:	volume:14 ; year:2023 ; number:1 ; pages:9

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.1038/s41467-023-43916-6

Katalog-ID:	DOAJ100205275

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allfields	10.1038/s41467-023-43916-6 doi (DE-627)DOAJ100205275 (DE-599)DOAJ9ef9717b0d834ebc90f989b7b7574f06 DE-627 ger DE-627 rakwb eng Hongzheng Dong verfasserin aut Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage. Science Q Xiangyu Pan verfasserin aut Yuancai Gong verfasserin aut Mengfan Xue verfasserin aut Pin Wang verfasserin aut SocMan Ho-Kimura verfasserin aut Yingfang Yao verfasserin aut Hao Xin verfasserin aut Wenjun Luo verfasserin aut Zhigang Zou verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 9 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:9 https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 kostenfrei https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 9
spelling	10.1038/s41467-023-43916-6 doi (DE-627)DOAJ100205275 (DE-599)DOAJ9ef9717b0d834ebc90f989b7b7574f06 DE-627 ger DE-627 rakwb eng Hongzheng Dong verfasserin aut Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage. Science Q Xiangyu Pan verfasserin aut Yuancai Gong verfasserin aut Mengfan Xue verfasserin aut Pin Wang verfasserin aut SocMan Ho-Kimura verfasserin aut Yingfang Yao verfasserin aut Hao Xin verfasserin aut Wenjun Luo verfasserin aut Zhigang Zou verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 9 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:9 https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 kostenfrei https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 9
allfields_unstemmed	10.1038/s41467-023-43916-6 doi (DE-627)DOAJ100205275 (DE-599)DOAJ9ef9717b0d834ebc90f989b7b7574f06 DE-627 ger DE-627 rakwb eng Hongzheng Dong verfasserin aut Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage. Science Q Xiangyu Pan verfasserin aut Yuancai Gong verfasserin aut Mengfan Xue verfasserin aut Pin Wang verfasserin aut SocMan Ho-Kimura verfasserin aut Yingfang Yao verfasserin aut Hao Xin verfasserin aut Wenjun Luo verfasserin aut Zhigang Zou verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 9 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:9 https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 kostenfrei https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 9
allfieldsGer	10.1038/s41467-023-43916-6 doi (DE-627)DOAJ100205275 (DE-599)DOAJ9ef9717b0d834ebc90f989b7b7574f06 DE-627 ger DE-627 rakwb eng Hongzheng Dong verfasserin aut Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage. Science Q Xiangyu Pan verfasserin aut Yuancai Gong verfasserin aut Mengfan Xue verfasserin aut Pin Wang verfasserin aut SocMan Ho-Kimura verfasserin aut Yingfang Yao verfasserin aut Hao Xin verfasserin aut Wenjun Luo verfasserin aut Zhigang Zou verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 9 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:9 https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 kostenfrei https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 9
allfieldsSound	10.1038/s41467-023-43916-6 doi (DE-627)DOAJ100205275 (DE-599)DOAJ9ef9717b0d834ebc90f989b7b7574f06 DE-627 ger DE-627 rakwb eng Hongzheng Dong verfasserin aut Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage. Science Q Xiangyu Pan verfasserin aut Yuancai Gong verfasserin aut Mengfan Xue verfasserin aut Pin Wang verfasserin aut SocMan Ho-Kimura verfasserin aut Yingfang Yao verfasserin aut Hao Xin verfasserin aut Wenjun Luo verfasserin aut Zhigang Zou verfasserin aut In Nature Communications Nature Portfolio, 2016 14(2023), 1, Seite 9 (DE-627)626457688 (DE-600)2553671-0 20411723 nnns volume:14 year:2023 number:1 pages:9 https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 kostenfrei https://doi.org/10.1038/s41467-023-43916-6 kostenfrei https://doaj.org/toc/2041-1723 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_211 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_2110 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2023 1 9
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author	Hongzheng Dong
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title	Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis
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title_sort	potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis
title_auth	Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis
abstract	Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage.
abstractGer	Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage.
abstract_unstemmed	Abstract In the past decades, a band alignment theory has become a basis for designing different high-performance semiconductor devices, such as photocatalysis, photoelectrocatalysis, photoelectrostorage and third-generation photovoltaics. Recently, a faradaic junction model (coupled electron and ion transfer) has been proposed to explain charge transfer phenomena in these semiconductor heterojunctions. However, the classic band alignment theory cannot explain coupled electron and ion transfer processes because it only regulates electron transfer. Therefore, it is very significant to explore a suitable design concept for regulating coupled electron and ion transfer in order to improve the performance of semiconductor heterojunctions. Herein, we propose a potential window alignment theory for regulating ion transfer and remarkably improving the photoelectrocatalytic performance of a MoS2/Cd-Cu2ZnSnS4 heterojunction photocathode. Moreover, we find that a faradaic potential window, rather than the band position of the intermediate layer, is a criterion for identifying interface charge transfer direction. This finding can offer different perspectives for designing high-performance semiconductor heterojunctions with suitable potential windows for solar energy conversion and storage.
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title_short	Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis
url	https://doi.org/10.1038/s41467-023-43916-6 https://doaj.org/article/9ef9717b0d834ebc90f989b7b7574f06 https://doaj.org/toc/2041-1723
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Potential window alignment regulating ion transfer in faradaic junctions for efficient photoelectrocatalysis

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