Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries

Lithium iron phosphate (LiFePO<sub<4</sub<, LFP), an olivine–type cathode material, represents a highly suitable cathode option for lithium–ion batteries that is widely applied in electric vehicles and renewable energy storage systems. This work employed the ball milling technique to syn...
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Autor*in:	Xiukun Jiang [verfasserIn] Yan Xin [verfasserIn] Bijiao He [verfasserIn] Fang Zhang [verfasserIn] Huajun Tian [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2024

Schlagwörter:	LiFePO lithium–ion batteries cathode heteroatom doping electrochemical performance

Übergeordnetes Werk:	In: Materials - MDPI AG, 2009, 17(2024), 6, p 1299
Übergeordnetes Werk:	volume:17 ; year:2024 ; number:6, p 1299

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/ma17061299

Katalog-ID:	DOAJ10047120X

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callnumber-first	T - Technology
author	Xiukun Jiang
spellingShingle	Xiukun Jiang misc TK1-9971 misc TA1-2040 misc QH201-278.5 misc QC120-168.85 misc LiFePO<sub<4</sub< misc lithium–ion batteries misc cathode misc heteroatom doping misc electrochemical performance misc Technology misc T misc Electrical engineering. Electronics. Nuclear engineering misc Engineering (General). Civil engineering (General) misc Microscopy misc Descriptive and experimental mechanics Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries
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topic_title	TK1-9971 TA1-2040 QH201-278.5 QC120-168.85 Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries LiFePO<sub<4</sub< lithium–ion batteries cathode heteroatom doping electrochemical performance
topic	misc TK1-9971 misc TA1-2040 misc QH201-278.5 misc QC120-168.85 misc LiFePO<sub<4</sub< misc lithium–ion batteries misc cathode misc heteroatom doping misc electrochemical performance misc Technology misc T misc Electrical engineering. Electronics. Nuclear engineering misc Engineering (General). Civil engineering (General) misc Microscopy misc Descriptive and experimental mechanics
topic_unstemmed	misc TK1-9971 misc TA1-2040 misc QH201-278.5 misc QC120-168.85 misc LiFePO<sub<4</sub< misc lithium–ion batteries misc cathode misc heteroatom doping misc electrochemical performance misc Technology misc T misc Electrical engineering. Electronics. Nuclear engineering misc Engineering (General). Civil engineering (General) misc Microscopy misc Descriptive and experimental mechanics
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title	Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries
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title_full	Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries
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title_sort	effect of heteroatom doping on electrochemical properties of olivine lifepo<sub<4</sub< cathodes for high-performance lithium-ion batteries
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title_auth	Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries
abstract	Lithium iron phosphate (LiFePO<sub<4</sub<, LFP), an olivine–type cathode material, represents a highly suitable cathode option for lithium–ion batteries that is widely applied in electric vehicles and renewable energy storage systems. This work employed the ball milling technique to synthesize LiFePO<sub<4</sub</carbon (LFP/C) composites and investigated the effects of various doping elements, including F, Mn, Nb, and Mg, on the electrochemical behavior of LFP/C composite cathodes. Our comprehensive work indicates that optimized F doping could improve the discharge capacity of the LFP/C composites at high rates, achieving 113.7 mAh g<sup<−1</sup< at 10 C. Rational Nb doping boosted the cycling stability and improved the capacity retention rate (above 96.1% after 100 cycles at 0.2 C). The designed Mn doping escalated the discharge capacity of the LFP/C composite under a low temperature of −15 °C (101.2 mAh g<sup<−1</sup< at 0.2 C). By optimizing the doping elements and levels, the role of doping as a modification method on the diverse properties of LFP/C cathode materials was effectively explored.
abstractGer	Lithium iron phosphate (LiFePO<sub<4</sub<, LFP), an olivine–type cathode material, represents a highly suitable cathode option for lithium–ion batteries that is widely applied in electric vehicles and renewable energy storage systems. This work employed the ball milling technique to synthesize LiFePO<sub<4</sub</carbon (LFP/C) composites and investigated the effects of various doping elements, including F, Mn, Nb, and Mg, on the electrochemical behavior of LFP/C composite cathodes. Our comprehensive work indicates that optimized F doping could improve the discharge capacity of the LFP/C composites at high rates, achieving 113.7 mAh g<sup<−1</sup< at 10 C. Rational Nb doping boosted the cycling stability and improved the capacity retention rate (above 96.1% after 100 cycles at 0.2 C). The designed Mn doping escalated the discharge capacity of the LFP/C composite under a low temperature of −15 °C (101.2 mAh g<sup<−1</sup< at 0.2 C). By optimizing the doping elements and levels, the role of doping as a modification method on the diverse properties of LFP/C cathode materials was effectively explored.
abstract_unstemmed	Lithium iron phosphate (LiFePO<sub<4</sub<, LFP), an olivine–type cathode material, represents a highly suitable cathode option for lithium–ion batteries that is widely applied in electric vehicles and renewable energy storage systems. This work employed the ball milling technique to synthesize LiFePO<sub<4</sub</carbon (LFP/C) composites and investigated the effects of various doping elements, including F, Mn, Nb, and Mg, on the electrochemical behavior of LFP/C composite cathodes. Our comprehensive work indicates that optimized F doping could improve the discharge capacity of the LFP/C composites at high rates, achieving 113.7 mAh g<sup<−1</sup< at 10 C. Rational Nb doping boosted the cycling stability and improved the capacity retention rate (above 96.1% after 100 cycles at 0.2 C). The designed Mn doping escalated the discharge capacity of the LFP/C composite under a low temperature of −15 °C (101.2 mAh g<sup<−1</sup< at 0.2 C). By optimizing the doping elements and levels, the role of doping as a modification method on the diverse properties of LFP/C cathode materials was effectively explored.
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container_issue	6, p 1299
title_short	Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries
url	https://doi.org/10.3390/ma17061299 https://doaj.org/article/7db6e60b3d2a43d68d34e953537d5771 https://www.mdpi.com/1996-1944/17/6/1299 https://doaj.org/toc/1996-1944
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up_date	2024-07-03T14:51:58.060Z
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Effect of Heteroatom Doping on Electrochemical Properties of Olivine LiFePO<sub<4</sub< Cathodes for High-Performance Lithium-Ion Batteries

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