One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation

The development of high-entropy anodes, known for their excellent catalytic activity for water oxidation, can depress the energy consumption of hydrogen production by water electrolysis. However, the complex preparation methods and poor stability hindered their practical application. In this work, a...
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Autor*in:	Jianlei Jing [verfasserIn] Wei Liu [verfasserIn] Tianshui Li [verfasserIn] Xiaoqian Ding [verfasserIn] Wenhai Xu [verfasserIn] Mengze Ma [verfasserIn] Daojin Zhou [verfasserIn] Yaping Li [verfasserIn] Xiaoming Sun [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2024

Schlagwörter:	high entropy layered double hydroxides oxygen evolution reaction

Übergeordnetes Werk:	In: Catalysts - MDPI AG, 2012, 14(2024), 3, p 171
Übergeordnetes Werk:	volume:14 ; year:2024 ; number:3, p 171

Links:	Link aufrufen Link aufrufen Link aufrufen Journal toc

DOI / URN:	10.3390/catal14030171

Katalog-ID:	DOAJ10053595X

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allfieldsSound	10.3390/catal14030171 doi (DE-627)DOAJ10053595X (DE-599)DOAJ215e1111b76749b3a241dcbfde12ce2e DE-627 ger DE-627 rakwb eng TP1-1185 QD1-999 Jianlei Jing verfasserin aut One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of high-entropy anodes, known for their excellent catalytic activity for water oxidation, can depress the energy consumption of hydrogen production by water electrolysis. However, the complex preparation methods and poor stability hindered their practical application. In this work, a one-step co-precipitation method has been modified to rapidly synthesize ultrathin high-entropy layered double hydroxide containing Ni, Co, Fe, Cr, Zn. Through the rational selection of metal elements, the stability of the optimized anode under Ampere-level current density has been significantly improved. Compared to NiFe-LDH, the active site leaching of high-entropy LDH is reduced by 42.7%, and as a result, it achieves a performance decay that is approximately eight times lower than that of NiFe-LDH. Experiment results show that the active sites in the high-entropy LDH can maintain a relatively low oxidation state both before and after activation, thus preventing material deactivation caused by excessive oxidation. high entropy layered double hydroxides oxygen evolution reaction Chemical technology Chemistry Wei Liu verfasserin aut Tianshui Li verfasserin aut Xiaoqian Ding verfasserin aut Wenhai Xu verfasserin aut Mengze Ma verfasserin aut Daojin Zhou verfasserin aut Yaping Li verfasserin aut Xiaoming Sun verfasserin aut In Catalysts MDPI AG, 2012 14(2024), 3, p 171 (DE-627)71862646X (DE-600)2662126-5 20734344 nnns volume:14 year:2024 number:3, p 171 https://doi.org/10.3390/catal14030171 kostenfrei https://doaj.org/article/215e1111b76749b3a241dcbfde12ce2e kostenfrei https://www.mdpi.com/2073-4344/14/3/171 kostenfrei https://doaj.org/toc/2073-4344 Journal toc kostenfrei GBV_USEFLAG_A SYSFLAG_A GBV_DOAJ GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 14 2024 3, p 171
language	English
source	In Catalysts 14(2024), 3, p 171 volume:14 year:2024 number:3, p 171
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callnumber-first	T - Technology
author	Jianlei Jing
spellingShingle	Jianlei Jing misc TP1-1185 misc QD1-999 misc high entropy misc layered double hydroxides misc oxygen evolution reaction misc Chemical technology misc Chemistry One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation
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topic_title	TP1-1185 QD1-999 One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation high entropy layered double hydroxides oxygen evolution reaction
topic	misc TP1-1185 misc QD1-999 misc high entropy misc layered double hydroxides misc oxygen evolution reaction misc Chemical technology misc Chemistry
topic_unstemmed	misc TP1-1185 misc QD1-999 misc high entropy misc layered double hydroxides misc oxygen evolution reaction misc Chemical technology misc Chemistry
topic_browse	misc TP1-1185 misc QD1-999 misc high entropy misc layered double hydroxides misc oxygen evolution reaction misc Chemical technology misc Chemistry
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title	One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation
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title_full	One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation
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author_browse	Jianlei Jing Wei Liu Tianshui Li Xiaoqian Ding Wenhai Xu Mengze Ma Daojin Zhou Yaping Li Xiaoming Sun
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title_sort	one-step synthesis of ultrathin high-entropy layered double hydroxides for ampere-level water oxidation
callnumber	TP1-1185
title_auth	One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation
abstract	The development of high-entropy anodes, known for their excellent catalytic activity for water oxidation, can depress the energy consumption of hydrogen production by water electrolysis. However, the complex preparation methods and poor stability hindered their practical application. In this work, a one-step co-precipitation method has been modified to rapidly synthesize ultrathin high-entropy layered double hydroxide containing Ni, Co, Fe, Cr, Zn. Through the rational selection of metal elements, the stability of the optimized anode under Ampere-level current density has been significantly improved. Compared to NiFe-LDH, the active site leaching of high-entropy LDH is reduced by 42.7%, and as a result, it achieves a performance decay that is approximately eight times lower than that of NiFe-LDH. Experiment results show that the active sites in the high-entropy LDH can maintain a relatively low oxidation state both before and after activation, thus preventing material deactivation caused by excessive oxidation.
abstractGer	The development of high-entropy anodes, known for their excellent catalytic activity for water oxidation, can depress the energy consumption of hydrogen production by water electrolysis. However, the complex preparation methods and poor stability hindered their practical application. In this work, a one-step co-precipitation method has been modified to rapidly synthesize ultrathin high-entropy layered double hydroxide containing Ni, Co, Fe, Cr, Zn. Through the rational selection of metal elements, the stability of the optimized anode under Ampere-level current density has been significantly improved. Compared to NiFe-LDH, the active site leaching of high-entropy LDH is reduced by 42.7%, and as a result, it achieves a performance decay that is approximately eight times lower than that of NiFe-LDH. Experiment results show that the active sites in the high-entropy LDH can maintain a relatively low oxidation state both before and after activation, thus preventing material deactivation caused by excessive oxidation.
abstract_unstemmed	The development of high-entropy anodes, known for their excellent catalytic activity for water oxidation, can depress the energy consumption of hydrogen production by water electrolysis. However, the complex preparation methods and poor stability hindered their practical application. In this work, a one-step co-precipitation method has been modified to rapidly synthesize ultrathin high-entropy layered double hydroxide containing Ni, Co, Fe, Cr, Zn. Through the rational selection of metal elements, the stability of the optimized anode under Ampere-level current density has been significantly improved. Compared to NiFe-LDH, the active site leaching of high-entropy LDH is reduced by 42.7%, and as a result, it achieves a performance decay that is approximately eight times lower than that of NiFe-LDH. Experiment results show that the active sites in the high-entropy LDH can maintain a relatively low oxidation state both before and after activation, thus preventing material deactivation caused by excessive oxidation.
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container_issue	3, p 171
title_short	One-Step Synthesis of Ultrathin High-Entropy Layered Double Hydroxides for Ampere-Level Water Oxidation
url	https://doi.org/10.3390/catal14030171 https://doaj.org/article/215e1111b76749b3a241dcbfde12ce2e https://www.mdpi.com/2073-4344/14/3/171 https://doaj.org/toc/2073-4344
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