Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al
In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Rategarpanah, Ali [verfasserIn] Meshkani, Fereshteh [verfasserIn] Wang, Yuan [verfasserIn] Arandiyan, Hamidreza [verfasserIn] Rezaei, Mehran [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Energy conversion and management - Amsterdam [u.a.] : Elsevier Science, 1980, 166, Seite 268-280 |
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| Übergeordnetes Werk: |
volume:166 ; pages:268-280 |
| DOI / URN: |
10.1016/j.enconman.2018.04.033 |
|---|
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ELV001169602 |
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| 245 | 1 | 0 | |a Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al |
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| 520 | |a In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. | ||
| 650 | 4 | |a Thermocatalytic decomposition of methane | |
| 650 | 4 | |a Noble metals | |
| 650 | 4 | |a Copper | |
| 650 | 4 | |a Hydrogen | |
| 650 | 4 | |a Nickel catalysts | |
| 700 | 1 | |a Meshkani, Fereshteh |e verfasserin |0 (orcid)0000-0001-5836-4841 |4 aut | |
| 700 | 1 | |a Wang, Yuan |e verfasserin |4 aut | |
| 700 | 1 | |a Arandiyan, Hamidreza |e verfasserin |4 aut | |
| 700 | 1 | |a Rezaei, Mehran |e verfasserin |4 aut | |
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10.1016/j.enconman.2018.04.033 doi (DE-627)ELV001169602 (ELSEVIER)S0196-8904(18)30369-8 DE-627 ger DE-627 rda eng 620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Rategarpanah, Ali verfasserin aut Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts Meshkani, Fereshteh verfasserin (orcid)0000-0001-5836-4841 aut Wang, Yuan verfasserin aut Arandiyan, Hamidreza verfasserin aut Rezaei, Mehran verfasserin aut Enthalten in Energy conversion and management Amsterdam [u.a.] : Elsevier Science, 1980 166, Seite 268-280 Online-Ressource (DE-627)320407659 (DE-600)2000891-0 (DE-576)12088352X nnns volume:166 pages:268-280 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 50.70 Energie: Allgemeines 83.65 Versorgungswirtschaft 52.57 Energiespeicherung 52.56 Regenerative Energieformen alternative Energieformen AR 166 268-280 |
| spelling |
10.1016/j.enconman.2018.04.033 doi (DE-627)ELV001169602 (ELSEVIER)S0196-8904(18)30369-8 DE-627 ger DE-627 rda eng 620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Rategarpanah, Ali verfasserin aut Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts Meshkani, Fereshteh verfasserin (orcid)0000-0001-5836-4841 aut Wang, Yuan verfasserin aut Arandiyan, Hamidreza verfasserin aut Rezaei, Mehran verfasserin aut Enthalten in Energy conversion and management Amsterdam [u.a.] : Elsevier Science, 1980 166, Seite 268-280 Online-Ressource (DE-627)320407659 (DE-600)2000891-0 (DE-576)12088352X nnns volume:166 pages:268-280 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 50.70 Energie: Allgemeines 83.65 Versorgungswirtschaft 52.57 Energiespeicherung 52.56 Regenerative Energieformen alternative Energieformen AR 166 268-280 |
| allfields_unstemmed |
10.1016/j.enconman.2018.04.033 doi (DE-627)ELV001169602 (ELSEVIER)S0196-8904(18)30369-8 DE-627 ger DE-627 rda eng 620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Rategarpanah, Ali verfasserin aut Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts Meshkani, Fereshteh verfasserin (orcid)0000-0001-5836-4841 aut Wang, Yuan verfasserin aut Arandiyan, Hamidreza verfasserin aut Rezaei, Mehran verfasserin aut Enthalten in Energy conversion and management Amsterdam [u.a.] : Elsevier Science, 1980 166, Seite 268-280 Online-Ressource (DE-627)320407659 (DE-600)2000891-0 (DE-576)12088352X nnns volume:166 pages:268-280 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 50.70 Energie: Allgemeines 83.65 Versorgungswirtschaft 52.57 Energiespeicherung 52.56 Regenerative Energieformen alternative Energieformen AR 166 268-280 |
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10.1016/j.enconman.2018.04.033 doi (DE-627)ELV001169602 (ELSEVIER)S0196-8904(18)30369-8 DE-627 ger DE-627 rda eng 620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Rategarpanah, Ali verfasserin aut Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts Meshkani, Fereshteh verfasserin (orcid)0000-0001-5836-4841 aut Wang, Yuan verfasserin aut Arandiyan, Hamidreza verfasserin aut Rezaei, Mehran verfasserin aut Enthalten in Energy conversion and management Amsterdam [u.a.] : Elsevier Science, 1980 166, Seite 268-280 Online-Ressource (DE-627)320407659 (DE-600)2000891-0 (DE-576)12088352X nnns volume:166 pages:268-280 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 50.70 Energie: Allgemeines 83.65 Versorgungswirtschaft 52.57 Energiespeicherung 52.56 Regenerative Energieformen alternative Energieformen AR 166 268-280 |
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10.1016/j.enconman.2018.04.033 doi (DE-627)ELV001169602 (ELSEVIER)S0196-8904(18)30369-8 DE-627 ger DE-627 rda eng 620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Rategarpanah, Ali verfasserin aut Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts Meshkani, Fereshteh verfasserin (orcid)0000-0001-5836-4841 aut Wang, Yuan verfasserin aut Arandiyan, Hamidreza verfasserin aut Rezaei, Mehran verfasserin aut Enthalten in Energy conversion and management Amsterdam [u.a.] : Elsevier Science, 1980 166, Seite 268-280 Online-Ressource (DE-627)320407659 (DE-600)2000891-0 (DE-576)12088352X nnns volume:166 pages:268-280 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 50.70 Energie: Allgemeines 83.65 Versorgungswirtschaft 52.57 Energiespeicherung 52.56 Regenerative Energieformen alternative Energieformen AR 166 268-280 |
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Rategarpanah, Ali @@aut@@ Meshkani, Fereshteh @@aut@@ Wang, Yuan @@aut@@ Arandiyan, Hamidreza @@aut@@ Rezaei, Mehran @@aut@@ |
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Rategarpanah, Ali |
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620 DE-600 50.70 bkl 83.65 bkl 52.57 bkl 52.56 bkl Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al Thermocatalytic decomposition of methane Noble metals Copper Hydrogen Nickel catalysts |
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Rategarpanah, Ali Meshkani, Fereshteh Wang, Yuan Arandiyan, Hamidreza Rezaei, Mehran |
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thermocatalytic conversion of methane to highly pure hydrogen over ni–cu/mgo·al |
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Thermocatalytic conversion of methane to highly pure hydrogen over Ni–Cu/MgO·Al |
| abstract |
In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. |
| abstractGer |
In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. |
| abstract_unstemmed |
In this article, the synthesis, characterization and catalytic performance of the Pd and Pt promoted Ni-Cu/MgO·Al2O3 catalysts were investigated in the thermocatalytic dehydrogenation of methane to highly pure hydrogen. The physicochemical properties of the prepared catalysts were investigated using different characterization methods such as XRD, BET, SEM, TEM, XPS, H2-TPR and TPO techniques. The Ni–Cu/MgO·Al2O3 catalyst possessing mesoporous structure and large BET surface area (126.28 m2 g−1) was successfully synthesized by facile simultaneous sol-gel method (SSGM) in the absence of surfactants. The results showed that the addition of Pd significantly improved the catalytic activity and stability. The effect of different nominal loadings of palladium (2, 4 and 6 wt%) on the catalytic performance was also studied. Among the prepared samples, the promoted sample with 4 wt% of palladium showed optimal catalytic performance and stability at higher temperatures towards methane thermocatalytic decomposition. |
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Meshkani, Fereshteh Wang, Yuan Arandiyan, Hamidreza Rezaei, Mehran |
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